522 research outputs found
Theoretical and computational analysis of second- and third-harmonic generation in periodically patterned graphene and transition-metal dichalcogenide monolayers
Remarkable optical and electrical properties of two-dimensional (2D)
materials, such as graphene and transition-metal dichalcogenide (TMDC)
monolayers, offer vast technological potential for novel and improved
optoelectronic nanodevices, many of which relying on nonlinear optical effects
in these 2D materials. This article introduces a highly effective numerical
method for efficient and accurate description of linear and nonlinear optical
effects in nanostructured 2D materials embedded in periodic photonic structures
containing regular three-dimensional (3D) optical materials, such as
diffraction gratings and periodic metamaterials. The proposed method builds
upon the rigorous coupled-wave analysis and incorporates the nonlinear optical
response of 2D materials by means of modified electromagnetic boundary
conditions. This allows one to reduce the mathematical framework of the
numerical method to an inhomogeneous scattering matrix formalism, which makes
it more accurate and efficient than previously used approaches. An overview of
linear and nonlinear optical properties of graphene and TMDC monolayers is
given and the various features of the corresponding optical spectra are
explored numerically and discussed. To illustrate the versatility of our
numerical method, we use it to investigate the linear and nonlinear
multiresonant optical response of 2D-3D heteromaterials for enhanced and
tunable second- and third-harmonic generation. In particular, by employing a
structured 2D material optically coupled to a patterned slab waveguide, we
study the interplay between geometric resonances associated to guiding modes of
periodically patterned slab waveguides and plasmon or exciton resonances of 2D
materials.Comment: 28 pages, 21 figure
Accurate near-field calculation in the rigorous coupled-wave analysis method
The rigorous coupled-wave analysis (RCWA) is one of the most successful and
widely used methods for modeling periodic optical structures. It yields fast
convergence of the electromagnetic far-field and has been adapted to model
various optical devices and wave configurations. In this article, we
investigate the accuracy with which the electromagnetic near-field can be
calculated by using RCWA and explain the observed slow convergence and
numerical artifacts from which it suffers, namely unphysical oscillations at
material boundaries due to the Gibb's phenomenon. In order to alleviate these
shortcomings, we also introduce a mathematical formulation for accurate
near-field calculation in RCWA, for one- and two-dimensional straight and
slanted diffraction gratings. This accurate near-field computational approach
is tested and evaluated for several representative test-structures and
configurations in order to illustrate the advantages provided by the proposed
modified formulation of the RCWA.Comment: 13 pages, 12 figure
Mapping Itinerant Electrons around Kondo Impurities
We investigate single Fe and Co atoms buried below a Cu(100) surface using
low temperature scanning tunneling spectroscopy. By mapping the local density
of states of the itinerant electrons at the surface, the Kondo resonance near
the Fermi energy is analyzed. Probing bulk impurities in this well-defined
scattering geometry allows separating the physics of the Kondo system and the
measuring process. The line shape of the Kondo signature shows an oscillatory
behavior as a function of depth of the impurity as well as a function of
lateral distance. The oscillation period along the different directions reveals
that the spectral function of the itinerant electrons is anisotropic.Comment: 5 pages, 4 figures, accepted by Physical Review Letter
Long-range Kondo signature of a single magnetic impurity
The Kondo effect, one of the oldest correlation phenomena known in condensed
matter physics, has regained attention due to scanning tunneling spectroscopy
(STS) experiments performed on single magnetic impurities. Despite the
sub-nanometer resolution capability of local probe techniques one of the
fundamental aspects of Kondo physics, its spatial extension, is still subject
to discussion. Up to now all STS studies on single adsorbed atoms have shown
that observable Kondo features rapidly vanish with increasing distance from the
impurity. Here we report on a hitherto unobserved long range Kondo signature
for single magnetic atoms of Fe and Co buried under a Cu(100) surface. We
present a theoretical interpretation of the measured signatures using a
combined approach of band structure and many-body numerical renormalization
group (NRG) calculations. These are in excellent agreement with the rich
spatially and spectroscopically resolved experimental data.Comment: 7 pages, 3 figures + 8 pages supplementary material; Nature Physics
(Jan 2011 - advanced online publication
Cytogerontology since 1881: A reappraisal of August Weismann and a review of modern progress
Cytogerontology, the science of cellular ageing, originated in 1881 with the prediction by August Weismann that the somatic cells of higher animals have limited division potential. Weismann's prediction was derived by considering the role of natural selection in regulating the duration of an organism's life. For various reasons, Weismann's ideas on ageing fell into neglect following his death in 1914, and cytogerontology has only reappeared as a major research area following the demonstration by Hayflick and Moorhead in the early 1960s that diploid human fibroblasts are restricted to a finite number of divisions in vitro.
In this review we give a detailed account of Weismann's theory, and we reveal that his ideas were both more extensive in their scope and more pertinent to current research than is generally recognised. We also appraise the progress which has been made over the past hundred years in investigating the causes of ageing, with particular emphasis being given to (i) the evolution of ageing, and (ii) ageing at the cellular level. We critically assess the current state of knowledge in these areas and recommend a series of points as primary targets for future research
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Come back Marshall, all is forgiven? : Complexity, evolution, mathematics and Marshallian exceptionalism
Marshall was the great synthesiser of neoclassical economics. Yet with his qualified assumption of self-interest, his emphasis on variation in economic evolution and his cautious attitude to the use of mathematics, Marshall differs fundamentally from other leading neoclassical contemporaries. Metaphors inspire more specific analogies and ontological assumptions, and Marshall used the guiding metaphor of Spencerian evolution. But unfortunately, the further development of a Marshallian evolutionary approach was undermined in part by theoretical problems within Spencer's theory. Yet some things can be salvaged from the Marshallian evolutionary vision. They may even be placed in a more viable Darwinian framework.Peer reviewedFinal Accepted Versio
Change and Aging Senescence as an adaptation
Understanding why we age is a long-lived open problem in evolutionary
biology. Aging is prejudicial to the individual and evolutionary forces should
prevent it, but many species show signs of senescence as individuals age. Here,
I will propose a model for aging based on assumptions that are compatible with
evolutionary theory: i) competition is between individuals; ii) there is some
degree of locality, so quite often competition will between parents and their
progeny; iii) optimal conditions are not stationary, mutation helps each
species to keep competitive. When conditions change, a senescent species can
drive immortal competitors to extinction. This counter-intuitive result arises
from the pruning caused by the death of elder individuals. When there is change
and mutation, each generation is slightly better adapted to the new conditions,
but some older individuals survive by random chance. Senescence can eliminate
those from the genetic pool. Even though individual selection forces always win
over group selection ones, it is not exactly the individual that is selected,
but its lineage. While senescence damages the individuals and has an
evolutionary cost, it has a benefit of its own. It allows each lineage to adapt
faster to changing conditions. We age because the world changes.Comment: 19 pages, 4 figure
Learning From Early Attempts to Generalize Darwinian Principles to Social Evolution
Copyright University of Hertfordshire & author.Evolutionary psychology places the human psyche in the context of evolution, and addresses the Darwinian processes involved, particularly at the level of genetic evolution. A logically separate and potentially complementary argument is to consider the application of Darwinian principles not only to genes but also to social entities and processes. This idea of extending Darwinian principles was suggested by Darwin himself. Attempts to do this appeared as early as the 1870s and proliferated until the early twentieth century. But such ideas remained dormant in the social sciences from the 1920s until after the Second World War. Some lessons can be learned from this earlier period, particularly concerning the problem of specifying the social units of selection or replication
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