412 research outputs found

    Nature of magnetism in Ca3_3Co2_2O6_6

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    We find using LSDA+U band structure calculations that the novel one-dimensional cobaltate Ca3_3Co2_2O6_6 is not a ferromagnetic half-metal but a Mott insulator. Both the octahedral and the trigonal Co ions are formally trivalent, with the octahedral being in the low-spin and the trigonal in the high-spin state. The inclusion of the spin-orbit coupling leads to the occupation of the minority-spin d2d_{2} orbital for the unusually coordinated trigonal Co, producing a giant orbital moment (1.57 ÎŒB\mu_{B}). It also results in an anomalously large magnetocrystalline anisotropy (of order 70 meV), elucidating why the magnetism is highly Ising-like. The role of the oxygen holes, carrying an induced magnetic moment of 0.13 ÎŒB\mu_{B} per oxygen, for the exchange interactions is discussed.Comment: 5 pages, 4 figures, and 1 tabl

    Photoluminescence from low temperature grown InAs/GaAs quantum dots

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    The authors investigated a set of self-assembled InAs/GaAs quantum dots (QDs) formed by mol. beam epitaxy at low temp. (LT, 250 DegC) and postgrowth annealing. A QD photoluminescence (PL) peak around 1.01 eV was obsd. The PL efficiency quickly quenches between 6 and 40 K due to the tunneling out of the QD into traps within the GaAs barrier. The PL efficiency increases by a factor of 45-280 when exciting below the GaAs band gap, directly into the InAs QD layer. This points towards good optical quality QDs, which are embedded in a LT-GaAs barrier with a high trapping efficiency. [on SciFinder (R)

    Spin-state transition in LaCoO3: direct neutron spectroscopic evidence of excited magnetic states

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    A gradual spin-state transition occurs in LaCoO3 around T~80-120 K, whose detailed nature remains controversial. We studied this transition by means of inelastic neutron scattering (INS), and found that with increasing temperature an excitation at ~0.6 meV appears, whose intensity increases with temperature, following the bulk magnetization. Within a model including crystal field interaction and spin-orbit coupling we interpret this excitation as originating from a transition between thermally excited states located about 120 K above the ground state. We further discuss the nature of the magnetic excited state in terms of intermediate-spin (IS, S=1) vs. high-spin (HS, S=2) states. Since the g-factor obtained from the field dependence of the INS is g~3, the second interpretation looks more plausible.Comment: 10 pages, 4 figure

    Bubble transport by electro-magnetophoretic forces at anode bottom of aluminium cells

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    Electrically conducting and nonconducting particles and bubbles experience additional forcing in a liquid which carries electric current. These so called electro-magnetophoretic forces are well known in metallurgical applications, like metal purification in vacuum-arc remelting, electro-slag processes, impurity removal or concentration change in special castings. However, the effect of electro-magnetophoretic forces has never been considered for aluminium cells where the gas bubbles evolving in the liquid electrolyte are surrounded by an electric current and significant magnetic fields. We present models to estimate the effect of electric current flow in the vicinity of the bubbles and the additional pressure distribution resulting from the magnetic forces in the surrounding liquid electrolyte. According to the estimates, this force becomes important for bubbles exceeding 2 mm in size, and could be sufficient to overcome the typical drag force associated with electrolyte flow thereby opposing motion of the bubble along the base of the anode when it is inclined at a slight angle. The effect could explain certain features of the anode effect onset. Mathematical models and numerical results are presented and a further implementation in the general MHD code for the aluminium cell design is discussed

    Nonlinear stabilization of tokamak microturbulence by fast ions

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    Nonlinear electromagnetic stabilization by suprathermal pressure gradients found in specific regimes is shown to be a key factor in reducing tokamak microturbulence, augmenting significantly the thermal pressure electromagnetic stabilization. Based on nonlinear gyrokinetic simulations investigating a set of ion heat transport experiments on the JET tokamak, described by Mantica et al. [Phys. Rev. Lett. 107 135004 (2011)], this result explains the experimentally observed ion heat flux and stiffness reduction. These findings are expected to improve the extrapolation of advanced tokamak scenarios to reactor relevant regimes.Comment: 5 pages, 5 figure

    Bulk and surface electronic properties of SmB6: a hard x-ray photoelectron spectroscopy study

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    We have carried out bulk-sensitive hard x-ray photoelectron spectroscopy (HAXPES) measurements on in-situ cleaved and ex-situ polished SmB6 single crystals. Using the multiplet-structure in the Sm 3d core level spectra, we determined reliably that the valence of Sm in bulk SmB6 is close to 2.55 at ~5 K. Temperature dependent measurements revealed that the Sm valence gradually increases to 2.64 at 300 K. From a detailed line shape analysis we can clearly observe that not only the J=0 but also the J=1 state of the Sm 4f 6 configuration becomes occupied at elevated temperatures. Making use of the polarization dependence, we were able to identify and extract the Sm 4f spectral weight of the bulk material. Finally, we revealed that the oxidized or chemically damaged surface region of the ex-situ polished SmB6 single crystal is surprisingly thin, about 1 nm only.Comment: 11 pages, 8 figure
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