373 research outputs found
Electronic Raman scattering in correlated materials: exact treatment of nonresonant, mixed, and resonant scattering with dynamical mean field theory
We solve for the electronic Raman scattering response functions on an
infinite-dimensional hypercubic lattice employing dynamical mean field theory.
This contribution extends previous work on the nonresonant response to include
the mixed and resonant contributions. We focus our attention on the spinless
Falicov-Kimball model, where the problem can be solved exactly, and the system
can be tuned to go through a Mott-Hubbard-like metal-insulator transition.
Resonant effects vary in different scattering geometries, corresponding to the
symmetries of the charge excitations scattered by the light. We do find that
the Raman response is large near the double resonance, where the transfered
frequency is close to the incident photon frequency. We also find a joint
resonance of both the charge-transfer peak and the low-energy peak when the
incident photon frequency is on the order of the interaction strength. In
general, the resonance effects can create order of magnitude (or more)
enhancements of features in the nonresonant response, especially when the
incident photon frequency is somewhat larger than the frequency of the
nonresonant feature. Finally, we find that the resonant effects also exhibit
isosbestic behavior, even in the A1g and B2g sectors, and it is most prominent
when the incident photon frequency is on the order of the interaction energy.Comment: (20 pages, 13 figures
Strong diamagnetic response and specific heat anomaly above T_c in underdoped La_(2-x)Sr_xCuO_4
By measuring AC susceptibility using a very low amplitude of the AC field (<1
mG) it is shown that underdoped samples of La_(2-x)Sr_xCuO_4 (LASCO), are
diamagnetic in a temperature region above T_c up to a temperature T^*. This
behavior is only observed with AC fields along the c-axis whereas for fields in
the ab-plane no diamagnetism above Tc was detected. The diamagnetism is almost
frequency independent in the frequency range 0.1-10 kHz. At T* a broad step
anomaly in the specific heat is inferred through measurements of the elastic
constant c33. We suggest that the observed diamagnetism and the anomaly in the
elastic constant are associated with the existence of phase incoherent Cooper
pairs between Tc and T*.Comment: 5 pages 7 figures, to appear in Phys. rev
Raman scattering through a metal-insulator transition
The exact solution for nonresonant A1g and B1g Raman scattering is presented
for the simplest model that has a correlated metal-insulator transition--the
Falicov-Kimball model, by employing dynamical mean field theory. In the general
case, the A1g response includes nonresonant, resonant, and mixed contributions,
the B1g response includes nonresonant and resonant contributions (we prove the
Shastry-Shraiman relation for the nonresonant B1g response) while the B2g
response is purely resonant. Three main features are seen in the nonresonant
B1g channel: (i) the rapid appearance of low-energy spectral weight at the
expense of higher-energy weight; (b) the frequency range for this low-energy
spectral weight is much larger than the onset temperature, where the response
first appears; and (iii) the occurrence of an isosbestic point, which is a
characteristic frequency where the Raman response is independent of temperature
for low temperatures. Vertex corrections renormalize away all of these
anomalous features in the nonresonant A1g channel. The calculated results
compare favorably to the Raman response of a number of correlated systems on
the insulating side of the quantum-critical point (ranging from Kondo
insulators, to mixed-valence materials, to underdoped high-temperature
superconductors). We also show why the nonresonant B1g Raman response is
``universal'' on the insulating side of the metal-insulator transition.Comment: 12 pages, 11 figures, ReVTe
Level densities and thermodynamical properties of Pt and Au isotopes
The nuclear level densities of Pt and Au below the
neutron separation energy have been measured using transfer and scattering
reactions. All the level density distributions follow the constant-temperature
description. Each group of isotopes is characterized by the same temperature
above the energy threshold corresponding to the breaking of the first Cooper
pair. A constant entropy excess and is observed in
Pt and Au with respect to Pt and Au,
respectively, giving information on the available single-particle level space
for the last unpaired valence neutron. The breaking of nucleon Cooper pairs is
revealed by sequential peaks in the microcanonical caloric curve
Evolution of magnetic polarons and spin-carrier interactions through the metal-insulator transition in EuGdO
Raman scattering studies as functions of temperature, magnetic field, and
Gd-substitution are used to investigate the evolution of magnetic polarons and
spin-carrier interactions through the metal-insulator transition in
EuGdO. These studies reveal a greater richness of phase behavior
than have been previously observed using transport measurements: a
spin-fluctuation-dominated paramagnetic (PM) phase regime for T T
T, a two-phase regime for T T in which magnetic polarons
develop and coexist with a remnant of the PM phase, and an inhomogeneous
ferromagnetic phase regime for T T
La(, ) cross sections constrained with statistical decay properties of La nuclei
The nuclear level densities and -ray strength functions of
La were measured using the La(He, ),
La(He, He) and La(d, p) reactions. The
particle- coincidences were recorded with the silicon particle
telescope (SiRi) and NaI(Tl) (CACTUS) arrays. In the context of these
experimental results, the low-energy enhancement in the A140 region is
discussed. The La( cross sections were calculated
at - and -process temperatures using the experimentally measured nuclear
level densities and -ray strength functions. Good agreement is found
between La( calculated cross sections and previous
measurements
- …