13,764 research outputs found
GW quasiparticle calculations with spin-orbit coupling for the light actinides
We report on the importance of GW self-energy corrections for the electronic
structure of light actinides in the weak-to-intermediate coupling regime. Our
study is based on calculations of the band structure and total density of
states of Np, U, and Pu using a one-shot GW approximation that includes
spin-orbit coupling within a full potential LAPW framework. We also present RPA
screened effective Coulomb interactions for the f-electron orbitals for
different lattice constants, and show that there is an increased contribution
from electron-electron correlation in these systems for expanded lattices. We
find a significant amount of electronic correlation in these highly localized
electronic systems.Comment: Accepted and to appear in Phys. Rev.
Structural Control of Metamaterial Oscillator Strength and Electric Field Enhancement at Terahertz Frequencies
The design of artificial nonlinear materials requires control over the
internal resonant charge densities and local electric field distributions. We
present a MM design with a structurally controllable oscillator strength and
local electric field enhancement at terahertz frequencies. The MM consists of a
split ring resonator (SRR) array stacked above an array of nonresonant closed
conducting rings. An in-plane, lateral shift of a half unit cell between the
SRR and closed ring arrays results in a decrease of the MM oscillator strength
by a factor of 4 and a 40% change in the amplitude of the resonant electric
field enhancement in the SRR capacitive gap. We use terahertz time-domain
spectroscopy and numerical simulations to confirm our results and we propose a
qualitative inductive coupling model to explain the observed electromagnetic
reponse.Comment: 11 pages, 5 figure
Spin Hall Effect in Atoms
We propose an optical means to realize a spin hall effect (SHE) in neutral
atomic system by coupling the internal spin states of atoms to radiation. The
interaction between the external optical fields and the atoms creates effective
magnetic fields that act in opposite directions on "electrically" neutral atoms
with opposite spin polarizations. This effect leads to a Landau level structure
for each spin orientation in direct analogy with the familiar SHE in
semiconductors. The conservation and topological properties of the spin
current, and the creation of a pure spin current are discussed.Comment: 4 pages, 2 figure; Final versio
Performance of a non-empirical meta-GGA density functional for excitation energies
It is known that the adiabatic approximation in time-dependent density
functional theory usually provides a good description of low-lying excitations
of molecules. In the present work, the capability of the adiabatic nonempirical
meta-generalized gradient approximation (meta-GGA) of Tao, Perdew, Staroverov,
and Scuseria (TPSS) to describe atomic and molecular excitations is tested. The
adiabatic (one-parameter) hybrid version of the TPSS meta-GGA and the adiabatic
GGA of Perdew, Burke, and Ernzerhof (PBE) are also included in the test. The
results are compared to experiments and to two well-established hybrid
functionals PBE0 and B3LYP. Calculations show that both adiabatic TPSS and
TPSSh functionals produce excitation energies in fairly good agreement with
experiments, and improve upon the adiabatic local spin density approximation
and, in particular, the adiabatic PBE GGA. This further confirms that TPSS is
indeed a reliable nonhybrid universal functional which can serve as the
starting point from which higher-level approximations can be constructed. The
systematic underestimate of the low-lying vertical excitation energies of
molecules with time-dependent density functionals within the adiabatic
approximation suggests that further improvement can be made with nonadiabatic
corrections.Comment: 7 page
Decoupling Crossover in Asymmetric Broadside Coupled Split Ring Resonators at Terahertz Frequencies
We investigate the electromagnetic response of asymmetric broadside coupled
split ring resonators (ABC-SRRs) as a function of the relative in-plane
displacement between the two component SRRs. The asymmetry is defined as the
difference in the capacitive gap widths (\Delta g) between the two resonators
comprising a coupled unit. We characterize the response of ABC-SRRs both
numerically and experimentally via terahertz time-domain spectroscopy. As with
symmetric BC-SRRs (\Delta g=0 \mu m), a large redshift in the LC resonance is
observed with increasing displacement, resulting from changes in the capacitive
and inductive coupling. However, for ABC-SRRs, in-plane shifting between the
two resonators by more than 0.375Lo (Lo=SRR sidelength) results in a transition
to a response with two resonant modes, associated with decoupling in the
ABC-SRRs. For increasing \Delta g, the decoupling transition begins at the same
relative shift (0.375Lo), though with an increase in the oscillator strength of
the new mode. This strongly contrasts with symmetric BC-SRRs which present only
one resonance for shifts up to 0.75Lo. Since all BC-SRRs are effectively
asymmetric when placed on a substrate, an understanding of ABC-SRR behavior is
essential for a complete understanding of BC-SRR based metamaterials
Comparison of Power Dependence of Microwave Surface Resistance of Unpatterned and Patterned YBCO Thin Film
The effect of the patterning process on the nonlinearity of the microwave
surface resistance of YBCO thin films is investigated. With the use of a
sapphire dielectric resonator and a stripline resonator, the microwave of
YBCO thin films was measured before and after the patterning process, as a
function of temperature and the rf peak magnetic field in the film. The
microwave loss was also modeled, assuming a dependence of
on current density . Experimental and modeled results
show that the patterning has no observable effect on the microwave residual
or on the power dependence of .Comment: Submitted to IEEE Trans. MT
Continuous quantum phase transition in a Kondo lattice model
We study the magnetic quantum phase transition in an anisotropic Kondo
lattice model. The dynamical competition between the RKKY and Kondo
interactions is treated using an extended dynamic mean field theory (EDMFT)
appropriate for both the antiferromagnetic and paramagnetic phases. A quantum
Monte Carlo approach is used, which is able to reach very low temperatures, of
the order of 1% of the bare Kondo scale. We find that the finite-temperature
magnetic transition, which occurs for sufficiently large RKKY interactions, is
first order. The extrapolated zero-temperature magnetic transition, on the
other hand, is continuous and locally critical.Comment: 4 pages, 4 figures; updated, to appear in PR
Coulomb correlation in presence of spin-orbit coupling: application to plutonium
Attempts to go beyond the local density approximation (LDA) of Density
Functional Theory (DFT) have been increasingly based on the incorporation of
more realistic Coulomb interactions. In their earliest implementations, methods
like LDA+, LDA + DMFT (Dynamical Mean Field Theory), and LDA+Gutzwiller used
a simple model interaction . In this article we generalize the solution of
the full Coulomb matrix involving to parameters, which is
usually presented in terms of an basis, into a basis of
the total angular momentum, where we also include spin-orbit coupling; this
type of theory is needed for a reliable description of -state elements like
plutonium, which we use as an example of our theory. Close attention will be
paid to spin-flip terms, which are important in multiplet theory but that have
been usually neglected in these kinds of studies. We find that, in a
density-density approximation, the basis results provide a very good
approximation to the full Coulomb matrix result, in contrast to the much less
accurate results for the more conventional basis
The Electronic Correlation Strength of Pu
An electronic quantity, the correlation strength, is defined as a necessary
step for understanding the properties and trends in strongly correlated
electronic materials. As a test case, this is applied to the different phases
of elemental Pu. Within the GW approximation we have surprisingly found a
"universal" scaling relationship, where the f-electron bandwidth reduction due
to correlation effects is shown to depend only on the local density
approximation bandwidth and is otherwise independent of crystal structure and
lattice constant.Comment: 7 pages, 4 figures, This version of the paper has been revised to add
additional background informatio
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