Low Loss and Magnetic Field-tuned Superconducting THz Metamaterial

Superconducting terahertz (THz) metamaterial (MM) made from superconducting Nb film has been investigated using a continuous-wave THz spectroscopy with a superconducting split-coil magnet. The obtained quality factors of the resonant modes at 132 GHz and 450 GHz are about three times as large as those calculated for a metal THz MM operating at 1 K, which indicates that superconducting THz MM is a very nice candidate to achieve low loss performance. In addition, the magnetic field-tuning on superconducting THz MM is also demonstrated, which offer an alternative tuning method apart from the existed electric, optical and thermal tuning on THz MM

Antiferromagnetic magnonic charge current generation via ultrafast optical excitation

N\'eel spin-orbit torque allows a charge current pulse to efficiently manipulate the N\'eel vector in antiferromagnets, which offers a unique opportunity for ultrahigh density information storage with high speed. However, the reciprocal process of N\'eel spin-orbit torque, the generation of ultrafast charge current in antiferromagnets has not been demonstrated. Here, we report the experimental observation of charge current generation in antiferromagnetic metallic Mn2Au thin films using ultrafast optical excitation. The ultrafast laser pulse excites antiferromagnetic magnons, resulting in instantaneous non-equilibrium spin polarization at the antiferromagnetic spin sublattices with broken spatial symmetry. Then the charge current is generated directly via spin-orbit fields at the two sublattices, which is termed as the reciprocal phenomenon of N\'eel spin-orbit torque, and the associated THz emission can be detected at room temperature. Besides the fundamental significance on the Onsager reciprocity, the observed magnonic charge current generation in antiferromagnet would advance the development of antiferromagnetic THz emitter.Comment: 15 pages, 4 figures, this work was submitted to Nature Communications on Jan. 4th, 2023, now is under the 3rd review proces

Terahertz Spin Current Dynamics in Antiferromagnetic Hematite

An important vision of modern magnetic research is to use antiferromagnets (AFMs) as controllable and active ultrafast components in spintronic devices. Hematite (α-Fe2O3) is a promising model material in this respect because its pronounced Dzyaloshinskii-Moriya interaction leads to the coexistence of antiferromagnetism and weak ferromagnetism. Here, femtosecond laser pulses are used to drive terahertz (THz) spin currents from α-Fe2O3 into an adjacent Pt layer. Two contributions to the generation of the spin current with distinctly different dynamics are found: the impulsive stimulated Raman scatting that relies on the AFM order and the ultrafast spin Seebeck effect that relies on the net magnetization. The total THz spin current dynamics can be manipulated by a medium-strength magnetic field below 1 T. The control of the THz spin current achieved in α-Fe2O3 opens the pathway toward tailoring the exact spin current dynamics from ultrafast AFM spin sources

Defect-induced helicity-dependent terahertz emission in Dirac semimetal PtTe2 thin films

Nonlinear transport enabled by symmetry breaking in quantum materials has aroused considerable interest in condensed matter physics and interdisciplinary electronics. However, the nonlinear optical response in centrosymmetric Dirac semimetals via the defect engineering has remained highly challenging. Here, we observe the helicity-dependent terahertz (THz) emission in Dirac semimetal PtTe2 thin films via circular photogalvanic effect (CPGE) under normal incidence. This is activated by artificially controllable out-of-plane Te-vacancy defect gradient, which is unambiguously evidenced by the electron ptychography. The defect gradient lowers the symmetry, which not only induces the band spin splitting, but also generates the giant Berry curvature dipole (BCD) responsible for the CPGE. Such BCD-induced helicity-dependent THz emission can be manipulated by the Te-vacancy defect concentration. Furthermore, temperature evolution of the THz emission features the minimum of the THz amplitude due to the carrier compensation. Our work provides a universal strategy for symmetry breaking in centrosymmetric Dirac materials for efficient nonlinear transport and facilitates the promising device applications in integrated optoelectronics and spintronics.Comment: 27 pages, 5 figure

Frequency-selective terahertz wave amplification by a time-boundary-engineered Huygens metasurface

Ultrafast manipulation of optical resonance can establish the time-boundary effect in time-variant media leading to a new degree of freedom for coherent control of electromagnetic waves. Here, we demonstrate that a free-standing all dielectric Huygens metasurface of degenerate electric and magnetic resonances can prompt the broadband near-unity transmission in its static state, whereas it enables wave amplification in the presence of time boundary. The time boundary is realized by femtosecond laser excitations that transiently inject free carriers into the constituent meta-atoms for dynamic removal of a pre-established two-fold degeneracy. We observe that the transmittance in the photo-excited Huygens metasurface can exceed unity transmittance, i.e., THz wave amplification, by a factor over 20% in intensity at frequencies tunable by varying the arrival of time boundary with respect to that of the seed terahertz pulse. By numerical simulations and analysis with time-dependent coupled mode theory, we show that the wave amplification results from the ultrafast Q-switching and shift in resonant frequencies. This work demonstrates a new approach to achieve tunable amplification in an optical microcavity by exploiting the concept of time-variant media and the unique electromagnetic properties of Huygens metasurface