10 research outputs found
Resonant Raman Scattering by quadrupolar vibrations of Ni-Ag Core-shell Nanoparticles
Low-frequency Raman scattering experiments have been performed on thin films
consisting of nickel-silver composite nanoparticles embedded in alumina matrix.
It is observed that the Raman scattering by the quadrupolar modes, strongly
enhanced when the light excitation is resonant with the surface dipolar
excitation, is mainly governed by the silver electron contribution to the
plasmon excitation. The Raman results are in agreement with a core-shell
structure of the nanoparticles, the silver shell being loosely bonded to the
nickel core.Comment: 3 figures. To be published in Phys. Rev.
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Acoustic vibrations of monoclinic zirconia nanocrystals
International audiencePolarized low-frequency Raman spectra originating from confined acoustic vibrations are reported for monoclinic ZrO2 nanoparticles with a narrow size distribution synthesized from a continuous supercritical water process. The monoclinic lattice structure is taken into account for the interpretation of the spectra by comparing with isotropic and anisotropic continuum elasticity calculations for monodomain nanocrystals. The various mechanisms leading to the broadening of the Raman peaks are discussed. We demonstrate that an accurate determination of the size distribution of the nanoparticles is possible using the Raman peak due to the fundamental breathing vibration which is hardly broadened by the elastic anisotropy and the shape distribution