107 research outputs found
Electron doping evolution of the magnetic excitations in BaFe2-xNixAs2
We use inelastic neutron scattering (INS) spectroscopy to study the magnetic
excitations spectra throughout the Brioullion zone in electron-doped iron
pnictide superconductors BaFeNiAs with .
While the sample is near optimal superconductivity with K
and has coexisting static incommensurate magnetic order, the
samples are electron-overdoped with reduced of 14 K and 8 K,
respectively, and have no static antiferromagnetic (AF) order. In previous INS
work on undoped () and electron optimally doped () samples, the
effect of electron-doping was found to modify spin waves in the parent compound
BaFeAs below 100 meV and induce a neutron spin resonance at the
commensurate AF ordering wave vector that couples with superconductivity. While
the new data collected on the sample confirms the overall features of
the earlier work, our careful temperature dependent study of the resonance
reveals that the resonance suddenly changes its -width below similar
to that of the optimally hole-doped iron pnictides
BaKFeAs. In addition, we establish the dispersion of
the resonance and find it to change from commensurate to transversely
incommensurate with increasing energy. Upon further electron-doping to
overdoped iron pnictides with and 0.18, the resonance becomes weaker
and transversely incommensurate at all energies, while spin excitations above
100 meV are still not much affected. Our absolute spin excitation
intensity measurements throughout the Brillouin zone for
confirm the notion that the low-energy spin excitation coupling with itinerant
electron is important for superconductivity in these materials, even though the
high-energy spin excitations are weakly doping dependent.Comment: 16 pages, 16 figure
Neutron scattering and scaling behavior in URu2Zn20 and YbFe2Zn20
The dynamic susceptibility chi"(deltaE), measured by inelastic neutron
scattering measurements, shows a broad peak centered at Emax = 16.5 meV for the
cubic actinide compound URu2Zn20 and 7 meV at the (1/2, 1/2, 1/2) zone boundary
for the rare earth counterpart compound YbFe2Zn20. For URu2Zn20, the low
temperature susceptibility and magnetic specific heat coefficient gamma =
Cmag/T take the values chi = 0.011 emu/mole and gamma = 190 mJ/mole-K2 at T = 2
K. These values are roughly three times smaller, and Emax is three times
larger, than recently reported for the related compound UCo2Zn20, so that chi
and gamma scale inversely with the characteristic energy for spin fluctuations,
Tsf = Emax/kB. While chi(T), Cmag(T), and Emax of the 4f compound YbFe2Zn20 are
very well described by the Kondo impurity model, we show that the model works
poorly for URu2Zn20 and UCo2Zn20, suggesting that the scaling behavior of the
actinide compounds arises from spin fluctuations of itinerant 5f electrons.Comment: 7 pages, 5 figure
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