88 research outputs found

    Magnetism in La2O3(Fe1-xMnx)2Se2 tuned by Fe/Mn ratio

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    We report the evolution of structural and magnetic properties in La2O3(Fe1-xMnx)2Se2. Heat capacity and bulk magnetization indicate an increased ferromagnetic component of the long-range magnetic order and possible increased degree of frustration. Atomic disorder on Fe(Mn) sites suppresses the temperature of the long-range order whereas intermediate alloys show a rich magnetic phase diagram.Comment: 7 pages, 7 figure

    Mixed-state twin observables

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    Twin observables, i.e. opposite subsystem observables A+ and A- that are indistinguishable in measurement in a given mixed or pure state W, are investigated in detail algebraicly and geometrically. It is shown that there is a far-reaching correspondence between the detectable (in W) spectral entities of the two operators. Twin observables are state-dependently quantum-logically equivalent, and direct subsystem measurement of one of them ipso facto gives rise to the indirect (i.e. distant) measurement of the other. Existence of nontrivial twins requires singularity of W. Systems in thermodynamic equilibrium do not admit subsystem twins. These observables may enable one to simplify the matrix representing W.Comment: 13 page

    Smoothness of de nite unitary eigenvarieties at critical points

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    We compute an upper bound for the dimension of the tangent spaces at classical points of certain eigenvarieties associated with definite unitary groups, especially including the so-called critically refined cases. Our bound is given in terms of “critical types” and when our bound is minimized it matches the dimension of the eigenvariety. In those cases, which we explicitly determine, the eigenvariety is necessarily smooth and our proof also shows that the completed local ring on the eigenvariety is naturally a certain universal Galois deformation ring

    Vacancy-Driven Noncubic Local Structure and Magnetic Anisotropy Tailoring in FeₓO-Fe₃-{δ}_O₄ Nanocrystals

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    In contrast to bulk materials, nanoscale crystal growth is critically influenced by size- and shape-dependent properties. However, it is challenging to decipher how stoichiometry, in the realm of mixed-valence elements, can act to control physical properties, especially when complex bonding is implicated by short- and long-range ordering of structural defects. Here, solution-grown iron-oxide nanocrystals (NCs) of the pilot wüstite system are found to convert into iron-deficient rock-salt and ferro-spinel subdomains but attain a surprising tetragonally distorted local structure. Cationic vacancies within chemically uniform NCs are portrayed as the parameter to tweak the underlying properties. These lattice imperfections are shown to produce local exchange-anisotropy fields that reinforce the nanoparticles’ magnetization and overcome the influence of finite-size effects. The concept of atomic-scale defect control in subcritical-size NCs aspires to become a pathway to tailor-made properties with improved performance for hyperthermia heating over defect-free NCs

    Theory of the Diamagnetism Above the Critical Temperature for Cuprates

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    Recently experiments on high critical temperature superconductors has shown that the doping levels and the superconducting gap are usually not uniform properties but strongly dependent on their positions inside a given sample. Local superconducting regions develop at the pseudogap temperature (TT^*) and upon cooling, grow continuously. As one of the consequences a large diamagnetic signal above the critical temperature (TcT_c) has been measured by different groups. Here we apply a critical-state model for the magnetic response to the local superconducting domains between TT^* and TcT_c and show that the resulting diamagnetic signal is in agreement with the experimental results.Comment: published versio

    Polaron and bipolaron formation in the Hubbard-Holstein model: role of next-nearest neighbor electron hopping

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    The influence of next-nearest neighbor electron hopping, tt^{\prime}, on the polaron and bipolaron formation in a square Hubbard-Holstein model is investigated within a variational approach. The results for electron-phonon and electron-electron correlation functions show that a negative value of tt^{\prime} induces a strong anisotropy in the lattice distortions favoring the formation of nearest neighbor intersite bipolaron. The role of tt^{\prime}, electron-phonon and electron-electron interactions is briefly discussed in view of the formation of charged striped domains.Comment: 4 figure

    Pressure Studies on a High-TcT_c Superconductor Pseudogap and Critical Temperatures

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    We report simultaneous hydrostatic pressure studies on the critical temperature TcT_c and on the pseudogap temperature TT^* performed through resistivity measurements on an optimally doped high-TcT_c oxide Hg0.82Re0.18Ba2Ca2Cu3O8+δHg_{0.82}Re_{0.18}Ba_2Ca_2Cu_3O_{8+\delta}. The resistivity is measured as function of the temperature for several different applied pressure below 1GPa. We find that both TcT_c and TT^* increases linearly with the pressure. This result demonstrate that the well known intrinsic pressure effect on TcT_c is also present at TT^* and both temperatures are originated by the same superconducting mechanism.Comment: 4 pages and 2 figures in eps, final versio
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