224 research outputs found
Wetting to Non-wetting Transition in Sodium-Coated C_60
Based on ab initi and density-functional theory calculations, an empirical
potential is proposed to model the interaction between a fullerene molecule and
many sodium atoms. This model predicts homogeneous coverage of C_60 below 8 Na
atoms, and a progressive droplet formation above this size. The effects of
ionization, temperature, and external electric field indicate that the various,
and apparently contradictory, experimental results can indeed be put into
agreement.Comment: 4 pages, 4 postscript figure
Effect of in-plane line defects on field-tuned superconductor-insulator transition behavior in homogeneous thin film
Field-tuned superconductor-insulator transition (FSIT) behavior in 2D
isotropic and homogeneous thin films is usually accompanied by a nonvanishing
critical resistance at low . It is shown that, in a 2D film including line
defects paralle to each other but with random positions perpendicular to them,
the (apparent) critical resistance in low limit vanishes, as in the 1D
quantum superconducting (SC) transition, under a current parallel to the line
defects. This 1D-like critical resistive behavior is more clearly seen in
systems with weaker point disorder and may be useful in clarifying whether the
true origin of FSIT behavior in the parent superconductor is the glass
fluctuation or the quantum SC fluctuation. As a by-product of the present
calculation, it is also pointed out that, in 2D films with line-like defects
with a long but {\it finite} correlation length parallel to the lines, a
quantum metallic behavior intervening the insulating and SC ones appears in the
resistivity curves.Comment: 16 pages, 14 figure
Coexistence of glassy antiferromagnetism and giant magnetoresistance (GMR) in Fe/Cr multilayer structures
Using temperature-dependent magnetoresistance and magnetization measurements
on Fe/Cr multilayers that exhibit pronounced giant magnetoresistance (GMR), we
have found evidence for the presence of a glassy antiferromagnetic (GAF) phase.
This phase reflects the influence of interlayer exchange coupling (IEC) at low
temperature (T < 140K) and is characterized by a field-independent glassy
transition temperature, Tg, together with irreversible behavior having
logarithmic time dependence below a "de Almeida and Thouless" (AT) critical
field line. At room temperature, where the GMR effect is still robust, IEC
plays only a minor role, and it is the random potential variations acting on
the magnetic domains that are responsible for the antiparallel interlayer
domain alignment.Comment: 5 pages, 4 figure
Important role of alkali atoms in A4C60
We show that hopping via the alkali atoms plays an important role for the t1u
band of A4C60 (A=K, Rb), in strong contrast to A3C60. Thus the t1u band is
broadened by more than 40 % by the presence of the alkali atoms. The difference
between A4C60 and A3C60 is in particular due to the less symmetric location of
the alkali atoms in A4C60.Comment: 5 pages, revtex, 2 figures, submitted to Phys. Rev. B more
information at http://www.mpi-stuttgart.mpg.de/dokumente/andersen/fullerene
Vertex-corrected tunneling inversion in superconductors: Pb
The McMillan-Rowell tunneling inversion program, which extracts the
electron-phonon spectral function and the Coulomb
pseudopotential from experimental tunneling data, is generalized to
include the lowest-order vertex correction. We neglect the momentum dependence
of the electron-phonon matrix elements, which is equivalent to using a local
approximation. The perturbation theory is performed on the imaginary axis and
then an exact analytic continuation is employed to produce the density of
states on the real axis. Comparison is made with the experimental data for Pb.Comment: 14 pages, typeset in ReVTeX, including three encapsulated postscript
figure
Electronic interactions in fullerene spheres
The electron-phonon and Coulomb interactions inC, and larger fullerene
spheres are analyzed. The coupling between electrons and intramolecular
vibrations give corrections meV to the electronic energies for
C, and scales as in larger molecules. The energies associated
with electrostatic interactions are of order eV, in C and
scale as . Charged fullerenes show enhanced electron-phonon coupling,
meV, which scales as . Finally, it is argued that non only
C, but also C are highly polarizable molecules. The
polarizabilities scale as and , respectively. The role of this large
polarizability in mediating intermolecular interactions is also discussed.Comment: 12 pages. No figure
Mean Field Theory of the Localization Transition
A mean field theory of the localization transition for bosonic systems is
developed. Localization is shown to be sensitive to the distribution of the
random site energies. It occurs in the presence of a triangular distribution,
but not a uniform one. The inverse participation ratio, the single site Green's
function, the superfluid order parameter and the corresponding susceptibility
are calculated, and the appropriate exponents determined. All of these
quantities indicate the presence of a new phase, which can be identified as the
{\it Bose-glass}.Comment: 4 pages, Revtex, 2 figures appende
Possible first order transition in the two-dimensional Ginzburg-Landau model induced by thermally fluctuating vortex cores
We study the two-dimensional Ginzburg-Landau model of a neutral superfluid in
the vicinity of the vortex unbinding transition. The model is mapped onto an
effective interacting vortex gas by a systematic perturbative elimination of
all fluctuating degrees of freedom (amplitude {\em and} phase of the order
parameter field) except the vortex positions. In the Coulomb gas descriptions
derived previously in the literature, thermal amplitude fluctuations were
neglected altogether. We argue that, if one includes the latter, the vortices
still form a two- dimensional Coulomb gas, but the vortex fugacity can be
substantially raised. Under the assumption that Minnhagen's generic phase
diagram of the two- dimensional Coulomb gas is correct, our results then point
to a first order transition rather than a Kosterlitz-Thouless transition,
provided the Ginzburg-Landau correlation length is large enough in units of a
microscopic cutoff length for fluctuations. The experimental relevance of these
results is briefly discussed. [Submitted to J. Stat. Phys.]Comment: 36 pages, LaTeX, 6 figures upon request, UATP2-DB1-9
Anomalous Quantum Diffusion at the Superfluid-Insulator Transition
We consider the problem of the superconductor-insulator transition in the
presence of disorder, assuming that the fermionic degrees of freedom can be
ignored so that the problem reduces to one of Cooper pair localization. Weak
disorder drives the critical behavior away from the pure critical point,
initially towards a diffusive fixed point. We consider the effects of Coulomb
interactions and quantum interference at this diffusive fixed point. Coulomb
interactions enhance the conductivity, in contrast to the situation for
fermions, essentially because the exchange interaction is opposite in sign. The
interaction-driven enhancement of the conductivity is larger than the
weak-localization suppression, so the system scales to a perfect conductor.
Thus, it is a consistent possibility for the critical resistivity at the
superconductor-insulator transition to be zero, but this value is only
approached logarithmically. We determine the values of the critical exponents
and comment on possible implications for the interpretation of
experiments
Electron--Vibron Interactions and Berry Phases in Charged Buckminsterfullerene: Part I
A simple model for electron-vibron interactions on charged
buckminsterfullerene C, , is solved both at weak and
strong couplings. We consider a single vibrational multiplet interacting
with electrons. At strong coupling the semiclassical dynamical
Jahn-Teller theory is valid. The Jahn-Teller distortions are unimodal for
=1,2,4,5 electrons, and bimodal for 3 electrons. The distortions are
quantized as rigid body pseudo--rotators which are subject to geometrical Berry
phases. These impose ground state degeneracies and dramatically change zero
point energies. Exact diagonalization shows that the semiclassical level
degeneracies and ordering survive well into the weak coupling regime. At weak
coupling, we discover an enhancement factor of for the pair binding
energies over their classical values. This has potentially important
implications for superconductivity in fullerides, and demonstrates the
shortcoming of Migdal--Eliashberg theory for molecular crystals.Comment: 29 pages (+7 figures, 3 available upon request), LATEX,
report-number: BM515
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