74 research outputs found
Surface induced magnetization reversal of MnP nanoclusters embedded in GaP
We investigate the quasi-static magnetic behavior of ensembles of
non-interacting ferromagnetic nanoparticles consisting of MnP nanoclusters
embedded in GaP(001) epilayers grown at 600, 650 and 700{\deg}C. We use a
phenomenological model, in which surface effects are included, to reproduce the
experimental hysteresis curves measured as a function of temperature (120-260
K) and direction of the applied field. The slope of the hysteresis curve during
magnetization reversal is determined by the MnP nanoclusters size distribution,
which is a function of the growth temperature. Our results show that the
coercive field is very sensitive to the strength of the surface anisotropy,
which reduces the energy barrier between the two states of opposite
magnetization. Notably, this reduction in the energy barrier increases by a
factor of 3 as the sample temperature is lowered from 260 to 120 K.Comment: 7 pages, 5 figure
High quality factor nitride-based optical cavities: microdisks with embedded GaN/Al(Ga)N quantum dots
We compare the quality factor values of the whispery gallery modes of
microdisks incorporating GaN quantum dots (QDs) grown on AlN and AlGaN barriers
by performing room temperature photoluminescence (PL) spectroscopy. The PL
measurements show a large number of high Q factor (Q) resonant modes on the
whole spectrum which allows us to identify the different radial mode families
and to compare them with simulations. We report a considerable improvement of
the Q factor which reflect the etching quality and the relatively low cavity
loss by inserting QDs into the cavity. GaN/AlN QDs based microdisks show very
high Q values (Q > 7000) whereas the Q factor is only up to 2000 in microdisks
embedding QDs grown on AlGaN barrier layer. We attribute this difference to the
lower absorption below bandgap for AlN barrier layers at the energies of our
experimental investigation
Influence of magnetostatic interactions on first-order-reversal-curve (FORC) diagrams: a micromagnetic approach
Accepted versio
Lorentz transmission electron microscopy and magnetic force microscopy characterization of NiFe/Al-oxide/Co films
Magnetization reversal process of NiFe/Al-oxide/Co junction films was observed directly using Lorentztransmission electron microscopy (LTEM) and magnetic force microscopy(MFM).In situmagnetizing experiments performed in both LTEM and MFM were facilitated by a pair of electromagnets, which were mounted on the sample stages. A two-stage magnetization reversal process for the junction film was clearly observed in LTEM with NiFe magnetization reversed first via domain wall motion followed by Co magnetization reversal via moment rotation and domain wall motion. Reversal mechanism and domain characteristics of the NiFe and Co layers showed very distinctive features. The magnetization curve of the junction filmmeasured using alternating gradient force magnetometry showed a nonzero slope at the antiparallel magnetization configuration region, which implies that magnetization directions of the NiFe and Co layers were not exactly antiparallel due to Co moment rotation existed in that region. After the magnetization reversal of the Co was complete, MFM images revealed some magnetic contrast, which suggests that an out-of-plane magnetization component remained in the Co layer. Such magnetic contrast disappeared at higher magnetic fields when the Co moments further rotated and aligned parallel to the applied field direction
The Kondo effect in ferromagnetic atomic contacts
Iron, cobalt and nickel are archetypal ferromagnetic metals. In bulk,
electronic conduction in these materials takes place mainly through the and
electrons, whereas the magnetic moments are mostly in the narrow
-electron bands, where they tend to align. This general picture may change
at the nanoscale because electrons at the surfaces of materials experience
interactions that differ from those in the bulk. Here we show direct evidence
for such changes: electronic transport in atomic-scale contacts of pure
ferromagnets (iron, cobalt and nickel), despite their strong bulk
ferromagnetism, unexpectedly reveal Kondo physics, that is, the screening of
local magnetic moments by the conduction electrons below a characteristic
temperature. The Kondo effect creates a sharp resonance at the Fermi energy,
affecting the electrical properties of the system;this appears as a Fano-Kondo
resonance in the conductance characteristics as observed in other artificial
nanostructures. The study of hundreds of contacts shows material-dependent
lognormal distributions of the resonance width that arise naturally from Kondo
theory. These resonances broaden and disappear with increasing temperature,
also as in standard Kondo systems. Our observations, supported by calculations,
imply that coordination changes can significantly modify magnetism at the
nanoscale. Therefore, in addition to standard micromagnetic physics, strong
electronic correlations along with atomic-scale geometry need to be considered
when investigating the magnetic properties of magnetic nanostructures.Comment: 7 pages, 5 figure
Hematopoietic origin of Langerhans cell histiocytosis and Erdheim-Chester disease in adults.
Langerhans cell histiocytosis (LCH) and Erdheim-Chester disease (ECD) are rare histiocytic disorders induced by somatic mutation of MAPK pathway genes. BRAFV600E mutation is the most common mutation in both conditions and also occurs in the hematopoietic neoplasm hairy cell leukemia (HCL). It is not known if adult LCH or ECD arises from hematopoietic stem cells (HSCs), nor which potential blood borne precursors lead to the formation of histiocytic lesions. In this study, BRAFV600E allele-specific polymerase chain reaction was used to map the neoplastic clone in 20 adults with LCH, ECD, and HCL. BRAFV600E was tracked to classical monocytes, nonclassical monocytes, and CD1c+ myeloid dendritic cells (DCs) in the blood, and mutations were observed in HSCs and myeloid progenitors in the bone marrow of 4 patients. The pattern of involvement of peripheral blood myeloid cells was indistinguishable between LCH and ECD, although the histiocytic disorders were distinct to HCL. As reported in children, detection of BRAFV600E in peripheral blood of adults was a marker of active multisystem LCH. The healthy counterparts of myeloid cells affected by BRAF mutation had a range of differentiation potentials depending on exogenous signals. CD1c+ DCs acquired high langerin and CD1a with granulocyte-macrophage colony-stimulating factor and transforming growth factor β alone, whereas CD14+ classical monocytes required additional notch ligation. Both classical and nonclassical monocytes, but not CD1c+ DCs, made foamy macrophages easily in vitro with macrophage colony-stimulating factor and human serum. These studies are consistent with a hematopoietic origin and >1 immediate cellular precursor in both LCH and ECD
First-principles study of the inversion thermodynamics and electronic structure of FeM2X4 (thio)spinels (M = Cr, Mn, Co, Ni; X = O, S)
FeM2X4 spinels, where M is a transition metal and X is oxygen or sulfur, are candidate materials for spin filters, one of the key devices in spintronics. We present here a computational study of the inversion thermodynamics and the electronic structure of these (thio)spinels for M = Cr, Mn, Co, Ni, using calculations based on the density functional theory with on-site Hubbard corrections (DFT+U). The analysis of the configurational free energies shows that different behaviour is expected for the equilibrium cation distributions in these structures: FeCr2X4 and FeMn2S4 are fully normal, FeNi2X4 and FeCo2S4 are intermediate, and FeCo2O4 and FeMn2O4 are fully inverted. We have analyzed the role played by the size of the ions and by the crystal field stabilization effects in determining the equilibrium inversion degree. We also discuss how the electronic and magnetic structure of these spinels is modified by the degree of inversion, assuming that this could be varied from the equilibrium value. We have obtained electronic densities of states for the completely normal and completely inverse cation distribution of each compound. FeCr2X4, FeMn2X4, FeCo2O4 and FeNi2O4 are half-metals in the ferrimagnetic state when Fe is in tetrahedral positions. When M is filling the tetrahedral positions, the Cr-containing compounds and FeMn2O4 are half-metallic systems, while the Co and Ni spinels are insulators. The Co and Ni sulfide counterparts are metallic for any inversion degree together with the inverse FeMn2S4. Our calculations suggest that the spin filtering properties of the FeM2X4 (thio)spinels could be modified via the control of the cation distribution through variations in the synthesis conditions
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