401 research outputs found
High-spin structures as the probes of proton-neutron pairing
Rotating nuclei in the mass region have been studied within
the framework of isovector mean field theory. Available data is well and
systematically described in the calculations. The present study supports the
presence of strong isovector pair field at low spin, which is, however,
destroyed at high spin. No clear evidence for the existence of the isoscalar
pairing has been found.Comment: Invited talk presented at the XIII Nuclear Physics Workshop,
Kazimierz Dolny, Sept. 27 - Oct. 1, Poland; submitted to International
Journal of Modern Physics
Cyclotron production and cyclometallation chemistry of 192Ir
Introduction
To explore new questions and techniques in nuclear medicine, new isotopes with novel chemical and nuclear properties must be developed. We are interested in the small cyclotron production of new radiometals for the development of new radiopharmaceuticals (RX). In an example of RX multifunctionality, Luminescence Cell Imaging (LCI) has been combined with radio-isotopes to allow compounds that can be imaged with both optical microscopy and nuclear techniques [1]. Within this field, iridium cy-clometalates have good potential with excellent photophysical properties [2]. As well, low specific activity iridium-192 has found use in brachy-therapy as a high-intensity beta emitter [3]. Despite this, iridium radioisotopes have yet to be applied to cyclometalation chemistry, or a radiochemical isolation method developed for carrier free production on a medical cyclotron. Our goal is to demonstrate the feasibility of the production and isolation of radio-iridium, and its application to cyclometalate chemistry as a potentially interesting tool for nuclear medicine research.
Materials and Methods
Following literature precedent [4], natural osmium was electroplated onto a silver disc from basic media containing osmium tetroxide and sulphamic acid. The thin deposits obtained (15–20 mg cm−2) were weighed and characterized with scanning electron microscopy.
Targets were irradiated using the TRIUMF TR13 cyclotron, delivering 12.5 MeV protons to the target disc. Initial bombardments were per-formed at 5 μA; gamma spectra of the targets were collected 24 hours after end of bombardment.
The irradiated material was oxidized, dissolved from the target backing, and separated via anion exchange.
In parallel to the isotope production work, non-radioactive iridium was used to define a chemical procedure suitable for the synthesis of model iridium cyclometalate compounds given low concentrations of radioiridium. These experiments will be performed with radioactive iridium in the next step of the research project.
Results and Conclusion
Proton bombardment of natural osmium yielded a range of iridium isotopes, with characteristic spectral lines corresponding to 186-190Ir, and 192Ir; no other characteristic radiation was observed. The EOB activity of each isotope was then used in thin target calculations to approximate their (p,n) cross section. Preliminary cross section measurements of the 192Os(p,n)192Ir reaction (53 ± 13 mb @ 12.5 MeV) confirm published data (52.3 ± 5.7 mb @ 12.2 MeV) [6], and provide as-yet unpublished data on the lower mass number isotopes.
The progress of radioactive iridium through the radiochemical separation was tracked with a dose calibrator; the osmium complex formed was brightly coloured and could be seen retained on the column. The overall efficiency of the process is estimated at 80 %. Radioactive cyclometallation chemistry is currently under-way.
The production and isolation of a range of iridium isotopes in a chemically useful form was demonstrated, and is ready to be applied to a cyclometalate model compound. Future work will investigate the production of 192Ir from enriched 192Os
Highly charged ions in Penning traps, a new tool for resolving low lying isomeric states
The use of highly charged ions increases the precision and resolving power,
in particular for short-lived species produced at on-line radio-isotope beam
facilities, achievable with Penning trap mass spectrometers. This increase in
resolving power provides a new and unique access to resolving low-lying
long-lived ( ms) nuclear isomers. Recently, the keV
(determined from -ray spectroscopy) isomeric state in Rb has
been resolved from the ground state, in a charge state of with the TITAN
Penning trap at the TRIUMF-ISAC facility. The excitation energy of the isomer
was measured to be keV above the ground state. The extracted
masses for both the ground and isomeric states, and their difference, agree
with the AME2003 and Nuclear Data Sheet values. This proof of principle
measurement demonstrates the feasibility of using Penning trap mass
spectrometers coupled to charge breeders to study nuclear isomers and opens a
new route for isomer searches.Comment: 8 pages, 6 figure
Extinction of the N=20 neutron-shell closure for 32Mg examined by direct mass measurements
The 'island of inversion' around Mg is one of the most important
paradigm for studying the disappearance of the stabilizing 'magic' of a shell
closure. We present the first Penning-trap mass measurements of the exotic
nuclides Na and Mg, which allow a precise determination of
the empirical shell gap for Mg. The new value of 1.10(3) MeV is the
lowest observed shell gap for any nuclide with a canonical magic number.Comment: 6 pages, 4 figures, submitted to Physical Review
Trapped-ion decay spectroscopy towards the determination of ground-state components of double-beta decay matrix elements
A new technique has been developed at TRIUMF's TITAN facility to perform
in-trap decay spectroscopy. The aim of this technique is to eventually measure
weak electron capture branching ratios (ECBRs) and by this to consequently
determine GT matrix elements of decaying nuclei. These branching
ratios provide important input to the theoretical description of these decays.
The feasibility and power of the technique is demonstrated by measuring the
ECBR of Cs.Comment: 9 pages, 9 figure
Low-Background In-Trap Decay Spectroscopy with TITAN at TRIUMF
An in-trap decay spectroscopy setup has been developed and constructed for
use with the TITAN facility at TRIUMF. The goal of this device is to observe
weak electron-capture (EC) branching ratios for the odd-odd intermediate nuclei
in the decay process. This apparatus consists of an up-to 6 Tesla,
open-access spectroscopy ion-trap, surrounded radially by up to 7 planar Si(Li)
detectors which are separated from the trap by thin Be windows. This
configuration provides a significant increase in sensitivity for the detection
of low-energy photons by providing backing-free ion storage and eliminating
charged-particle-induced backgrounds. An intense electron beam is also employed
to increase the charge-states of the trapped ions, thus providing storage times
on the order of minutes, allowing for decay-spectroscopy measurements. The
technique of multiple ion-bunch stacking was also recently demonstrated, which
further extends the measurement possibilities of this apparatus. The current
status of the facility and initial results from a In measurement are
presented.Comment: Proceedings for the 2nd International Conference on Advances in
Radioactive Isotope Science (ARIS2014
Z=50 shell gap near Sn from intermediate-energy Coulomb excitations in even-mass Sn isotopes
Rare isotope beams of neutron-deficient Sn nuclei from the
fragmentation of Xe were employed in an intermediate-energy Coulomb
excitation experiment yielding transition strengths.
The results indicate that these values are much larger
than predicted by current state-of-the-art shell model calculations. This
discrepancy can be explained if protons from within the Z = 50 shell are
contributing to the structure of low-energy excited states in this region. Such
contributions imply a breaking of the doubly-magic Sn core in the light
Sn isotopes.Comment: 4 pages, 4 figure
Far From \u27Easy\u27 Spectroscopy with the 8Ï€ and GRIFFIN Spectrometers at TRIUMF-ISAC
The 8π spectrometer, installed at the TRIUMF-ISAC facility, was the world\u27s most sensitive γ-ray spectrometer dedicated to β-decay studies. A description is given of the 8π spectrometer and its auxiliary detectors including the plastic scintillator array SCEPTAR used for β-particle tagging and the Si(Li) array PACES for conversion electron measurements, its moving tape collector, and its data acquisition system. The recent investigation of the decay of 124Cs to study the nuclear structure of 124Xe, and how the β-decay measurements complemented previous Coulomb excitation studies, is highlighted, including the extraction of the deformation parameters for the excited 0+ bands in 124Xe. As a by-product, the decay scheme of the (7+) 124Cs isomeric state, for which the data from the PACES detectors were vital, was studied. Finally, a description of the new GRIFFIN spectrometer, which uses the same auxiliary detectors as the 8π spectrometer, is given
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