2,917 research outputs found
Orbital excitations in LaMnO
We study the recently observed orbital excitations, orbitons, and treat
electron-electron correlations and lattice dynamics on equal footing. It is
shown that the orbiton energy and dispersion are determined by both
correlations and lattice-vibrations. The electron-phonon coupling causes
satellite structures in the orbiton spectral function and the elementary
excitations of the system are mixed modes with both orbital and phonon
character. It is proposed that the satellite structures observed in recent
Raman-scattering experiments on LaMnO are actually orbiton derived
satellites in the phonon spectral function, caused by the phonon-orbiton
interaction.Comment: 4 pages, 3 figures embedde
Orbital order-disorder transition in La(1-x)Nd(x)MnO(3) (x = 0.0-1.0) and La(1-x-y)Nd(yx)Sr(y)MnO(3) (x = 0.1; y = 0.05,0.1)
The nature of orbital order-disorder transition has been studied in the
La(1-x)Nd(x)MnO(3) (x = 0.0-1.0) series which covers the entire range between
two end points - LaMnO(3) and NdMnO(3) - as well as in
La(0.85)Nd(0.1)Sr(0.05)MnO(3) and La(0.8)Nd(0.1)Sr(0.1)MnO(3). It has been
observed that the first-order nature of the transition gives way to higher
order with the increase in "x" in the case of pure manganites. The latent heat
(L) associated with the transition, first, drops with a steeper slope within x
= 0.0-0.3 and, then, gradually over a range 0.3<x<0.9. This drop could,
possibly, be due to evolution of finer orbital domain structure with "x". In
the case of Sr-doped samples, the transition appears to be of higher-order
nature even for a doping level 5 at%. In both cases, of course, the transition
temperature T(JT) rises systematically with the drop in average A-site radius
or rise in average Mn-O-Mn bond bending angle while no
apparent correlation could be observed with doping induced disorder sigma^2.
The cooperative nature of the orbital order, therefore, appears to be robust.Comment: 15 pages including 4 figures; pdf onl
Interface-induced d-wave pairing
We discuss a scenario for interface-induced superconductivity involving
pairing by dipolar excitations proximate to a two-dimensional electron system
controlled by a transverse electric field. If the interface consists of
transition metal oxide materials, the repulsive on-site Coulomb interaction is
typically strong and a superconducting state is formed via exchange of
non-local dipolar excitations in the d-wave channel. Perspectives to enhance
the superconducting transition temperature are discussed.Comment: 4 pages, 3 figure
The quantum origins of skyrmions and half-skyrmions in Cu2OSeO3
The Skyrme-particle, the , was introduced over half a century ago
and used to construct field theories for dense nuclear matter. But with
skyrmions being mathematical objects - special types of topological solitons -
they can emerge in much broader contexts. Recently skyrmions were observed in
helimagnets, forming nanoscale spin-textures that hold promise as information
carriers. Extending over length-scales much larger than the inter-atomic
spacing, these skyrmions behave as large, classical objects, yet deep inside
they are of quantum origin. Penetrating into their microscopic roots requires a
multi-scale approach, spanning the full quantum to classical domain. By
exploiting a natural separation of exchange energy scales, we achieve this for
the first time in the skyrmionic Mott insulator CuOSeO. Atomistic ab
initio calculations reveal that its magnetic building blocks are strongly
fluctuating Cu tetrahedra. These spawn a continuum theory with a skyrmionic
texture that agrees well with reported experiments. It also brings to light a
decay of skyrmions into half-skyrmions in a specific temperature and magnetic
field range. The theoretical multiscale approach explains the strong
renormalization of the local moments and predicts further fingerprints of the
quantum origin of magnetic skyrmions that can be observed in CuOSeO,
like weakly dispersive high-energy excitations associated with the Cu
tetrahedra, a weak antiferromagnetic modulation of the primary ferrimagnetic
order, and a fractionalized skyrmion phase.Comment: 5 pages, 3 figure
Strong-field approximation for Coulomb explosion of H_2^+ by short intense laser pulses
We present a simple quantum mechanical model to describe Coulomb explosion of
H by short, intense, infrared laser pulses. The model is based on the
length gauge version of the molecular strong-field approximation and is valid
for pulses shorter than 50 fs where the process of dissociation prior to
ionization is negligible. The results are compared with recent experimental
results for the proton energy spectrum [I. Ben-Itzhak et al., Phys. Rev. Lett.
95, 073002 (2005), B. D. Esry et al., Phys. Rev. Lett. 97, 013003 (2006)]. The
predictions of the model reproduce the profile of the spectrum although the
peak energy is slightly lower than the observations. For comparison, we also
present results obtained by two different tunneling models for this process.Comment: 8 pages, 4 figure
Establishing the fundamental magnetic interactions in the chiral skyrmionic Mott insulator Cu2OSeO3 by terahertz electron spin resonance
The recent discovery of skyrmions in CuOSeO has established a new
platform to create and manipulate skyrmionic spin textures. We use high-field
electron spin resonance (ESR) spectroscopy combining a terahertz free electron
laser and pulsed magnetic fields up to 64 T to probe and quantify its
microscopic spin-spin interactions. Besides providing direct access to the
long-wavelength Goldstone mode, this technique probes also the high-energy part
of the excitation spectrum which is inaccessible by standard low-frequency ESR.
Fitting the behavior of the observed modes in magnetic field to a theoretical
framework establishes experimentally that the fundamental magnetic building
blocks of this skyrmionic magnet are rigid, highly entangled and weakly coupled
tetrahedra.Comment: 5 pages, 3 Figure
Reentrant metallic transition at a temperature above Tc at the breakdown of cooperative Jahn-Teller orbital order in perovskite manganites
We report an interesting reentrant metallic resistivity pattern beyond a
characteristic temperature T* which is higher than other such characteristic
transition temperatures like T(c)(Curie point), T(N) (Neel point), T(CO)
(charge order onset point) or T(OO) (orbital order onset point) in a range of
rare-erath perovskite manganites (RE(1-x)A(x)MnO(3); RE = La, Nd, Y; A = Sr,
Ca; x = 0.0-0.5). Such a behavior is normally observed in doped manganites with
doping level (x) higher than the critical doping level x(c) (= 0.17-0.22)
required for the metallic ground state to emerge and hence in a system where
cooperative Jahn-Teller orbital order has already undergone a breakdown.
However, the observation made in the La(1-x)Ca(x)MnO(3) (x = 0.0-0.5) series
turns out to be an exception to this general trend.Comment: 15 pages including 3 figures; pdf onl
Kitaev interactions between j=1/2 moments in honeycomb Na2IrO3 are large and ferromagnetic: insights from ab initio quantum chemistry calculations
NaIrO, a honeycomb 5 oxide, has been recently identified as a
potential realization of the Kitaev spin lattice. The basic feature of this
spin model is that for each of the three metal-metal links emerging out of a
metal site, the Kitaev interaction connects only spin components perpendicular
to the plaquette defined by the magnetic ions and two bridging ligands. The
fact that reciprocally orthogonal spin components are coupled along the three
different links leads to strong frustration effects and nontrivial physics.
While the experiments indicate zigzag antiferromagnetic order in NaIrO,
the signs and relative strengths of the Kitaev and Heisenberg interactions are
still under debate. Herein we report results of ab initio many-body electronic
structure calculations and establish that the nearest-neighbor exchange is
strongly anisotropic with a dominant ferromagnetic Kitaev part, whereas the
Heisenberg contribution is significantly weaker and antiferromagnetic. The
calculations further reveal a strong sensitivity to tiny structural details
such as the bond angles. In addition to the large spin-orbit interactions, this
strong dependence on distortions of the IrO plaquettes singles out the
honeycomb 5 oxides as a new playground for the realization of
unconventional magnetic ground states and excitations in extended systems.Comment: 13 pages, 2 tables, 3 figures, accepted in NJ
Rodrigues Formula for Hi-Jack Symmetric Polynomials Associated with the Quantum Calogero Model
The Hi-Jack symmetric polynomials, which are associated with the simultaneous
eigenstates for the first and second conserved operators of the quantum
Calogero model, are studied. Using the algebraic properties of the Dunkl
operators for the model, we derive the Rodrigues formula for the Hi-Jack
symmetric polynomials. Some properties of the Hi-Jack polynomials and the
relationships with the Jack symmetric polynomials and with the basis given by
the QISM approach are presented. The Hi-Jack symmetric polynomials are strong
candidates for the orthogonal basis of the quantum Calogero model.Comment: 17 pages, LaTeX file using jpsj.sty (ver. 0.8), cite.sty,
subeqna.sty, subeqn.sty, jpsjbs1.sty and jpsjbs2.sty (all included.) You can
get all the macros from ftp.u-tokyo.ac.jp/pub/SOCIETY/JPSJ
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