2,084 research outputs found
Antiferromagnetic and Orbital Ordering on a Diamond Lattice Near Quantum Criticality
We present neutron scattering measurements on powder samples of the spinel
FeSc2S4 that reveal a previously unobserved magnetic ordering transition
occurring at 11.8(2)~K. Magnetic ordering occurs subsequent to a subtle
cubic-to-tetragonal structural transition which distorts Fe coordinating sulfur
tetrahedra lifting the orbital degeneracy. The application of 1~GPa hydrostatic
pressure appears to destabilize this N\'eel state, reducing the transition
temperature to 8.6(8)~K and redistributing magnetic spectral weight to higher
energies. The relative magnitudes of ordered
and fluctuating moments show that the
magnetically ordered ground state of FeSc2S4 is drastically renormalized and in
proximity to criticality.Comment: 16 pages, 12 figure
Recommended from our members
Quantifying the relationships between linguistic experience, general cognitive skills and linguistic processing skills
Humans differ greatly in their ability to use language. Contemporary psycholinguistic theories assume that individual differences in language skills arise from variability in linguistic experience and in general cognitive skills. While much previous research has tested the involvement of select verbal and non-verbal variables in select domains of linguistic processing, comprehensive characterizations of the relationships among the skills underlying language use are rare. We contribute to such a research program by re-analyzing a publicly available set of data from 112 young adults tested on 35 behavioral tests. The tests assessed nine key constructs reflecting linguistic processing skills, linguistic experience and general cognitive skills. Correlation and hierarchical clustering analyses of the test scores showed that most of the tests assumed to measure the same construct correlated moderately to strongly and largely clustered together. Furthermore, the results suggest important roles of processing speed in comprehension, and of linguistic experience in production
Iron Displacements and Magnetoelastic Coupling in the Spin-Ladder Compound BaFe2Se3
We report long-range ordered antiferromagnetism concomitant with local iron
displacements in the spin-ladder compound BaFeSe. Short-range magnetic
correlations, present at room temperature, develop into long-range
antiferromagnetic order below T = 256 K, with no superconductivity down to
1.8 K. Built of ferromagnetic Fe plaquettes, the magnetic ground state
correlates with local displacements of the Fe atoms. These iron displacements
imply significant magnetoelastic coupling in FeX-based materials, an
ingredient hypothesized to be important in the emergence of superconductivity.
This result also suggests that knowledge of these local displacements is
essential for properly understanding the electronic structure of these systems.
As with the copper oxide superconductors two decades ago, our results highlight
the importance of reduced dimensionality spin ladder compounds in the study of
the coupling of spin, charge, and atom positions in superconducting materials
Explanation for Anomalous Shock Temperatures Measured by Neutron Resonance Spectroscopy
Neutron resonance spectrometry (NRS) has been used to measure the temperature
inside Mo samples during shock loading. The temperatures obtained were
significantly higher than predicted assuming ideal hydrodynamic loading. The
effect of plastic flow and non-ideal projectile behavior were assessed. Plastic
flow was calculated self-consistently with the shock jump conditions: this is
necessary for a rigorous estimate of the locus of shock states accessible.
Plastic flow was estimated to contribute a temperature rise of 53K compared
with hydrodynamic flow. Simulations were performed of the operation of the
explosively-driven projectile system used to induce the shock in the Mo sample.
The simulations predicted that the projectile was significantly curved on
impact, and still accelerating. The resulting spatial variations in load,
including radial components of velocity, were predicted to increase the
apparent temperature that would be deduced from the width of the neutron
resonance by 160K. These corrections are sufficient to reconcile the apparent
temperatures deduced using NRS with the accepted properties of Mo, in
particular its equation of state.Comment: near-final version, waiting for final consent from an autho
Density of Phonon States in Superconducting FeSe as a Function of Temperature and Pressure
The temperature and pressure dependence of the partial density of phonon
states of iron atoms in superconducting Fe1.01Se was studied by 57Fe nuclear
inelastic scattering (NIS). The high energy resolution allows for a detailed
observation of spectral properties. A sharpening of the optical phonon modes
and shift of all spectral features towards higher energies by ~4% with
decreasing temperature from 296 K to 10 K was found. However, no detectable
change at the tetragonal - orthorhombic phase transition around 100 K was
observed. Application of a pressure of 6.7 GPa, connected with an increase of
the superconducting temperature from 8 K to 34 K, results in an increase of the
optical phonon mode energies at 296 K by ~12%, and an even more pronounced
increase for the lowest-lying transversal acoustic mode. Despite these strong
pressure-induced modifications of the phonon-DOS we conclude that the
pronounced increase of Tc in Fe1.01Se with pressure cannot be described in the
framework of classical electron-phonon coupling. This result suggests the
importance of spin fluctuations to the observed superconductivity
Allozyme variation and genetic relationships among species in the Carex willdenowii complex (Cyperaceae)
Peer Reviewedhttps://deepblue.lib.umich.edu/bitstream/2027.42/142149/1/ajb20546.pd
- …