Cosmogenic radionuclide production in NaI(Tl) crystals

arXiv:1411.0106v2.-- et al.The production of long-lived radioactive isotopes in materials due to the exposure to cosmic rays on Earth surface can be an hazard for experiments demanding ultra-low background conditions, typically performed deep underground. Production rates of cosmogenic isotopes in all the materials present in the experimental set-up, as well as the corresponding cosmic rays exposure history, must be both well known in order to assess the relevance of this effect in the achievable sensitivity of a given experiment. Although NaI(Tl) scintillators are being used in experiments aiming at the direct detection of dark matter since the first nineties of the last century, very few data about cosmogenic isotopes production rates have been published up to date. In this work we present data from two 12.5 kg NaI(Tl) detectors, developed in the frame of the ANAIS project, which were installed inside a convenient shielding at the Canfranc Underground Laboratory just after finishing surface exposure to cosmic rays. The very fast start of data taking allowed to identify and quantify isotopes with half-lives of the order of tens of days. Initial activities underground have been measured and then production rates at sea level have been estimated following the history of detectors; values of about a few tens of nuclei per kg and day for Te isotopes and 22Na and of a few hundreds for I isotopes have been found. These are the first direct estimates of production rates of cosmogenic nuclides in NaI crystals. A comparison of the so deduced rates with calculations using typical cosmic neutron flux at sea level and a carefully selected description of excitation functions will be also presented together with an estimate of the corresponding contribution to the background at low and high energies, which can be relevant for experiments aiming at rare events searches.This work has been supported by the Spanish Ministerio de Economía y Competitividad and the European Regional Development Fund (MINECO-FEDER) (FPA2011-23749), the Consolider-Ingenio 2010 Programme under grants MULTIDARK CSD2009-00064 and CPAN CSD2007-00042, and the Gobierno de Aragón (Group in Nuclear and Astroparticle Physics, ARAID Foundation and C. Cuesta predoctoral grant). C. Ginestra and P. Villar are supported by the MINECO Subprograma de Formación de Personal Investigador.Peer Reviewe

Exploring the Proximity Effect in Mo/Au Bilayers

We report on the sensitivity of superconducting transition temperature (T c ) to the individual layers' thickness in Mo/Au proximity bilayers to be used in transition-edge sensors (TESs). The achieved good reproducibility and quality of the bilayers allow a clear determination of the superconducting critical temperature T c as a function of the Mo and Au thicknesses. One objective of this work is to analyse the quality of the Mo/Au interface and to assess the possible effects of the double Au layer we use to fabricate these bilayers and TESs based on them. Experimental data are analysed on the basis of Usadel equations using the model developed by Martinis and co-workers, in which the proximity effect in the bilayer is mainly governed by the interface transparency between the superconductor and the normal metal. We find that this model describes quite well the behavior of T c , even for quite thick Au layers, and that the double Au layer does not play any relevant role on the proximity effect

Exploring the Proximity Effect in Mo/Au Bilayers

We report on the sensitivity of superconducting transition temperature (T c ) to the individual layers' thickness in Mo/Au proximity bilayers to be used in transition-edge sensors (TESs). The achieved good reproducibility and quality of the bilayers allow a clear determination of the superconducting critical temperature T c as a function of the Mo and Au thicknesses. One objective of this work is to analyse the quality of the Mo/Au interface and to assess the possible effects of the double Au layer we use to fabricate these bilayers and TESs based on them. Experimental data are analysed on the basis of Usadel equations using the model developed by Martinis and co-workers, in which the proximity effect in the bilayer is mainly governed by the interface transparency between the superconductor and the normal metal. We find that this model describes quite well the behavior of T c , even for quite thick Au layers, and that the double Au layer does not play any relevant role on the proximity effect

Large current-induced broadening of the superconducting transition in Mo/Au transition edge sensors

The R(T, I) shape of the superconducting transition in transition edge sensors (TESs) is of crucial importance to determine their ultimate performance. This paper reports a study of the temperature and current dependences of the transition of Mo/Au TESs, focused on the low resistance region, where these devices preferentially operate. A large broadening of the transition is observed when increasing the applied current. An empirical analytic expression for R(T, I) is found, which describes the transition of devices with different critical temperatures, from R = 0 up to at least 30% R-n (in some cases nearly 80% R-n). Several mechanisms for this behaviour are considered; results show that a current assisted vortex pair unbinding mechanism (Berezinskii-Kosterlitz-Thouless transition) could be the possible origin for this behaviour. Finally, the consequences of the current-induced transition broadening for TES properties and operation are outlined

Background analysis and status of the ANAIS dark matter project

ANAIS (Annual modulation with NaI Scintillators) is a project aiming to set up at the new facilities of the Canfranc Underground Laboratory (LSC), a large scale NaI(Tl) experiment in order to explore the DAMA/LIBRA annual modulation positive result using the same target and technique. Two 12.5 kg each NaI(Tl) crystals provided by Alpha Spectra took data at the LSC in the ANAIS-25 set-up. The comparison of the background model for the ANAIS-25 prototypes with the experimental results is presented. ANAIS crystal radiopurity goals have been achieved for Th-232 and U-238 chains, but a Pb-210 contamination out-of-equilibrium was identified, whose origin has been studied. The high light collection efficiency obtained with these prototypes allows to anticipate an energy threshold of the order of 1 keVee. A new detector, with improved performances, was received in March 2015 and very preliminary results are shown.Comment: 6 pages, 7 figure

Status of the ANAIS Dark Matter Project at the Canfranc Underground Laboratory

The ANAIS experiment aims at the confirmation of the DAMA/LIBRA signal. A detailed analysis of two NaI(Tl) crystals of 12.5 kg each grown by Alpha Spectra will be shown: effective threshold at 1 keVee is at reach thanks to outstanding light collection and robust PMT noise filtering protocols and the measured background is well understood down to 3 keVee, having quantified K, U and Th content and cosmogenic activation in the crystals. A new detector was installed in Canfranc in March 2015 together with the two previous modules and preliminary characterization results will be presented. Finally, the status and expected sensitivity of the full experiment with 112 kg will be reviewed.Comment: Contributed to the 11th Patras Workshop on Axions, WIMPs and WISPs, Zaragoza, June 22 to 26, 201

Production and relevance of cosmogenic radionuclides in NaI(Tl) crystals

The cosmogenic production of long-lived radioactive isotopes in materials is an hazard for experiments demanding ultra-low background conditions. Although NaI(Tl) scintillators have been used in this context for a long time, very few activation data were available. We present results from two 12.5 kg NaI(Tl) detectors, developed within the ANAIS project and installed at the Canfranc Underground Laboratory. The prompt data taking starting made possible a reliable quantification of production of some I, Te and Na isotopes with half-lives larger than ten days. Initial activities underground were measured and then production rates at sea level were estimated following the history of detectors; a comparison of these rates with calculations using typical cosmic neutron flux at sea level and a selected description of excitation functions was also carried out. After including the contribution from the identified cosmogenic products in the detector background model, we found that the presence of 3H in the crystal bulk would help to fit much better our background model and experimental data. We have analyzed the cosmogenic production of 3H in NaI, and although precise quantification has not been attempted, we can conclude that it could imply a very relevant contribution to the total background below 15 keV in NaI detectors.Comment: Proceedings of the Low Radioactivity Techniques 2015 workshop, March 2015, Seattle (US

Preliminary results of ANAIS-25

The ANAIS (Annual Modulation with NaI(Tl) Scintillators) experiment aims at the confirmation of the DAMA/LIBRA signal using the same target and technique at the Canfranc Underground Laboratory. 250 kg of ultrapure NaI(Tl) crystals will be used as a target, divided into 20 modules, each coupled to two photomultipliers. Two NaI(Tl) crystals of 12.5 kg each, grown by Alpha Spectra from a powder having a potassium level under the limit of our analytical techniques, form the ANAIS-25 set-up. The background contributions are being carefully studied and preliminary results are presented: their natural potassium content in the bulk has been quantified, as well as the uranium and thorium radioactive chains presence in the bulk through the discrimination of the corresponding alpha events by PSA, and due to the fast commissioning, the contribution from cosmogenic activated isotopes is clearly identified and their decay observed along the first months of data taking. Following the procedures established with ANAIS-0 and previous prototypes, bulk NaI(Tl) scintillation events selection and light collection efficiency have been also studied in ANAIS-25.Comment: 4 pages, 6 Figure