Non-adiabatic cluster expansion after ultrashort laser interaction

AbstractWe used X-ray spectroscopy as a diagnostic tool for investigating the properties of laser-cluster interactions at the stage in which non-adiabatic cluster expansion takes place and a quasi-homogeneous plasma is produced. The experiment was carried out with a 10 TW, 65 fs Ti:Sa laser focused on CO2 cluster jets. The effect of different laser-pulse contrast ratios and cluster concentrations was investigated. The X-ray emission associated to the Rydberg transitions allowed us to retrieve, through the density and temperature of the emitting plasma, the time after the beginning of the interaction at which the emission occurred. The comparison of this value with the estimated time for the "homogeneous" plasma formation shows that the degree of adiabaticity depends on both the cluster concentration and the pulse contrast. Interferometric measurements support the X-ray data concerning the plasma electron density

X-ray radiation from ions with K-shell vacancies

Abstract New types of space resolved X-ray spectra produced in light matter experiments with high intensity lasers have been investigated experimentally and theoretically. This type of spectra is characterised by the disappearance of distinct resonance line emission and the appearance of very broad emission structures due to the dielectronic satellite transitions associated to the resonance lines. Atomic data calculations have shown, that rather exotic states with K-shell vacancies are involved. For quantitative spectra interpretation we developed a model for dielectronic satellite accumulation (DSA-model) in cold dense optically thick plasmas which are tested by rigorous comparison with space resolved spectra from ns-lasers. In experiments with laser intensities up to 10 19 W/cm 2 focused into nitrogen gas targets, hollow ion configurations are observed by means of soft X-ray spectroscopy. It is shown that transitions in hollow ions can be used for plasma diagnostic. The determination of the electron temperature in the long lasting recombining regime is demonstrated. In Light-matter interaction experiments with extremely high contrast (up to 10 10 ) short pulse (400 fs) lasers electron densities of n e ≈3×10 23 cm −3 at temperatures between kT e =200–300 eV have been determined by means of spectral simulations developed previously for ns-laser produced plasmas. Expansion velocities are determined analysing asymmetric optically thick line emission. Further, the results are checked by observing the spectral windows involving the region about the He α -line and the region from the He β -line to the He-like continuum. Finally, plasmas of solid density are characteristic in experiments with heavy ion beams heating massive targets. We report the first spectroscopic investigations in plasmas of this type with results on solid neon heated by Ar-ions. A spectroscopic method for the determination of the electron temperature in extreme optically thick plasmas is developed

Time resolved study of laser induced coloured centres in SiO2

We report the investigation of the onset of an absorption band in the UV in crystalline quartz (alpha-SiO2) induced by an intense femtosecond laser pulse. Using a conventional pump– probe technique, we have measured the absorptions at 219 nm (5.66 eV) and at 240 nm (5.16 eV) as functions of time, at two different temperatures (10 and 300 K). The rise time of the absorption is measured to be 150 (50) fs. It is independent of probe wavelength and sample temperature. The absorption coefficients are similar at both probe wavelengths and the values at room temperature are about twice these at 10 K. We attribute the onset of the absorption to the ultra-fast formation of self-trapped excitons (STEs). The STEs recombine radiatively at a low temperature. At room temperature, we observe a cumulative effect. This demonstrates that, at 300 K, some of the STEs are converted to permanent colour centres, which we tentatively identify as neutral oxygen vacancies

High-efficiency, simple setup for pulse cleaning at the millijoule level by nonlinear induced birefringence

International audienceNonlinear elliptical polarization rotation is used to improve the contrast of femtosecond pulses by several orders of magnitude. Using nonlinear induced birefringence in air, we produced cleaned pulses with an energy of a few hundreds of microjoules. This technique presents several major advantages, such as convenience and stability of the setup. We investigated the phase profile required for obtaining high-energy pulses. No phase distortion is observed, and the spatial quality of the beam is preserved

ASE contrast improvement with a non-linear filtering Sagnac interferometer

International audienceA new method to improve the temporal contrast of an ultra-short laser pulse has been developed. This technique uses a Sagnac interferometer in combination with a non-linear medium. A phase shift induced in the ultra-short pulse by non-linear effect separates it from the amplified spontaneous emission background. Experiments with a 1 kHz, 55 fs, 1 mJ Ti:Sa laser were performed. The temporal contrast measurements have shown a contrast improvement of four orders of magnitude