Probing the superconducting gap symmetry of PrRu4_{4}Sb12_{12}: A comparison with PrOs4_{4}Sb12_{12}

We report measurements of the magnetic penetration depth $\lambda$ in single crystals of PrRu$_{4}$Sb$_{12}$ down to 0.1 K. Both $\lambda$ and superfluid density $\rho_{s}$ exhibit an exponential behavior for $T$ $<$ 0.5$T_{c}$, with parameters $\Delta$(0)/\textit{k}$_{B}$\textit{T}$_{c}$ = 1.9 and $\lambda(0)$ = 2900 \AA. The value of $\Delta$(0) is consistent with the specific-heat jump value of $\Delta C/\gamma T_{c}$ = 1.87 measured elsewhere, while the value of $\lambda(0)$ is consistent with the measured value of the electronic heat-capacity coefficient $\gamma$. Our data are consistent with PrRu$_{4}$Sb$_{12}$ being a moderate-coupling, fully-gapped superconductor. We suggest experiments to study how the nature of the superconducting state evolves with increasing Ru substitution for Os

Mixed-parity superconductivity in centrosymmetric crystals

A weak-coupling formalism for superconducting states possessing both singlet (even parity) and triplet (odd parity) components of the order parameter in centrosymmetric crystals is developed. It is shown that the quasiparticle energy spectrum may be non-degenerate even if the triplet component is unitary. The superconducting gap of a mixed-parity state may have line nodes in the strong spin-orbit coupling limit. The pseudospin carried by the superconducting electrons is calculated, from which follows a prediction of a kink anomaly in the temperature dependence of muon spin relaxation rate. The anomaly occurs at the phase boundary between the bare triplet and mixed-parity states. The stability of mixed-parity states is discussed within Ginzburg-Landau theory. The results may have immediate application to the superconducting series Pr(Os,Ru)4Sb12.Comment: 5 pages, 2 figures. Final version accepted to PR

Superconductivity and crystalline electric field effects in the filled skutterudite series Pr(Os1−x_{1-x}Rux_x)4_4Sb12_{12}

X-ray powder diffraction, magnetic susceptibility $\chi(T)$, and electrical resistivity $\rho(T)$ measurements were made on single crystals of the filled skutterudite series Pr(Os$_{1-x}$Ru$_x$)$_4$Sb$_{12}$. One end of the series ($x = 0$) is a heavy fermion superconductor with a superconducting critical temperature $T_{c} = 1.85$ K, while the other end ($x = 1$) is a conventional superconductor with $T_{c} \approx 1$ K. The lattice constant $a$ decreases approximately linearly with increasing Ru concentration $x$. As Ru (Os) is substituted for Os (Ru), $T_{c}$ decreases nearly linearly with substituent concentration and exhibits a minimum with a value of $T_{c} = 0.75$ K at $x = 0.6$, suggesting that the two types of superconductivity compete with one another. Crystalline electric field (CEF) effects in $\chi_\mathrm{dc}(T)$ and $\rho(T)$ due to the splitting of the Pr$^{3+}$ nine-fold degenerate Hund's rule $J = 4$ multiplet are observed throughout the series, with the splitting between the ground state and the first excited state increasing monotonically as $x$ increases. The fits to the $\chi_\mathrm{dc}(T)$ and $\rho(T)$ data are consistent with a $\Gamma_{3}$ doublet ground state for all values of x, although reasonable fits can be obtained for a $\Gamma_{1}$ ground state for $x$ values near the end member compounds ($x = 0$ or $x = 1$).Comment: 10 pages, 8 figures, submitted to Phys. Rev.

Evidence for Photoinduced Insulator-to-Metal transition in B-phase vanadium dioxide

10.1038/srep25538Scientific Reports62553

Dual phases of crystalline and electronic structures in the nanocrystalline perovskite CsPbBr3

NPG Asia Materials1117

Terahertz conductivity of twisted bilayer graphene

10.1103/PhysRevLett.110.067401Physical Review Letters1106-PRLT

Ultrafast optical spectroscopy of strongly correlated materials and high-temperature superconductors: a non-equilibrium approach

In the last two decades non-equilibrium spectroscopies have evolved from avant-garde studies to crucial tools for expanding our understanding of the physics of strongly correlated materials. The possibility of obtaining simultaneously spectroscopic and temporal information has led to insights that are complementary to (and in several cases beyond) those attainable by studying the matter at equilibrium. From this perspective, multiple phase transitions and new orders arising from competing interactions are benchmark examples where the interplay among electrons, lattice and spin dynamics can be disentangled because of the different timescales that characterize the recovery of the initial ground state. For example, the nature of the broken-symmetry phases and of the bosonic excitations that mediate the electronic interactions, eventually leading to superconductivity or other exotic states, can be revealed by observing the sub-picosecond dynamics of impulsively excited states. Furthermore, recent experimental and theoretical developments have made it possible to monitor the time-evolution of both the single-particle and collective excitations under extreme conditions, such as those arising from strong and selective photo-stimulation. These developments are opening the way for new, non-equilibrium phenomena that can eventually be induced and manipulated by short laser pulses. Here, we review the most recent achievements in the experimental and theoretical studies of the non-equilibrium electronic, optical, structural and magnetic properties of correlated materials. The focus will be mainly on the prototypical case of correlated oxides that exhibit unconventional superconductivity or other exotic phases. The discussion will also extend to other topical systems, such as iron-based and organic superconductors, (Formula presented.) and charge-transfer insulators. With this review, the dramatically growing demand for novel experimental tools and theoretical methods, models and concepts, will clearly emerge. In particular, the necessity of extending the actual experimental capabilities and the numerical and analytic tools to microscopically treat the non-equilibrium phenomena beyond the simple phenomenological approaches represents one of the most challenging new frontiers in physics