16 research outputs found
A possible mechanism for superconductivity in doped SrTiO3
The soft ferro-electric phonon in SrTiO3 observed with optical spectroscopy
has an extraordinary strong spectral weight which is much stronger than
expected in the limit of a perfectly ionic compound. The "charged phonon" in
SrTiO3 is caused by the close-to-covalent character of the Ti-O ionic bond and
implies a strong coupling between the soft ferro-electric phonon and the inter
band transitions across the 3 eV gap of SrTiO3. We demonstrate that this
coupling leads, in addition to the charged phonon effect, to a pairing
interaction involving the exchange of two transverse optical phonons. This
process owes its relevance to the strong electron-phonon coupling and to the
fact that the interaction mediated by a single transverse optical phonon
vanishes at low electron density. We use the experimental soft phonon spectral
weight to calculate the strength of the bi-phonon mediated pairing interaction
in the electron doped material and show that it is of the correct magnitude
when compared to the experimental value of the superconducting critical
temperature.Comment: Missing factors corrected in Eqs. 6 and
BaCu3O4: High Temperature Magnetic Order in One-Dimensional S=1/2 Diamond-Chains
The magnetic properties of the alkaline earth oxocuprate BaCu3O4 are
investigated. We show that the characteristic Cu3O4 layers of this material can
be described with diamond chains of antiferromagnetically coupled Cu 1/2 spins
with only a weak coupling between two adjacent chains. These Cu3O4 layers seem
to represent a so far unique system of weakly coupled one-dimensional magnetic
objects where the local AF ordering of the Cu2+ ions leads to an actual net
magnetic moment of an isolated diamond chain. We demonstrate a magnetic
transition at a high N\'eel temperature T_{N}=336 K
Mott transition and collective charge pinning in electron doped Sr2IrO4
We studied the in-plane dynamic and static charge conductivity of electron
doped Sr2IrO4 using optical spectroscopy and DC transport measurements. The
optical conductivity indicates that the pristine material is an indirect
semiconductor with a direct Mott-gap of 0.55 eV. Upon substitution of 2% La per
formula unit the Mott-gap is suppressed except in a small fraction of the
material (15%) where the gap survives, and overall the material remains
insulating. Instead of a zero energy mode (or Drude peak) we observe a soft
collective mode (SCM) with a broad maximum at 40 meV. Doping to 10% increases
the strength of the SCM, and a zero-energy mode occurs together with metallic
DC conductivity. Further increase of the La substitution doesn't change the
spectral weight integral up to 3 eV. It does however result in a transfer of
the SCM spectral weight to the zero-energy mode, with a corresponding reduction
of the DC resistivity for all temperatures from 4 to 300 K. The presence of a
zero-energy mode signals that at least part of the Fermi surface remains
ungapped at low temperatures, whereas the SCM appears to be caused by pinning a
collective frozen state involving part of the doped electrons
Mott transition and collective charge pinning in electron doped Sr_2IrO_4
We studied the in-plane dynamic and static charge conductivity of electron doped Sr_2IrO_4 using optical spectroscopy and DC transport measurements. The optical conductivity indicates that the pristine material is an indirect semiconductor with a direct Mott gap of 0.55 eV. Upon substitution of 2% La per formula unit the Mott gap is suppressed except in a small fraction of the material (15%) where the gap survives, and overall the material remains insulating. Instead of a zero energy mode (or Drude peak) we observe a soft collective mode (SCM) with a broad maximum at 40 meV. Doping to 10%
increases the strength of the SCM, and a zero-energy mode occurs together with metallic DC conductivity. Further increase of the La substitution doesn't change the spectral weight integral up to 3 eV. It does however result in a transfer of the SCM spectral weight to the zero-energy mode, with a corresponding reduction of the DC resistivity for all temperatures from 4 to 300 K. The presence of a zero-energy mode signals that at least part of the Fermi surface remains ungapped at low temperatures, whereas the SCM appears to be caused by pinning a collective frozen state involving part of the doped electrons
Mott transition and collective charge pinning in electron doped Sr_2IrO_4
We studied the in-plane dynamic and static charge conductivity of electron doped Sr_2IrO_4 using optical spectroscopy and DC transport measurements. The optical conductivity indicates that the pristine material is an indirect semiconductor with a direct Mott gap of 0.55 eV. Upon substitution of 2% La per formula unit the Mott gap is suppressed except in a small fraction of the material (15%) where the gap survives, and overall the material remains insulating. Instead of a zero energy mode (or Drude peak) we observe a soft collective mode (SCM) with a broad maximum at 40 meV. Doping to 10%
increases the strength of the SCM, and a zero-energy mode occurs together with metallic DC conductivity. Further increase of the La substitution doesn't change the spectral weight integral up to 3 eV. It does however result in a transfer of the SCM spectral weight to the zero-energy mode, with a corresponding reduction of the DC resistivity for all temperatures from 4 to 300 K. The presence of a zero-energy mode signals that at least part of the Fermi surface remains ungapped at low temperatures, whereas the SCM appears to be caused by pinning a collective frozen state involving part of the doped electrons
Charge puddles in a completely compensated topological insulator
International audienceCompensation of intrinsic charges is widely used to reduce the bulk conductivity of 3D topological insulators (TIs). Here we use low temperature electron irradiation-induced defects paired with in situ electrical transport measurements to fine-tune the degree of compensation in Bi2Te3. The coexistence of electrons and holes at the point of optimal compensation can only be explained by bulk carriers forming charge puddles. These need to be considered to understand the electric transport in compensated TI samples, irrespective of the method of compensation
Thermodynamic signatures of the field-induced states of graphite
Previous transport studies of graphite in strong magnetic fields have found a sequence of phase transitions with a still unresolved microscopic origin. Here the authors present ultrasound measurements enabling sharper resolution and demonstrating the thermodynamic nature of these transitions