5,096 research outputs found
Elucidating the role of hyperfine interactions on organic magnetoresistance using deuterated aluminium tris(8-hydroxyquinoline)
Measurements of the effect of a magnetic field on the light output and
current through an organic light emitting diode made with deuterated aluminium
tris(8-hydroxyquinoline) have shown that hyperfine coupling with protons is not
the cause of the intrinsic organic magnetoresistance. We suggest that
interactions with unpaired electrons in the device may be responsible.Comment: Submitte
Effect of excited states and applied magnetic fields on the measured hole mobility in an organic semiconductor
Copyright 2010 by the American Physical Society. Article is available at
Ferromagnetic-organic interfacial states and their role on low voltage current injection in tris-8-hydroxyquinloline (Alq(3)) organic spin valves
Recommended from our members
The tarantula toxin GxTx detains K+ channel gating charges in their resting conformation.
Allosteric ligands modulate protein activity by altering the energy landscape of conformational space in ligand-protein complexes. Here we investigate how ligand binding to a K+ channel's voltage sensor allosterically modulates opening of its K+-conductive pore. The tarantula venom peptide guangxitoxin-1E (GxTx) binds to the voltage sensors of the rat voltage-gated K+ (Kv) channel Kv2.1 and acts as a partial inverse agonist. When bound to GxTx, Kv2.1 activates more slowly, deactivates more rapidly, and requires more positive voltage to reach the same K+-conductance as the unbound channel. Further, activation kinetics are more sigmoidal, indicating that multiple conformational changes coupled to opening are modulated. Single-channel current amplitudes reveal that each channel opens to full conductance when GxTx is bound. Inhibition of Kv2.1 channels by GxTx results from decreased open probability due to increased occurrence of long-lived closed states; the time constant of the final pore opening step itself is not impacted by GxTx. When intracellular potential is less than 0 mV, GxTx traps the gating charges on Kv2.1's voltage sensors in their most intracellular position. Gating charges translocate at positive voltages, however, indicating that GxTx stabilizes the most intracellular conformation of the voltage sensors (their resting conformation). Kinetic modeling suggests a modulatory mechanism: GxTx reduces the probability of voltage sensors activating, giving the pore opening step less frequent opportunities to occur. This mechanism results in K+-conductance activation kinetics that are voltage-dependent, even if pore opening (the rate-limiting step) has no inherent voltage dependence. We conclude that GxTx stabilizes voltage sensors in a resting conformation, and inhibits K+ currents by limiting opportunities for the channel pore to open, but has little, if any, direct effect on the microscopic kinetics of pore opening. The impact of GxTx on channel gating suggests that Kv2.1's pore opening step does not involve movement of its voltage sensors
Infrared Hall effect in high Tc superconductors: Evidence for non-Fermi liquid Hall scattering
Infrared (20-120 cm-1 and 900-1100 cm-1) Faraday rotation and circular
dichroism are measured in high Tc superconductors using sensitive polarization
modulation techniques. Optimally doped YBCO thin films are studied at
temperatures down to 15 K and magnetic fields up to 8 T. At 1000 cm-1 the Hall
conductivity varies strongly with temperature in contrast to the longitudinal
conductivity which is nearly independent of temperature. The Hall scattering
rate has a T^2 temperature dependence but, unlike a Fermi liquid, depends only
weakly on frequency. The experiment puts severe constraints on theories of
transport in the normal state of high Tc superconductors.Comment: 8 pages, 3 figure
Magnetoresistance of YBa2Cu3O7 in the "cold spots" model
We calculate the in-plane magnetoresistance of
YBaCuO in a magnetic field applied perpendicular to the
planes for the ``cold spots'' model. In this model, the electron relaxation
time at small regions on the Fermi surface near the
Brillouin zone diagonals is much longer than the relaxation time
at the rest of the Fermi surface ( is temperature). In
qualitative agreement with the experiment, we find that Kohler's rule is
strongly violated, but the ratio ,
where is the Hall angle, is approximately
temperature-independent. We find the ratio is about 5.5, which is of the same
order of magnitude as in the experiment.Comment: RevTeX, 4 pages, 6 figures. V.2: 2 references adde
Mid-infrared Hall effect in thin-film metals: Probing the Fermi surface anisotropy in Au and Cu
A sensitive mid-infrared (MIR, 900-1100 cm-1, 112-136 meV) photo-elastic
polarization modulation technique is used to measure simultaneously Faraday
rotation and circular dichroism in thin metal films. These two quantities
determine the complex AC Hall conductivity. This novel technique is applied to
study Au and Cu thin films at temperatures down to 20 K and magnetic fields up
to 8 T. The Hall frequency is consistent with band theory predictions. We
report the first measurement of the MIR Hall scattering rate, which is
significantly lower than that derived from Drude analysis of zero magnetic
field MIR transmission measurements. This difference is qualitatively explained
in terms of the anisotropy of the Fermi surface in Au and Cu.Comment: 14 pages of text, 5 figure
Coexistence and competition of magnetism and superconductivity on the nanometer scale in underdoped BaFe1.89Co0.11As2
We report muon spin rotation (muSR) and infrared (IR) spectroscopy
experiments on underdoped BaFe1.89Co0.11As2 which show that bulk magnetism and
superconductivity (SC) coexist and compete on the nanometer length scale. Our
combined data reveal a bulk magnetic order, likely due to an incommensurate
spin density wave (SDW), which develops below Tmag \approx 32 K and becomes
reduced in magnitude (but not in volume) below Tc = 21.7 K. A slowly
fluctuating precursor of the SDW seems to develop alrady below the structural
transition at Ts \approx 50 K. The bulk nature of SC is established by the muSR
data which show a bulk SC vortex lattice and the IR data which reveal that the
majority of low-energy states is gapped and participates in the condensate at T
<< Tc
Measurement of the Far Infrared Magneto-Conductivity Tensor of Superconducting YBaCuO Thin Films
We report measurements of the far infrared transmission of superconducting
YBaCuO thin films from 5 cm to 200 cm in
fields up to 14. A Kramers-Kronig analysis of the magneto-transmission
spectrum yields the magneto-conductivity tensor. The result shows that the
magneto-conductivity of YBaCuO is dominated by three
terms: a London term, a low frequency Lorentzian ( 3 cm) of width 10 cm and a finite frequency Lorentzian of
width 17 cm at 24 cm in the hole
cyclotron resonance active mode of circular polarization.\\Comment: Revised LaTex file (12 pages) + 4 Postscript figures, uuencoded. In
response to referees' comments, we refined the paper a lot; we encourage you
to download this revised versio
- …