213 research outputs found
The electronic structure of LaSrMnO thin films and its dependence as studied by angle-resolved photoemission
We present angle-resolved photoemission spectroscopy results for thin films
of the three-dimensional manganese perovskite LaSrMnO. We
show that the transition temperature () from the paramagnetic insulating
to ferromagnetic metallic state is closely related to details of the electronic
structure, particularly to the spectral weight at the -point, where
the sharpest step at the Fermi level was observed. We found that this -point is the same for all the samples, despite their different . The
change of is discussed in terms of kinetic energy optimization. Our ARPES
results suggest that the change of the electronic structure for the samples
having different transition temperatures is different from the rigid band
shift.Comment: Accepted by Journal of Physics: Condensed Matte
Fermi surface of the colossal magnetoresistance perovskite La_{0.7}Sr_{0.3}MnO_{3}
Materials that exhibit colossal magnetoresistance (CMR) are currently the
focus of an intense research effort, driven by the technological applications
that their sensitivity lends them to. Using the angular correlation of photons
from electron-positron annihilation, we present a first glimpse of the Fermi
surface of a material that exhibits CMR, supported by ``virtual crystal''
electronic structure calculations. The Fermi surface is shown to be
sufficiently cubic in nature that it is likely to support nesting.Comment: 5 pages, 5 PS figure
Ab-initio electronic and magnetic structure in La_0.66Sr_0.33MnO_3: strain and correlation effects
The effects of tetragonal strain on electronic and magnetic properties of
strontium-doped lanthanum manganite, La_{2/3}Sr_{1/3}MnO_3 (LSMO), are
investigated by means of density-functional methods. As far as the structural
properties are concerned, the comparison between theory and experiments for
LSMO strained on the most commonly used substrates, shows an overall good
agreement: the slight overestimate (at most of 1-1.5 %) for the equilibrium
out-of-plane lattice constants points to possible defects in real samples. The
inclusion of a Hubbard-like contribution on the Mn d states, according to the
so-called "LSDA+U" approach, is rather ineffective from the structural point of
view, but much more important from the electronic and magnetic point of view.
In particular, full half-metallicity, which is missed within a bare
density-functional approach, is recovered within LSDA+U, in agreement with
experiments. Moreover, the half-metallic behavior, particularly relevant for
spin-injection purposes, is independent on the chosen substrate and is achieved
for all the considered in-plane lattice constants. More generally, strain
effects are not seen to crucially affect the electronic structure: within the
considered tetragonalization range, the minority gap is only slightly (i.e. by
about 0.1-0.2 eV) affected by a tensile or compressive strain. Nevertheless, we
show that the growth on a smaller in-plane lattice constant can stabilize the
out-of-plane vs in-plane e_g orbital and significatively change their relative
occupancy. Since e_g orbitals are key quantities for the double-exchange
mechanism, strain effects are confirmed to be crucial for the resulting
magnetic coupling.Comment: 16 pages, 7 figures, to be published on J. Phys.: Condensed Matte
Spin Wave Theory of Double Exchange Ferromagnets
We construct the 1/S spin-wave expansion for double exchange ferromagnets at
T=0. It is assumed that the value of Hund's rule coupling, J_H, is sufficiently
large, resulting in a fully saturated, ferromagnetic half-metallic ground
state. We evaluate corrections to the magnon dispersion law, and we also find
that, in contrast to earlier statements in the literature, magnon-electron
scattering does give rise to spin wave damping. We analyse the momentum
dependence of these quantities and discuss the experimental implications for
colossal magnetoresistance compounds.Comment: 4 pages, Latex-Revtex, 2 PostScript figures. Minor revisions,
references added. See also cond-mat/990921
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