Terahertz Quantum Cascade Lasers - The Past, Present, and Potential Future

Since their first demonstration in 2002, the development of terahertz frequency quantum cascade lasers has been extremely rapid. We overview some of the advances that have taken place and which have made the terahertz quantum cascade laser such a ubiquitous source. We also consider potential future directions for terahertz quantum cascade laser technology, including its use in satellite-borne instrumentation for future Earth observation and planetary science missions

Multimode, Aperiodic Terahertz Surface-Emitting Laser Resonators

Quasi-crystal structures are conventionally built following deterministic generation rules although they do not present a full spatial periodicity. If used as laser resonators, they open up intriguing design possibilities that are simply not possible in conventional periodic photonic crystals: the distinction between symmetric (vertically radiative but low quality factor Q) and anti-symmetric (non-radiative, high Q) modes is indeed here fully overcome, offering a concrete perspective of highly efficient vertical emitting resonators. We here exploit electrically pumped terahertz quantum cascade heterostructures to devise two-dimensional seven-fold quasi-crystal resonators, exploiting rotational order or irregularly distributed defects. By lithographically tuning the lattice quasi-periodicity and/or the hole radius of the imprinted patterns, efficient multimode surface emission with a rich sequence of spectral lines distributed over a 2.9–3.4 THz bandwidth was reached. We demonstrated multicolor emission with 67 mW of peak optical power, slope efficiencies up to ≈70 mW/A, 0.14% wall plug efficiencies and beam profile results of the rich quasi-crystal Fourier spectrum that, in the case of larger rotational order, can reach very low divergence

Low divergent, high-power, single-mode terahertz wire lasers

We devise arrays of surface emitting THz QCLs exploiting two novel lithographic configurations: a) a dual periodicity slit architecture and b) corrugated sinusoidal wire laser cavities. Extremely low divergent optical beams, with up to 85 mW of emitted optical powers and 245 mV/A slope efficiencies have been reached

Estimation of Spectroscopic Uncertainty and Correlation in Terahertz Time Domain Spectroscopy

We present a method of calculating the measurement variance-covariance matrix of a spectroscopic sample’s complex refractive index from time-domain statistics in order to estimate uncertainty of a measurement. We compare this method to a numerical analysis and previously derived methodology, and show that our time-based estimate is both accurate and adaptable to complex extraction models

Multilayer Extraction of Complex Refractive Index in Broadband Transmission Terahertz Time-Domain Spectroscopy

In terahertz spectroscopy, multi-layered samples often need to be measured, for instance in a liquid flow cell, and this complicates the extraction of material parameters. We present a spectroscopic parameter extraction algorithm for multilayer samples that can also be used to extract the thickness of an unknown sample laye

Wideband Electrically Controlled Vernier Frequency Tunable Terahertz Quantum Cascade Laser

Frequency tuning in terahertz frequency quantum cascade lasers is challenging because of low thermal and current tuning coefficients. Moreover, photonic designs like Vernier selection based sampled gratings, used in telecom lasers to tune emission frequency, are unsuitable due to the long terahertz wavelengths and will require impractically long cavities (>15 mm). Here, we report the first wideband frequency tuning from a monolithic device exploiting Vernier selection rules using a coupled-cavity laser with a defect engineered photonic lattice. A precisely positioned defect lattice allows us to engineer the free spectral range and finesse of one of the cavities, similar to a sampled grating but using shorter cavity lengths (<4 mm). A coupled-cavity was used to tune the emission frequency. We achieve frequency tuning over 209 GHz, including mode hop-free continuous tuning of ∼6–21 GHz across six frequency bands, controlled through Stark shift, cavity-pulling, localized Joule heating, and thermal effects

Near-Field Analysis of Terahertz Pulse Generation From Photo-Excited Charge Density Gradients

Excitation of photo-current transients at semiconductor surfaces by subpicosecond optical pulses gives rise to emission of electromagnetic pulses of terahertz (THz) frequency radiation. To correlate the THz emission with the photo-excited charge density distribution and the photo-current direction, we mapped near-field and far-field distributions of the generated THz waves from GaAs and Fe-doped InGaAs surfaces. The experimental results show that the charge dynamics in the plane of the surface can radiate substantially stronger THz pulses than the charge dynamics in the direction normal to the surface, which is generally regarded as the dominant origin of the emission

Ultra-fast sampling of terahertz pulses from a quantum cascade laser using superconducting antenna-coupled NbN and YBCO detectors

We demonstrate the ultra-fast detection of terahertz pulses from a quantum cascade laser (QCL) using superconducting NbN and YBCO detectors. This has enabled both the intrapulse and interpulse dynamics of a THz QCL to be measured directly, including interpulse heating effects on sub-μs timescales