26 research outputs found

    The effect of the Abrikosov vortex phase on spin and charge states in magnetic semiconductor-superconductor hybrids

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    We explore the possibility of using the inhomogeneous magnetic field carried by an Abrikosov vortex in a type-II superconductor to localize spin-polarized textures in a nearby magnetic semiconductor quantum well. We show how Zeeman-induced localization induced by a single vortex is indeed possible, and use these results to investigate the effect of a periodic vortex array on the transport properties of the magnetic semiconductor. In particular, we find an unconventional Integer Quantum Hall regime, and predict directly testable experimental consequences due to the presence of the periodic spin polarized structure induced by the superconducting vortex lattice in the magnetic semiconductor.Comment: 12 pages, 15 figure

    Nanoscale Zeeman localization of charge carriers in diluted magnetic semiconductor-permalloy hybrids

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    We investigate the possibility of charge carrier localization in magnetic semiconductors due to the presence of a highly inhomogeneous external magnetic field. As an example, we study in detail the properties of a magnetic semiconductor-permalloy disk hybrid system. We find that the giant Zeeman respose of the magnetic semiconductor in conjuction with the highly non-uniform magnetic field created by the vortex state of a permalloy disk can lead to Zeeman localized states at the interface of the two materials. These trapped state are chiral, with chirality controlled by the orientation of the core magnetization of the permalloy disk. We calculate the energy spectrum and the eigenstates of these Zeeman localized states, and discuss their experimental signatures in spectroscopic probes.Comment: 4 pages, 1 figur

    Binding energy of shallow donors in a quantum well in the presence of a tilted magnetic field

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    We present results of variational calculations of the binding energy of a neutral donor in a quantum well in the presence of a magnetic field tilted relative to the QW plane. Assuming that the donor is located in the center of the QW, we perform calculations for parameters typical of a II-VI wide-gap semiconductor heterostructure, using as an example the case of a rectangular CdTe quantum well with CdMgTe barriers. We present the dependence of the binding energy of a neutral donor on the tilt angle and on the magnitude of the applied magnetic filed. As a key result, we show that measurement of the binding energy of a donor at two angles of the magnetic field with respect to the quantum well plane can be used to unambiguously determined the conduction band offset of the materials building up heterostructure.Comment: 6 pages, 5 figure

    Enhanced robustness and dimensional crossover of superradiance in cuboidal nanocrystal superlattices

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    Cooperative emission of coherent radiation from multiple emitters (known as superradiance) has been predicted and observed in various physical systems, most recently in CsPbBr3_3 nanocrystal superlattices. Superradiant emission is coherent and occurs on timescales faster than the emission from isolated nanocrystals. Theory predicts cooperative emission being faster by a factor of up to the number of nanocrystals (NN). However, superradiance is strongly suppressed due to the presence of energetic disorder, stemming from nanocrystal size variations and thermal decoherence. Here, we analyze superradiance from superlattices of different dimensionalities (1D, 2D and 3D) with variable nanocrystal aspect ratios. We predict as much as a thirty-fold enhancement in robustness against realistic values of energetic disorder in three-dimensional (3D) superlattices composed of cuboid-shaped, as opposed to cube-shaped, nanocrystals. Superradiance from small (N103)(N\lesssim 10^3) two-dimensional (2D) superlattices is up to 10 times more robust to static disorder and up to twice as robust to thermal decoherence than three-dimensional (3D) superlattices with the same NN. As the number of NN increases, a crossover in the robustness of superradiance occurs from 2D to 3D superlattices. For large N (>103)N\ (> 10^3), the robustness in 3D superlattices increases with NN, showing cooperative robustness to disorder. This opens the possibility of observing superradiance even at room temperature in large 3D superlattices, if nanocrystal size fluctuations can be kept small

    Heterogeneous Fluorescence Intermittency in Single Layer Reduced Graphene Oxide

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    We provide, for the first time, direct experimental evidence for heterogeneous blinking in reduced graphene oxide (rGO) during photolysis. The spatially resolved intermittency originates from regions within individual rGO sheets and shows 1/f-like power spectral density. We describe the evolution of rGO blinking using the multiple recombination center (MRC) model that captures common features of nanoscale blinking. Our results illustrate the universal nature of blinking and suggest a common microscopic origin for the effect

    Origin of the pseudogap phase: Precursor superconductivity versus a competing energy gap scenario

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    In the last few years evidence has been accumulating that there are a multiplicity of energy scales which characterize superconductivity in the underdoped cuprates. In contrast to the situation in BCS superconductors, the phase coherence temperature Tc is different from the energy gap onset temperature T*. In addition, thermodynamic and tunneling spectroscopies have led to the inference that the order parameter Δsc\Delta_{sc} is to be distinguished from the excitation gap Δ\Delta; in this way, pseudogap effects persist below Tc. It has been argued by many in the community that the presence of these distinct energy scales demonstrates that the pseudogap is unrelated to superconductivity. In this paper we show that this inference is incorrect. We demonstrate that the difference between the order parameter and excitation gap and the contrasting dependences of T* and Tc on hole concentration xx and magnetic field HH follow from a natural generalization of BCS theory. This simple generalized form is based on a BCS-like ground state, but with self consistently determined chemical potential in the presence of arbitrary attractive coupling gg. We have applied this mean field theory with some success to tunneling, transport, thermodynamics and magnetic field effects. We contrast the present approach with the phase fluctuation scenario and discuss key features which might distinguish our precursor superconductivity picture from that involving a competing order parameter.Comment: 4 pages, 2 EPS figures, use LaTeX package espcrc2.sty from Elsevier, submitted to SNS'01 conference proceeding

    The electronic specific heat in the pairing pseudogap regime

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    When pairing correlations in a quasi two dimensional electron system induce a pseudogap in the single particle density of states, the specific heat must also contain a sizeable pair contribution. The theoretically calculated specific heat for such a system is compared to the experimental results of Loram and his collaborators for underdoped YBa_2Cu_3O_{6+x} and La_{2-x}Sr_{x}CuO_4 samples. The size and doping dependence of the extracted pseudogap energy scale for both materials is comparable to the values obtained from a variety of other experiments.Comment: 4 pages, 5 eps figure

    Resonant multiple-phonon absorption causes efficient anti-Stokes photoluminescence in CsPbBr3_3 nanocrystals

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    Lead-halide perovskite nanocrystals such as CsPbBr3_3, exhibit efficient photoluminescence (PL) up-conversion, also referred to as anti-Stokes photoluminescence (ASPL). This is a phenomenon where irradiating nanocrystals up to 100 meV below gap results in higher energy band edge emission. Most surprising is that ASPL efficiencies approach unity and involve single photon interactions with multiple phonons. This is unexpected given the statistically disfavored nature of multiple-phonon absorption. Here, we report and rationalize near-unity anti-Stokes photoluminescence efficiencies in CsPbBr3_3 nanocrystals and attribute it to resonant multiple-phonon absorption by polarons. The theory explains paradoxically large efficiencies for intrinsically disfavored, multiple-phonon-assisted ASPL in nanocrystals. Moreover, the developed microscopic mechanism has immediate and important implications for applications of ASPL towards condensed phase optical refrigeration
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