79 research outputs found

    Two-dimensional organization of a large number of stationary optical filaments by adaptive wave front control

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    We present an adaptive technique for the formation of multiple co-propagating and stationary filaments in a gaseous medium. Wavefront shaping of the initial beam is performed using a deformable mirror to achieve a complete two-dimensional control of the multi-spot intensity pattern in the laser focus. The spatial organization of these intensity spots yields reliable formation of up to five stable and stationary filaments providing a test bed for fundamental studies on multiple filamentatio

    Quasiparticles dynamics in high-temperature superconductors far from equilibrium: an indication of pairing amplitude without phase coherence

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    We perform time resolved photoelectron spectroscopy measurements of optimally doped \tn{Bi}_2\tn{Sr}_2\tn{CaCu}_2\tn{O}_{8+\delta} (Bi-2212) and \tn{Bi}_2\tn{Sr}_{2-x}\tn{La}_{x}\tn{Cu}\tn{O}_{6+\delta} (Bi-2201). The electrons dynamics show that inelastic scattering by nodal quasiparticles decreases when the temperature is lowered below the critical value of the superconducting phase transition. This drop of electronic dissipation is astonishingly robust and survives to photoexcitation densities much larger than the value sustained by long-range superconductivity. The unconventional behaviour of quasiparticle scattering is ascribed to superconducting correlations extending on a length scale comparable to the inelastic path. Our measurements indicate that strongly driven superconductors enter in a regime without phase coherence but finite pairing amplitude. The latter vanishes near to the critical temperature and has no evident link with the pseudogap observed by Angle Resolved Photoelectron Spectroscopy (ARPES).Comment: 7 pages, 5 Figure

    Angle-resolved photoemission study of the role of nesting and orbital orderings in the antiferromagnetic phase of BaFe2As2

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    We present a detailed comparison of the electronic structure of BaFe2As2 in its paramagnetic and antiferromagnetic (AFM) phases, through angle-resolved photoemission studies. Using different experimental geometries, we resolve the full elliptic shape of the electron pockets, including parts of dxy symmetry along its major axis that are usually missing. This allows us to define precisely how the hole and electron pockets are nested and how the different orbitals evolve at the transition. We conclude that the imperfect nesting between hole and electron pockets explains rather well the formation of gaps and residual metallic droplets in the AFM phase, provided the relative parity of the different bands is taken into account. Beyond this nesting picture, we observe shifts and splittings of numerous bands at the transition. We show that the splittings are surface sensitive and probably not a reliable signature of the magnetic order. On the other hand, the shifts indicate a significant redistribution of the orbital occupations at the transition, especially within the dxz/dyz system, which we discuss

    Surface effects on the Mott-Hubbard transition in archetypal V2_2O3_3

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    We present an experimental and theoretical study exploring surface effects on the evolution of the metal-insulator transition in the model Mott-Hubbard compound Cr-doped V2_2O3_3. We find a microscopic domain formation that is clearly affected by the surface crystallographic orientation. Using scanning photoelectron microscopy and X-ray diffraction, we find that surface defects act as nucleation centers for the formation of domains at the temperature-induced isostructural transition and favor the formation of microscopic metallic regions. A density functional theory plus dynamical mean field theory study of different surface terminations shows that the surface reconstruction with excess vanadyl cations leads to doped, and hence more metallic surface states, explaining our experimental observations.Comment: 5 pages, 4 figure

    Giant Anisotropy of Spin-Orbit Splitting at the Bismuth Surface

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    We investigate the bismuth (111) surface by means of time and angle resolved photoelectron spectroscopy. The parallel detection of the surface states below and above the Fermi level reveals a giant anisotropy of the Spin-Orbit (SO) spitting. These strong deviations from the Rashba-like coupling cannot be treated in kp\textbf{k}\cdot \textbf{p} perturbation theory. Instead, first principle calculations could accurately reproduce the experimental dispersion of the electronic states. Our analysis shows that the giant anisotropy of the SO splitting is due to a large out-of plane buckling of the spin and orbital texture.Comment: 5 pages, 4 figure

    Ultrafast filling of an electronic pseudogap in an incommensurate crystal

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    We investigate the quasiperiodic crystal (LaS)1.196(VS2) by angle and time resolved photoemission spectroscopy. The dispersion of electronic states is in qualitative agreement with band structure calculated for the VS2 slab without the incommensurate distortion. Nonetheless, the spectra display a temperature dependent pseudogap instead of quasiparticles crossing. The sudden photoexcitation at 50 K induces a partial filling of the electronic pseudogap within less than 80 fs. The electronic energy flows into the lattice modes on a comparable timescale. We attribute this surprisingly short timescale to a very strong electron-phonon coupling to the incommensurate distortion. This result sheds light on the electronic localization arising in aperiodic structures and quasicrystals

    Stacking, correlations and electronic dispersion in the photoexcited state of 1T-TaS<sub>2</sub>

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    Here we perform angle and time-resolved photoelectron spectroscopy on the commensurate Charge Density Wave phase of 1T-TaS2. Data with different probe pulse polarization are employed to map the dispersion of electronic states below or above the chemical potential. The experimental results are compared to Density-Functional Theory calculations with a self-consistent evaluation of the coulomb repulsion. Both out-of-plane dimerization and electronic correlations must be included in order to obtain good agreement with the experimental data. Upon Photoexcitation, the fluctuations of CDW order erase the band dispersion near to the chemical potential and halve the charge gap size. This transient phase sets within half a period of the coherent lattice motion and is likely favored by strong electronic correlations
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