175 research outputs found

    Competing charge density waves and temperature-dependent nesting in 2H-TaSe2

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    Multiple charge density wave (CDW) phases in 2H-TaSe2 are investigated by high-resolution synchrotron x-ray diffraction. In a narrow temperature range immediately above the commensurate CDW transition, we observe a multi-q superstructure with coexisting commensurate and incommensurate order parameters, clearly distinct from the fully incommensurate state at higher temperatures. This multi-q ordered phase, characterized by a temperature hysteresis, is found both during warming and cooling, in contrast to previous reports. In the normal state, the incommensurate superstructure reflection gives way to a broad diffuse peak that persists nearly up to room temperature. Its position provides a direct and accurate estimate of the Fermi surface nesting vector, which evolves non-monotonically and approaches the commensurate position as the temperature is increased. This behavior agrees with our recent observations of the temperature-dependent Fermi surface in the same compound [Phys. Rev. B 79, 125112 (2009)]

    Crossover from weak to strong pairing in unconventional superconductors

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    Superconductors are classified by their pairing mechanism and the coupling strength, measured as the ratio of the energy gap to the critical temperature, Tc. We present an extensive comparison of the gap ratios among many single- and multiband superconductors from simple metals to high-Tc cuprates and iron pnictides. Contrary to the recently suggested universality of this ratio in Fe-based superconductors, we find that the coupling in pnictides ranges from weak, near the BCS limit, to strong, as in cuprates, bridging the gap between these two extremes. Moreover, for Fe- and Cu-based materials, our analysis reveals a universal correlation between the gap ratio and Tc, which is not found in conventional superconductors and therefore supports a common unconventional pairing mechanism in both families. An important consequence of this result for ferropnictides is that the separation in energy between the excitonic spin-resonance mode and the particle-hole continuum, which determines the resonance damping, no longer appears independent of Tc.Comment: 15 pages, 3 figures, 5 tables with an exhaustive overview of the published gap and spin-resonance measurements in Fe-based superconductors. New in V3: updated references. To be published in Phys. Rev.

    Dispersion and damping of zone-boundary magnons in the noncentrosymmetric superconductor CePt3Si

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    Inelastic neutron scattering (INS) is employed to study damped spin-wave excitations in the noncentrosymmetric heavy-fermion superconductor CePt3Si along the antiferromagnetic Brillouin-zone boundary in the low-temperature magnetically ordered state. Measurements along the (1/2 1/2 L) and (H H 1/2-H) reciprocal-space directions reveal deviations in the spin-wave dispersion from the previously reported model. Broad asymmetric shape of the peaks in energy signifies strong spin-wave damping by interactions with the particle-hole continuum. Their energy width exhibits no evident anomalies as a function of momentum along the (1/2 1/2 L) direction, which could be attributed to Fermi-surface nesting effects, implying the absence of pronounced commensurate nesting vectors at the magnetic zone boundary. In agreement with a previous study, we find no signatures of the superconducting transition in the magnetic excitation spectrum, such as a magnetic resonant mode or a superconducting spin gap, either at the magnetic ordering wavevector (0 0 1/2) or at the zone boundary. However, the low superconducting transition temperature in this material still leaves the possibility of such features being weak and therefore hidden below the incoherent background at energies ~0.1 meV, precluding their detection by INS

    Quantitative assessment of pinning forces and the superconducting gap in NbN thin films from complementary magnetic force microscopy and transport measurements

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    Epitaxial niobium-nitride thin films with a critical temperature of Tc=16K and a thickness of 100nm were fabricated on MgO(100) substrates by pulsed laser deposition. Low-temperature magnetic force microscopy (MFM) images of the supercurrent vortices were measured after field cooling in a magnetic field of 3mT at various temperatures. Temperature dependence of the penetration depth has been evaluated by a two-dimensional fitting of the vortex profiles in the monopole-monopole model. Its subsequent fit to a single s-wave gap function results in the superconducting gap amplitude Delta(0) = 2.9 meV = 2.1*kB*Tc, in perfect agreement with previous reports. The pinning force has been independently estimated from local depinning of individual vortices by lateral forces exerted by the MFM tip and from transport measurements. A good quantitative agreement between the two techniques shows that for low fields, B << Hc2, MFM is a powerful and reliable technique to probe the local variations of the pinning landscape. We also demonstrate that the monopole model can be successfully applied even for thin films with a thickness comparable to the penetration depth.Comment: 6 pages, 6 figures, 2 table

    Surface properties of SmB6 from x-ray photoelectron spectroscopy

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    We have investigated the properties of cleaved SmB6_6 single crystals by x-ray photoelectron spectroscopy. At low temperatures and freshly cleaved samples a surface core level shift is observed which vanishes when the temperature is increased. A Sm valence between 2.5 - 2.6 is derived from the relative intensities of the Sm2+^{2+} and Sm3+^{3+} multiplets. The B/Sm intensity ratio obtained from the core levels is always larger than the stoichiometric value. Possible reasons for this deviation are discussed. The B 1s1s signal shows an unexpected complexity: an anomalous low energy component appears with increasing temperature and is assigned to the formation of a suboxide at the surface. While several interesting intrinsic and extrinsic properties of the SmB6_6 surface are elucidated in this manuscript no clear indication of a trivial mechanism for the prominent surface conductivity is found

    Magnetic-field and doping dependence of low-energy spin fluctuations in the antiferroquadrupolar compound Ce(1-x)La(x)B(6)

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    CeB(6) is a model compound exhibiting antiferroquadrupolar (AFQ) order, its magnetic properties being typically interpreted within localized models. More recently, the observation of strong and sharp magnetic exciton modes forming in its antiferromagnetic (AFM) state at both ferromagnetic and AFQ wave vectors suggested a significant contribution of itinerant electrons to the spin dynamics. Here we investigate the evolution of the AFQ excitation upon the application of an external magnetic field and the substitution of Ce with non-magnetic La, both parameters known to suppress the AFM phase. We find that the exciton energy decreases proportionally to T_N upon doping. In field, its intensity is suppressed, while its energy remains constant. Its disappearance above the critical field of the AFM phase is preceded by the formation of two modes, whose energies grow linearly with magnetic field upon entering the AFQ phase. These findings suggest a crossover from itinerant to localized spin dynamics between the two phases, the coupling to heavy-fermion quasiparticles being crucial for a comprehensive description of the magnon spectrum.Comment: Extended version with a longer introduction and an additional figure. 6 pages and 5 figure
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