186 research outputs found
Magnetic strong coupling in a spin-photon system and transition to classical regime
We study the energy level structure of the Tavis-Cumming model applied to an
ensemble of independent magnetic spins coupled to a variable number of
photons. Rabi splittings are calculated and their distribution is analyzed as a
functin of photon number and spin system size . A sharp
transition in the distribution of the Rabi frequency is found at . The width of the Rabi frequency spectrum diverges as
at this point. For increased number of photons , the Rabi
frequencies converge to a value proportional to . This
behavior is interpreted as analogous to the classical spin resonance mechanism
where the photon is treated as a classical field and one resonance peak is
expected. We also present experimental data demonstrating cooperative, magnetic
strong coupling between a spin system and photons, measured at room
temperature. This points towards quantum computing implementation with magnetic
spins, using cavity quantum-electrodynamics techniques.Comment: Received 8 April 2010; revised manuscript received 17 June 2010;
published 14 July 201
Spin-Orbit Coupling Fluctuations as a Mechanism of Spin Decoherence
We discuss a general framework to address spin decoherence resulting from
fluctuations in a spin Hamiltonian. We performed a systematic study on spin
decoherence in the compound K[VAsO(DO)]
8DO, using high-field Electron Spin Resonance (ESR). By analyzing the
anisotropy of resonance linewidths as a function of orientation, temperature
and field, we find that the spin-orbit term is a major decoherence source. The
demonstrated mechanism can alter the lifetime of any spin qubit and we discuss
how to mitigate it by sample design and field orientation.Comment: submitte
Entrapment of magnetic micro-crystals for on-chip electron spin resonance studies
On-chip Electron Spin Resonance (ESR) of magnetic molecules requires the
ability to precisely position nanosized samples in antinodes of the
electro-magnetic field for maximal magnetic interaction. A method is developed
to entrap micro-crystals containing spins in a well defined location on a
substrate's surface. Traditional cavity ESR measurements are then performed on
a mesoscopic crystal at 34 GHz. Polycrystalline diluted Cr spins were
entrapped as well and measured while approaching the lower limit of the ESR
sensitivity. This method suggests the feasibility of on-chip ESR measurements
at dilution refrigerator temperatures by enabling the positioning of samples
atop an on-chip superconducting cavity.Comment: to appear in Journal of Applied Physic
Photon and spin dependence of the resonance lines shape in the strong coupling regime
We study the quantum dynamics of a spin ensemble coupled to cavity photons.
Recently, related experimental results have been reported, showing the
existence of the strong coupling regime in such systems. We study the
eigenenergy distribution of the multi-spin system (following the Tavis-Cummings
model) which shows a peculiar structure as a function of the number of cavity
photons and of spins. We study how this structure causes changes in the
spectrum of the admittance in the linear response theory, and also the
frequency dependence of the excited quantities in the stationary state under a
probing field. In particular, we investigate how the structure of the higher
excited energy levels changes the spectrum from a double-peak structure (the
so-called vacuum field Rabi splitting) to a single peak structure. We also
point out that the spin dynamics in the region of the double-peak structure
corresponds to recent experiments using cavity ringing while in region of the
single peak structure, it corresponds to the coherent Rabi oscillation in a
driving electromagnetic filed. Using a standard Lindblad type mechanism, we
study the effect of dissipations on the line width and separation in the
computed spectra. In particular, we study the relaxation of the total spin in
the general case of a spin ensemble in which the total spin of the system is
not specified. The theoretical results are correlated with experimental
evidence of the strong coupling regime, achieved with a spin 1/2 ensemble
Tunable multi-photon Rabi oscillations in an electronic spin system
We report on multi-photon Rabi oscillations and controlled tuning of a
multi-level system at room temperature (S=5/2 for Mn2+:MgO) in and out of a
quasi-harmonic level configuration. The anisotropy is much smaller than the
Zeeman splittings, such as the six level scheme shows only a small deviation
from an equidistant diagram. This allows us to tune the spin dynamics by either
compensating the cubic anisotropy with a precise static field orientation, or
by microwave field intensity. Using the rotating frame approximation, the
experiments are very well explained by both an analytical model and a
generalized numerical model. The calculated multi-photon Rabi frequencies are
in excellent agreement with the experimental data
How Do Schr\"odinger's Cats Die?
Recent experiments with superconducting qubits are motivated by the goal of
fabricating a quantum computer, but at the same time they illuminate the more
fundamental aspects of quantum mechanics. In this paper we analyze the physics
of switching current measurements from the point of view of macroscopic quantum
mechanics.Comment: 4 figures, 12 page
Multi-photon Rabi oscillations in high spin paramagnetic impurity
We report on multiple photon monochromatic quantum oscillations (Rabi
oscillations) observed by pulsed EPR (Electron Paramagnetic Resonance) of
Mn (S=5/2) impurities in MgO. We find that when the microwave magnetic
field is similar or large than the anisotropy splitting, the Rabi oscillations
have a spectrum made of many frequencies not predicted by the S=1/2 Rabi model.
We show that these new frequencies come from multiple photon coherent
manipulation of the multi-level spin impurity. We develop a model based on the
crystal field theory and the rotating frame approximation, describing the
observed phenomenon with a very good agreement.Comment: International Conference: Resonance in Condensed Matter Altshuler 10
Coherent manipulation of electron spins up to ambient temperatures in Cr(S=1/2) doped KNbO
We report coherent spin manipulation on Cr (\emph{S} = 1/2, \emph{I} =
0) doped KNbO, which constitutes a dilute two-level model relevant for
use as a spin qubit. Rabi oscillations are observed for the first time in a
spin system based on transition metal oxides up to room temperature. At liquid
helium temperature the phase coherence relaxation time \emph{} reaches
s and, with a Rabi frequency of 20 MHz, yields a single qubit
figure of merit \emph{} of about 500. This shows that a diluted ensemble
of Cr (\emph{S} = 1/2) doped KNbO is a potential candidate for
solid-state quantum information processing.Comment: 4 page
Adiabatic Landau-Zener-St\"uckelberg transition with or without dissipation in low spin molecular system V15
The spin one half molecular system V15 shows no barrier against spin
reversal. This makes possible direct phonon activation between the two levels.
By tuning the field sweeping rate and the thermal coupling between sample and
thermal reservoir we have control over the phonon-bottleneck phenomena
previously reported in this system. We demonstrate adiabatic motion of molecule
spins in time dependent magnetic fields and with different thermal coupling to
the cryostat bath. We also discuss the origin of the zero-field tunneling
splitting for a half-integer spin.Comment: to appear in Phys. Rev. B - Rapid Communication
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