4,324 research outputs found
A possible chiral spin-liquid phase in non-centrosymmetric BaCoO
Based on a symmetry approach, we propose a possible explanation of the weak
ferromagnetic component recently observed in YBaCoFeO (Valldor et al.
Phys Rev B, 224426 (2011)) and other isostructural compounds in the
high-temperature spin-liquid phase. Due to the polar nature of their crystal
structure, a coupling between time-odd scalar spin chirality which we suggest
as the primary order parameter and macroscopic magnetization is possible as
follows from the general form of the appropriate free-energy invariant. The
deduced pseudoproper coupling between both physical quantities provides a
unique possibility to study the critical behaviour of the chiral order
parameter
Magnetically-induced ferroelectricity in the (ND4)2[FeCl5(D2O)] molecular compound
The number of magnetoelectric multiferroic materials reported to date is
scarce, as magnetic structures that break inversion symmetry and induce an
improper ferroelectric polarization typically arise through subtle competition
between different magnetic interactions. The (NH4)2[FeCl5(H2O)] compound is a
rare case where such improper ferroelectricity has been observed in a molecular
material. We have used single crystal and powder neutron diffraction to obtain
detailed solutions for the crystal and magnetic structures of
(NH4)2[FeCl5(H2O)], from which we determined the mechanism of multiferroicity.
From the crystal structure analysis, we observed an order-disorder phase
transition related to the ordering of the ammonium counterion. We have
determined the magnetic structure below TN, at 2K and zero magnetic field,
which corresponds to a cycloidal spin arrangement with magnetic moments
contained in the ac-plane, propagating parallel to the c-axis. The observed
ferroelectricity can be explained, from the obtained magnetic structure, via
the inverse Dzyaloshinskii-Moriya mechanism
Spin-stripe phase in a frustrated zigzag spin-1/2 chain
Motifs of periodic modulations are encountered in a variety of natural
systems, where at least two rival states are present. In strongly correlated
electron systems such behaviour has typically been associated with competition
between short- and long-range interactions, e.g., between exchange and
dipole-dipole interactions in the case of ferromagnetic thin films. Here we
show that spin-stripe textures may develop also in antiferromagnets, where
long-range dipole-dipole magnetic interactions are absent. A comprehensive
analysis of magnetic susceptibility, high-field magnetization, specific heat,
and neutron diffraction measurements unveils -TeVO as a nearly
perfect realization of a frustrated (zigzag) ferromagnetic spin-1/2 chain.
Strikingly, a narrow spin stripe phase develops at elevated magnetic fields due
to weak frustrated short-range interchain exchange interactions possibly
assisted by the symmetry allowed electric polarization. This concept provides
an alternative route for the stripe formation in strongly correlated electron
systems and may help understanding other widespread, yet still elusive,
stripe-related phenomena.Comment: accapted in Nature Communication
Enhanced ferroelectric polarization by induced Dy spin-order in multiferroic DyMnO3
Neutron powder diffraction and single crystal x-ray resonant magnetic
scattering measurements suggest that Dy plays an active role in enhancing the
ferroelectric polarization in multiferroic DyMnO3 above TNDy = 6.5 K. We
observe the evolution of an incommensurate ordering of Dy moments with the same
periodicity as the Mn spiral ordering. It closely tracks the evolution of the
ferroelectric polarization which reaches a maximum value of 0.2 muC/m^2. Below
TNDy, where Dy spins order commensurately, the polarization decreases to values
similar for those of TbMnO3
Trisomy 19 ependymoma, a newly recognized genetico-histological association, including clear cell ependymoma
Ependymal tumors constitute a clinicopathologically heterogeneous group of brain tumors. They vary in regard to their age at first symptom, localization, morphology and prognosis. Genetic data also suggests heterogeneity. We define a newly recognized subset of ependymal tumors, the trisomy 19 ependymoma. Histologically, they are compact lesions characterized by a rich branched capillary network amongst which tumoral cells are regularly distributed. When containing clear cells they are called clear cell ependymoma. Most trisomy 19 ependymomas are supratentorial WHO grade III tumors of the young. Genetically, they are associated with trisomy 19, and frequently with a deletion of 13q21.31-31.2, three copies of 11q13.3-13.4, and/or deletions on chromosome 9. These altered chromosomal regions are indicative of genes and pathways involved in trisomy 19 ependymoma tumorigenesis. Recognition of this genetico-histological entity allows better understanding and dissection of ependymal tumors
Electric field control of the magnetic chiralities in ferroaxial multiferroic RbFe(MoO4)2
The coupling of magnetic chiralities to the ferroelectric polarisation in
multiferroic RbFe(MoO) is investigated by neutron spherical
polarimetry. Because of the axiality of the crystal structure below
= 190 K, helicity and triangular chirality are
symmetric-exchange coupled, explaining the onset of the ferroelectricity in
this proper-screw magnetic structure - a mechanism that can be generalised to
other systems with "ferroaxial" distortions in the crystal structure. With an
applied electric field we demonstrate control of the chiralities in both
structural domains simultaneously.Comment: 5 pages, 4 figure
Magnetic order in the frustrated Ising-like chain compound SrNiIrO
We have studied the field and temperature dependence of the magnetization of
single crystals of Sr3NiIrO6. These measurements evidence the presence of an
easy axis of anisotropy and two anomalies in the magnetic susceptibility.
Neutron powder diffraction realized on a polycrystalline sample reveals the
emergence of magnetic reflections below 75 K with magnetic propagation vector k
~ (0, 0, 1), undetected in previous neutron studies [T.N. Nguyen and H.-C zur
Loye, J. Solid State Chem., 117, 300 (1995)]. The nature of the magnetic ground
state, and the presence of two anomalies common to this family of material, are
discussed on the basis of the results obtained by neutron diffraction,
magnetization measurements, and symmetry arguments
The structure of intercalated water in superconducting NaCoO1.37DO: Implications for the superconducting phase diagram
We have used electron and neutron powder diffraction to elucidate the
structural properties of superconducting \NaD. Our measurements show that our
superconducting sample exhbits a number of supercells ranging from
to , but the most predominant one, observed also in the neutron
data, is a double hexagonal cell with dimensions \dhx. Rietveld analysis
reveals that \deut\space is inserted between CoO sheets as to form a
layered network of NaO triangular prisms. Our model removes the need to
invoke a 5K superconducting point compound and suggests that a solid solution
of Na is possible within a constant amount of water .Comment: 4 pages, 3 figure
Prediction for new magnetoelectric fluorides
We use symmetry considerations in order to predict new magnetoelectric
fluorides. In addition to these magnetoelectric properties, we discuss among
these fluorides the ones susceptible to present multiferroic properties. We
emphasize that several materials present ferromagnetic properties. This
ferromagnetism should enhance the interplay between magnetic and dielectric
properties in these materials.Comment: 12 pages, 4 figures, To appear in Journal of Physics: Condensed
Matte
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