61 research outputs found
Measurement and Control of Single Nitrogen-Vacancy Center Spins above 600 K
We study the spin and orbital dynamics of single nitrogen-vacancy (NV)
centers in diamond between room temperature and 700 K. We find that the ability
to optically address and coherently control single spins above room temperature
is limited by nonradiative processes that quench the NV center's
fluorescence-based spin readout between 550 and 700 K. Combined with electronic
structure calculations, our measurements indicate that the energy difference
between the 3E and 1A1 electronic states is approximately 0.8 eV. We also
demonstrate that the inhomogeneous spin lifetime (T2*) is temperature
independent up to at least 625 K, suggesting that single NV centers could be
applied as nanoscale thermometers over a broad temperature range.Comment: 8 pages, 5 figures, and 14 pages of supplemental material with
additional figures. Title change and minor revisions from previous version.
DMT and DJC contributed equally to this wor
Resonance fluorescence from an artificial atom in squeezed vacuum
We present an experimental realization of resonance fluorescence in squeezed
vacuum. We strongly couple microwave-frequency squeezed light to a
superconducting artificial atom and detect the resulting fluorescence with high
resolution enabled by a broadband traveling-wave parametric amplifier. We
investigate the fluorescence spectra in the weak and strong driving regimes,
observing up to 3.1 dB of reduction of the fluorescence linewidth below the
ordinary vacuum level and a dramatic dependence of the Mollow triplet spectrum
on the relative phase of the driving and squeezed vacuum fields. Our results
are in excellent agreement with predictions for spectra produced by a two-level
atom in squeezed vacuum [Phys. Rev. Lett. \textbf{58}, 2539-2542 (1987)],
demonstrating that resonance fluorescence offers a resource-efficient means to
characterize squeezing in cryogenic environments
Engineering shallow spins in diamond with nitrogen delta-doping
We demonstrate nanometer-precision depth control of nitrogen-vacancy (NV)
center creation near the surface of synthetic diamond using an in situ nitrogen
delta-doping technique during plasma-enhanced chemical vapor deposition.
Despite their proximity to the surface, doped NV centers with depths (d)
ranging from 5 - 100 nm display long spin coherence times, T2 > 100 \mus at d =
5 nm and T2 > 600 \mus at d \geq 50 nm. The consistently long spin coherence
observed in such shallow NV centers enables applications such as atomic-scale
external spin sensing and hybrid quantum architectures.Comment: 14 pages, 4 figures, 11 pages of additional supplementary materia
Decoherence-protected quantum gates for a hybrid solid-state spin register
Protecting the dynamics of coupled quantum systems from decoherence by the
environment is a key challenge for solid-state quantum information processing.
An idle qubit can be efficiently insulated from the outside world via dynamical
decoupling, as has recently been demonstrated for individual solid-state
qubits. However, protection of qubit coherence during a multi-qubit gate poses
a non-trivial problem: in general the decoupling disrupts the inter-qubit
dynamics, and hence conflicts with gate operation. This problem is particularly
salient for hybrid systems, wherein different types of qubits evolve and
decohere at vastly different rates. Here we present the integration of
dynamical decoupling into quantum gates for a paradigmatic hybrid system, the
electron-nuclear spin register. Our design harnesses the internal resonance in
the coupled-spin system to resolve the conflict between gate operation and
decoupling. We experimentally demonstrate these gates on a two-qubit register
in diamond operating at room temperature. Quantum tomography reveals that the
qubits involved in the gate operation are protected as accurately as idle
qubits. We further illustrate the power of our design by executing Grover's
quantum search algorithm, achieving fidelities above 90% even though the
execution time exceeds the electron spin dephasing time by two orders of
magnitude. Our results directly enable decoherence-protected interface gates
between different types of promising solid-state qubits. Ultimately, quantum
gates with integrated decoupling may enable reaching the accuracy threshold for
fault-tolerant quantum information processing with solid-state devices.Comment: This is original submitted version of the paper. The revised and
finalized version is in print, and is subjected to the embargo and other
editorial restrictions of the Nature journa
Resonant enhancement of the zero-phonon emission from a color center in a diamond cavity
We demonstrate coupling of the zero-phonon line of individual
nitrogen-vacancy centers and the modes of microring resonators fabricated in
single-crystal diamond. A zero-phonon line enhancement exceeding ten-fold is
estimated from lifetime measurements at cryogenic temperatures. The devices are
fabricated using standard semiconductor techniques and off-the-shelf materials,
thus enabling integrated diamond photonics.Comment: 5 pages, 4 figure
Topologically Protected Quantum State Transfer in a Chiral Spin Liquid
Topology plays a central role in ensuring the robustness of a wide variety of
physical phenomena. Notable examples range from the robust current carrying
edge states associated with the quantum Hall and the quantum spin Hall effects
to proposals involving topologically protected quantum memory and quantum logic
operations. Here, we propose and analyze a topologically protected channel for
the transfer of quantum states between remote quantum nodes. In our approach,
state transfer is mediated by the edge mode of a chiral spin liquid. We
demonstrate that the proposed method is intrinsically robust to realistic
imperfections associated with disorder and decoherence. Possible experimental
implementations and applications to the detection and characterization of spin
liquid phases are discussed.Comment: 14 pages, 7 figure
Quantum wave mixing and visualisation of coherent and superposed photonic states in a waveguide
Superconducting quantum systems (artificial atoms) have been recently
successfully used to demonstrate on-chip effects of quantum optics with single
atoms in the microwave range. In particular, a well-known effect of four-wave
mixing could reveal a series of features beyond classical physics, when a
non-linear medium is scaled down to a single quantum scatterer. Here we
demonstrate a phenomenon of the quantum wave mixing (QWM) on a single
superconducting artificial atom. In the QWM, the spectrum of elastically
scattered radiation is a direct map of the interacting superposed and coherent
photonic states. Moreover, the artificial atom visualises photon-state
statistics, distinguishing coherent, one- and two-photon superposed states with
the finite (quantized) number of peaks in the quantum regime. Our results may
give a new insight into nonlinear quantum effects in microwave optics with
artificial atoms.Comment: 6 pages, 5 figures; accepted versio
Laser writing of coherent colour centres in diamond
Optically active point defects in crystals have gained widespread attention as photonic systems that can find use in quantum information technologies [1,2]. However challenges remain in the placing of individual defects at desired locations, an essential element of device fabrication. Here we report the controlled generation of single nitrogen-vacancy (NV) centres in diamond using laser writing [3]. The use of aberration correction in the writing optics allows precise positioning of vacancies within the diamond crystal, and subsequent annealing produces single NV centres with up to 45% success probability, within about 200 nm of the desired position. Selected NV centres fabricated by this method display stable, coherent optical transitions at cryogenic temperatures, a pre-requisite for the creation of distributed quantum networks of solid-state qubits. The results illustrate the potential of laser writing as a new tool for defect engineering in quantum technologies
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