Charge migration in organic materials: Can propagating charges affect the key physical quantities controlling their motion?

Charge migration is a ubiquitous phenomenon with profound implications throughout many areas of chemistry, physics, biology and materials science. The long-term vision of designing functional materials with tailored molecular scale properties has triggered an increasing quest to identify prototypical systems where truly molecular conduction pathways play a fundamental role. Such pathways can be formed due to the molecular organization of various organic materials and are widely used to discuss electronic properties at the nanometer scale. Here, we present a computational methodology to study charge propagation in organic molecular stacks at nano and sub-nanoscales and exploit this methodology to demonstrate that moving charge carriers strongly affect the values of the physical quantities controlling their motion. The approach is also expected to find broad application in the field of charge migration in soft matter systems.Comment: 18 pages, 6 figures, accepted for publication in the Israel Journal of Chemistr

Mixing by Swimming Algae

In this fluid dynamics video, we demonstrate the microscale mixing enhancement of passive tracer particles in suspensions of swimming microalgae, Chlamydomonas reinhardtii. These biflagellated, single-celled eukaryotes (10 micron diameter) swim with a "breaststroke" pulling motion of their flagella at speeds of about 100 microns/s and exhibit heterogeneous trajectory shapes. Fluorescent tracer particles (2 micron diameter) allowed us to quantify the enhanced mixing caused by the swimmers, which is relevant to suspension feeding and biogenic mixing. Without swimmers present, tracer particles diffuse slowly due solely to Brownian motion. As the swimmer concentration is increased, the probability density functions (PDFs) of tracer displacements develop strong exponential tails, and the Gaussian core broadens. High-speed imaging (500 Hz) of tracer-swimmer interactions demonstrates the importance of flagellar beating in creating oscillatory flows that exceed Brownian motion out to about 5 cell radii from the swimmers. Finally, we also show evidence of possible cooperative motion and synchronization between swimming algal cells.Comment: 1 page, APS-DFD 2009 Gallery of Fluid Motio

Domain Patterns in the Microwave-Induced Zero-Resistance State

It has been proposed that the microwave-induced ``zero-resistance'' phenomenon, observed in a GaAs two-dimensional electron system at low temperatures in moderate magnetic fields, results from a state with multiple domains, in which a large local electric field \bE(\br) is oriented in different directions. We explore here the questions of what may determine the domain arrangement in a given sample, what do the domains look like in representative cases, and what may be the consequences of domain-wall localization on the macroscopic dc conductance. We consider both effects of sample boundaries and effects of disorder, in a simple model, which has a constant Hall conductivity, and is characterized by a Lyapunov functional.Comment: 19 pages, 5 figures; submitted to a special issue of Journal of Statistical Physics, in honor of P. C. Hohenberg and J. S. Lange

Discovery potential for a charged Higgs boson decaying in the chargino-neutralino channel of the ATLAS detector at the LHC

We have investigated charged Higgs boson production via the gluon-bottom quark mode, gb -> tH+, followed by its decay into a chargino and a neutralino. The calculations are based on masses and couplings given by the Minimal Supersymmetric Standard Model (MSSM) for a specific choice of MSSM parameters. The signature of the signal is characterized by three hard leptons, a substantial missing transverse energy due to the decay of the neutralino and the chargino and three hard jets from the hadronic decay of the top quark. The possibility of detecting the signal over the Standard Model (SM) and non-SM backgrounds was studied for a set of tanBeta and mA. The existence of 5-sigma confidence level regions for H+ discovery at integrated luminosities of 100 fb-1 and 300 fb-1 is demonstrated, which cover also the intermediate region 4 < tanBeta < 10 where H+ decays to SM particles cannot be used for H+ discovery

Elastic Instabilities of Polymer Solutions in Cross-Channel Flow

When polymer molecules pass near the hyperbolic point of a microchannel cross flow, they are strongly stretched. As the strain rate is varied at low Reynolds number ( \u3c 10-2), tracer and particle-tracking experiments show that molecular stretching produces two flow instabilities: one in which the velocity field becomes strongly asymmetric, and a second in which it fluctuates nonperiodically in time. The flow is strongly perturbed even far from the region of instability, and this phenomenon can be used to produce mixing