Semiconductor-metal nanoparticle molecules: hybrid excitons and non-linear Fano effect

Modern nanotechnology opens the possibility of combining nanocrystals of various materials with very different characteristics in one superstructure. The resultant superstructure may provide new physical properties not encountered in homogeneous systems. Here we study theoretically the optical properties of hybrid molecules composed of semiconductor and metal nanoparticles. Excitons and plasmons in such a hybrid molecule become strongly coupled and demonstrate novel properties. At low incident light intensity, the exciton peak in the absorption spectrum is broadened and shifted due to incoherent and coherent interactions between metal and semiconductor nanoparticles. At high light intensity, the absorption spectrum demonstrates a surprising, strongly asymmetric shape. This shape originates from the coherent inter-nanoparticle Coulomb interaction and can be viewed as a non-linear Fano effect which is quite different from the usual linear Fano resonance.Comment: 5 pages, 5 figures, submitted to Phys. Rev. Let

Giant Modal Gain, Amplified Surface Plasmon Polariton Propagation, and Slowing Down of Energy Velocity in a Metal-Semiconductor-Metal Structure

We investigated surface plasmon polariton (SPP) propagation in a metal-semiconductor-metal structure where semiconductor is highly excited to have optical gain. We show that near the SPP resonance, the imaginary part of the propagation wavevector changes from positive to hugely negative, corresponding to an amplified SPP propagation. The SPP experiences a giant gain that is 1000 times of material gain in the excited semiconductor. We show that such a giant gain is related to the slowing down of average energy propagation in the structur

Direct Measurement of intermediate-range Casimir-Polder potentials

We present the first direct measurements of Casimir-Polder forces between solid surfaces and atomic gases in the transition regime between the electrostatic short-distance and the retarded long-distance limit. The experimental method is based on ultracold ground-state Rb atoms that are reflected from evanescent wave barriers at the surface of a dielectric glass prism. Our novel approach does not require assumptions about the potential shape. The experimental data confirm the theoretical prediction in the transition regime.Comment: 4 pages, 3 figure

One-electron states and interband optical absorption in single-wall carbon nanotubes

Explicit expressions for the wave functions and dispersion equation for the band p - electrons in single-wall carbon nanotubes are obtained within the method of zero-range potentials. They are then used to investigate the absorption spectrum of polarized light caused by direct interband transitions in isolated nanotubes. It is shown that, at least, under the above approximations, the circular dichroism is absent in chiral nanotubes for the light wave propagating along the tube axis. The results obtained are compared with those calculated in a similar way for a graphite plane.Comment: 16 pages, 8 figures, 1 tabl

Phase-change chalcogenide glass metamaterial

Combining metamaterials with functional media brings a new dimension to their performance. Here we demonstrate substantial resonance frequency tuning in a photonic metamaterial hybridized with an electrically/optically switchable chalcogenide glass. The transition between amorphous and crystalline forms brings about a 10% shift in the near-infrared resonance wavelength of an asymmetric split-ring array, providing transmission modulation functionality with a contrast ratio of 4:1 in a device of sub-wavelength thickness.Comment: 3 pages, 3 figure

Optical detection of spin transport in non-magnetic metals

We determine the dynamic magnetization induced in non-magnetic metal wedges composed of silver, copper and platinum by means of Brillouin light scattering (BLS) microscopy. The magnetization is transferred from a ferromagnetic Ni80Fe20 layer to the metal wedge via the spin pumping effect. The spin pumping efficiency can be controlled by adding an insulating but transparent interlayer between the magnetic and non-magnetic layer. By comparing the experimental results to a dynamical macroscopic spin-transport model we determine the transverse relaxation time of the pumped spin current which is much smaller than the longitudinal relaxation time

Exact microscopic theory of electromagnetic heat transfer between a dielectric sphere and plate

Near-field electromagnetic heat transfer holds great potential for the advancement of nanotechnology. Whereas far-field electromagnetic heat transfer is constrained by Planck's blackbody limit, the increased density of states in the near-field enhances heat transfer rates by orders of magnitude relative to the conventional limit. Such enhancement opens new possibilities in numerous applications, including thermal-photo-voltaics, nano-patterning, and imaging. The advancement in this area, however, has been hampered by the lack of rigorous theoretical treatment, especially for geometries that are of direct experimental relevance. Here we introduce an efficient computational strategy, and present the first rigorous calculation of electromagnetic heat transfer in a sphere-plate geometry, the only geometry where transfer rate beyond blackbody limit has been quantitatively probed at room temperature. Our approach results in a definitive picture unifying various approximations previously used to treat this problem, and provides new physical insights for designing experiments aiming to explore enhanced thermal transfer.Comment: 1 page title 8 page content 1 page references 2 page figure captions 4 page figure

Resonant absorption of electromagnetic fields by surface plasmons buried in a multilayered plasmonic nanostructure

Alastair P. Hibbins, W. Andrew Murray, J. Tyler, S. Wedge, William L. Barnes, and J. Roy Sambles, Physical Review B, Vol. 74, article 073408 (2006). "Copyright © 2006 by the American Physical Society."The optical reflectivity of a metal-dielectric-metal microcavity in which the upper layer is periodically perforated by narrow slits is explored. Complete characterization of the observed modes in terms of their resonant electromagnetic fields is achieved by comparison of the experimental data to the predictions of a finite-element model. In particular, we demonstrate that the slits provide efficient diffractive coupling to a surface plasmon mode buried within the microcavity whose propagation is strongly confined to the dielectric layer

Dual-tip-enhanced ultrafast CARS nanoscopy

Coherent anti-Stokes Raman scattering (CARS) and, in particular, femtosecond adaptive spectroscopic techniques (FAST CARS) have been successfully used for molecular spectroscopy and microscopic imaging. Recent progress in ultrafast nanooptics provides flexibility in generation and control of optical near fields, and holds promise to extend CARS techniques to the nanoscale. In this theoretical study, we demonstrate ultrafast subwavelentgh control of coherent Raman spectra of molecules in the vicinity of a plasmonic nanostructure excited by ultrashort laser pulses. The simulated nanostructure design provides localized excitation sources for CARS by focusing incident laser pulses into subwavelength hot spots via two self-similar nanolens antennas connected by a waveguide. Hot-spot-selective dual-tip-enhanced CARS (2TECARS) nanospectra of DNA nucleobases are obtained by simulating optimized pump, Stokes and probe near fields using tips, laser polarization- and pulse-shaping. This technique may be used to explore ultrafast energy and electron transfer dynamics in real space with nanometre resolution and to develop novel approaches to DNA sequencing.Comment: 11 pages, 6 figure

Casimir Force between a Dielectric Sphere and a Wall: A Model for Amplification of Vacuum Fluctuations

The interaction between a polarizable particle and a reflecting wall is examined. A macroscopic approach is adopted in which the averaged force is computed from the Maxwell stress tensor. The particular case of a perfectly reflecting wall and a sphere with a dielectric function given by the Drude model is examined in detail. It is found that the force can be expressed as the sum of a monotonically decaying function of position and of an oscillatory piece. At large separations, the oscillatory piece is the dominant contribution, and is much larger than the Casimir-Polder interaction that arises in the limit that the sphere is a perfect conductor. It is argued that this enhancement of the force can be interpreted in terms of the frequency spectrum of vacuum fluctuations. In the limit of a perfectly conducting sphere, there are cancellations between different parts of the spectrum which no longer occur as completely in the case of a sphere with frequency dependent polarizability. Estimates of the magnitude of the oscillatory component of the force suggest that it may be large enough to be observable.Comment: 18pp, LaTex, 7 figures, uses epsf. Several minor errors corrected, additional comments added in the final two sections, and references update