1 research outputs found
Charge Fluctuations in Geometrically Frustrated Charge Ordering System
Effects of geometrical frustration in low-dimensional charge ordering systems
are theoretically studied, mainly focusing on dynamical properties. We treat
extended Hubbard models at quarter-filling, where the frustration arises from
competing charge ordered patterns favored by different intersite Coulomb
interactions, which are effective models for various charge transfer-type
molecular conductors and transition metal oxides. Two different lattice
structures are considered: (a) one-dimensional chain with intersite Coulomb
interaction of nearest neighbor V_1 and that of next-nearest neighbor V_2, and
(b) two-dimensional square lattice with V_1 along the squares and V_2 along one
of the diagonals. From previous studies, charge ordered insulating states are
known to be unstable in the frustrated region, i.e., V_1 \simeq 2V_2 for case
(a) and V_1 \simeq V_2 for case (b), resulting in a robust metallic phase even
when the interaction strenghs are strong. By applying the Lanczos exact
diagonalization to finite-size clusters, we have found that fluctuations of
different charge order patterns exist in the frustration-induced metallic
phase, showing up as characteristic low energy modes in dynamical correlation
functions. Comparison of such features between the two models are discussed,
whose difference will be ascribed to the dimensionality effect. We also point
out incommensurate correlation in the charge sector due to the frustration,
found in one-dimensional clusters.Comment: 8 pages, 9 figure