111 research outputs found
Superexchange coupling and spin susceptibility spectral weight in undoped monolayer cuprates
A systematic inelastic neutron scattering study of the superexchange
interaction in three different undoped monolayer cuprates (La_2CuO_4, Nd_2CuO_4
and Pr_2CuO_4) has been performed using conventional triple axis technique. We
deduce the in-plane antiferromagnetic (AF) superexchange coupling which
actually presents no simple relation versus crystallographic parameters. The
absolute spectral weight of the spin susceptibility has been obtained and it is
found to be smaller than expected even when quantum corrections of the AF
ground state are taken into account.Comment: 13 pages, 1 table, 3 figure
Assessment of PM10 and heavy metal concentration in a ceramic cluster (NE Spain) and the influence on nearby soils
Environmental pollution control is one of the most important goals in pollution risk assessment today. The aim of this study is to conduct a retrospective view of the evolution of matter particulate (PM10) and the heavy metals (Cd, Ni and Pb) at different localities (Alcora, Castellón and Onda) in the Spanish cluster ceramic in a period between January 2007 and December 2011. The study area is in the province of Castellón. This province is a strategic area in the framework of European Union Pollution control. Approximately 80% of European ceramic tiles and ceramic frits manufacturers are concentrated in two areas, forming the so-called "ceramic clusters"; one is in Modena (Italy) and the other in Castellón (Spain). In these kind of areas, there are a lot of pollutants from this industry that represent an important contribution to soil contamination so it is necessary to control their air quality. In these areas atmospheric particles are deposited in the ground through both dry and wet deposition. Soil is a major sink for heavy metals released into the environment. For this purpose the levels of PM10 in ambient air and the corresponding annual and seasonal trend were calculated. The results of the study show that the PM10 and heavy metal concentrations are below the limit values recommended by European Union Legislation for the protection of human health and ecosystems in the study period. There is an important reduction of them from 2009 in all control stations due to economic crisis and subsequent decrease of industrial activity. The atmospheric seasonal tendency of pollutant concentrations is marked by the rate of industrial activity and additionally by the temperature. Complementarily, a comparative study of heavy metal levels in soils was performed in this area. Soils with low pollution by Ni and Pb were detected, while different pollution by Cd was found depending on the sampling site. Although there is an evident reduction of PM10 and heavy metal levels, the results show that these pollut
Model for the low-temperature magnetic phases observed in doped YBa_2Cu_3O_{6+x}
A classical statistical model for the antiferromagnetic (AFM) ordering of the
Cu-spins in the CuO_2 planes of reduced YBa_2Cu_3O_{6+x} type materials is
presented. The magnetic phases considered are the experimentally observed
high-temperature AFI phase with ordering vector Q_I=(1/2,1/2,0), and the
low-temperature phases: AFII with Q_II=(1/2,1/2,1/2) and intermediate TA (Turn
Angle) phases TAI, TAII and TAIII with components of both ordering vectors. It
is shown that the AFII and TA phases result from an effective ferromagnetic
(FM) type coupling mediated by free spins in the CuO_x basal plane. Good
agreement with experimental data is obtained for realistic model parameters.Comment: 11 pages, 2 Postscript figures, Submitted to Phys.Rev.Let
Neutron scattering search for static magnetism in oxygen ordered YBa2Cu3O6.5
We present elastic and inelastic neutron scattering results on highly oxygen
ordered YBa2Cu3O6.5 ortho-II. We find no evidence for the presence of ordered
magnetic moments to a sensitivity of 0.003 Bohr magnetons, an order of
magnitude smaller than has been suggested in theories of orbital or
d-density-wave (DDW) currents. The absence of sharp elastic peaks, shows that
the d-density-wave phase is not present, at least for the superconductor with
the doping of 6.5 and the ordered ortho-II structure. We cannot exclude the
possibility that a broad peak may exist with extremely short-range DDW
correlations. For less ordered or more doped crystals it is possible that
disorder may lead to static magnetism. We have also searched for the large
normal state spin gap that is predicted to exist in an ordered DDW phase.
Instead of a gap we find that the Q-correlated spin susceptibility persists to
the lowest energies studied, 6 meV. Our results are compatible with the
coexistence of superconductivity with orbital currents, but only if they are
dynamic, and exclude a sharp phase transition to an ordered d-density-wave
phase.Comment: 6 pages 4 figures RevTex Submitted to Phys Rev B January 23, 200
Beyond the limits of oxygen: effects of hypoxia in a hormone-independent prostate cancer cell line
Prostate cancer (PCa) has a high incidence worldwide. One of the major causes of PCa resistance is intratumoral hypoxia. In solid tumors, hypoxia is strongly associated with malignant progression and resistance to therapy, which is an indicator of poor prognosis. The antiproliferative effect and induced death caused by doxorubicin, epirubicin, cisplatin, and flutamide in a hormone-independent PCa cell line will be evaluated. The hypoxia effect on drug resistance to these drugs, as well as cell proliferation and migration, will be also analyzed. All drugs induced an antiproliferative effect and also cell death in the cell line under study. Hypoxia made the cells more resistant to all drugs. Moreover, our results reveal that long time cell exposure to hypoxia decreases cellular proliferation and migration. Hypoxia can influence cellular resistance, proliferation, and migration. This study shows that hypoxia may be a key factor in the regulation of PCa.info:eu-repo/semantics/publishedVersio
Low energy magnetic excitations of the Mn_{12}-acetate spin cluster observed by neutron scattering
We performed high resolution diffraction and inelastic neutron scattering
measurements of Mn_{12}-acetate. Using a very high energy resolution, we could
separate the energy levels corresponding to the splitting of the lowest S
multiplet. Data were analyzed within a single spin model (S=10 ground state),
using a spin Hamiltonian with parameters up to 4^{th} order.
The non regular spacing of the transition energies unambiguously shows the
presence of high order terms in the anisotropy (D= -0.457(2) cm^{-1}, B_4^0 =
-2.33(4) 10^{-5}cm^{-1}).
The relative intensity of the lowest energy peaks is very sensitive to the
small transverse term, supposed to be mainly responsible for quantum tunneling.
This allows an accurate determination of this term in zero magnetic field
(B_4^4 = \pm 3.0(5) 10^{-5} cm^{-1}). The neutron results are discussed in view
of recent experiments and theories.Comment: 4 pages ? 3 figures, submitted to Physical Review Lette
Antiferromagnetic ordering in a 90 K copper oxide superconductor
Using elastic neutron scattering, we evidence a commensurate
antiferromagnetic Cu(2) order (AF) in the superconducting (SC) high-
cuprate (y=0.013, =93 K). As
in the Co-free system, the spin excitation spectrum is dominated by a magnetic
resonance peak at 41 meV but with a reduced spectral weight. The substitution
of Co thus leads to a state where AF and SC cohabit showing that the CuO
plane is a highly antiferromagnetically polarizable medium even for a sample
where T remains optimum.Comment: 3 figure
4f-spin dynamics in La(2-x-y)Sr(x)Nd(y)CuO(4)
We have performed inelastic magnetic neutron scattering experiments on
La(2-x-y)Sr(x)Nd(y)CuO(4) in order to study the Nd 4f-spin dynamics at low
energies. In all samples we find at high temperatures a quasielastic line
(Lorentzian) with a line width which decreases on lowering the temperature. The
temperature dependence of the quasielastic line width Gamma/2(T) can be
explained with an Orbach-process, i.e. a relaxation via the coupling between
crystal field excitations and phonons. At low temperatures the Nd-4f magnetic
response S(Q,omega) correlates with the electronic properties of the
CuO(2)-layers. In the insulator La(2-y)Nd(y)CuO(4) the quasielastic line
vanishes below 80 K and an inelastic excitation occurs. This directly indicates
the splitting of the Nd3+ ground state Kramers doublet due to the static
antiferromagnetic order of the Cu moments. In La(1.7-x)Sr(x)Nd(0.3)CuO(4) with
x = 0.12, 0.15 and La(1.4-x)Sr(x)Nd(0.6)CuO(4) with x = 0.1, 0.12, 0.15, 0.18
superconductivity is strongly suppressed. In these compounds we observe a
temperature independent broad quasielastic line of Gaussian shape below T about
30 K. This suggests a distribution of various internal fields on different Nd
sites and is interpreted in the frame of the stripe model. In
La(1.8-y)Sr(0.2)Nd(y)CuO(4) (y = 0.3, 0.6) such a quasielastic broadening is
not observed even at lowest temperature.Comment: 8 pages, 10 figures included, to appear in Phys. Rev.
Systematics of two-component superconductivity in from microwave measurements of high quality single crystals
Systematic microwave surface impedance measurements of YBCO single crystals
grown in crucibles reveal new properties that are not directly seen
in similar measurements of other YBCO samples. Two key observations obtained
from complex conductivity are: a new normal conductivity peak at around 80K and
additional pairing below 65K. High pressure oxygenation of one of the crystals
still yields the same results ruling out any effect of macroscopic segregation
of O-deficient regions. A single complex order parameter cannot describe these
data, and the results suggest at least two superconducting components.
Comparisons with model calculations done for various decoupled two-component
scenarios (i.e. s+d, d+d) are presented. Systematics of three single crystals
show that the 80K quasiparticle peak is correlated with the normal state
inelastic scattering rate. Close to Tc, the data follow a mean-field behavior.
Overall, our results strongly suggest the presence of multiple pairing
temperature and energy scales in .Comment: 14 pages, 2-column, Revtex, 5 embedded postscript figures, uses
graphicx. Postscript version also available at
http://sagar.physics.neu.edu/preprints.htm
How to detect fluctuating order in the high-temperature superconductors
We discuss fluctuating order in a quantum disordered phase proximate to a
quantum critical point, with particular emphasis on fluctuating stripe order.
Optimal strategies for extracting information concerning such local order from
experiments are derived with emphasis on neutron scattering and scanning
tunneling microscopy. These ideas are tested by application to two model
systems - the exactly solvable one dimensional electron gas with an impurity,
and a weakly-interacting 2D electron gas. We extensively review experiments on
the cuprate high-temperature superconductors which can be analyzed using these
strategies. We adduce evidence that stripe correlations are widespread in the
cuprates. Finally, we compare and contrast the advantages of two limiting
perspectives on the high-temperature superconductor: weak coupling, in which
correlation effects are treated as a perturbation on an underlying metallic
(although renormalized) Fermi liquid state, and strong coupling, in which the
magnetism is associated with well defined localized spins, and stripes are
viewed as a form of micro-phase separation. We present quantitative indicators
that the latter view better accounts for the observed stripe phenomena in the
cuprates.Comment: 43 pages, 11 figures, submitted to RMP; extensively revised and
greatly improved text; one new figure, one new section, two new appendices
and more reference
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