25 research outputs found

    MADE-in : a new aerosol microphysics submodel for global simulation of insoluble particles and their mixing state

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    Black carbon (BC) and mineral dust are among the most abundant insoluble aerosol components in the atmosphere. When released, most BC and dust particles are externally mixed with other aerosol species. Through coagulation with particles containing soluble material and condensation of gases, the externally mixed particles may obtain a liquid coating and be transferred into an internal mixture. The mixing state of BC and dust aerosol particles influences their radiative and hygroscopic properties, as well as their ability of forming ice crystals. We introduce the new aerosol microphysics submodel MADE-in, implemented within the ECHAM/MESSy Atmospheric Chemistry global model (EMAC). MADE-in is able to track mass and number concentrations of BC and dust particles in their different mixing states, as well as particles free of BC and dust. MADE-in describes these three classes of particles through a superposition of seven log-normally distributed modes, and predicts the evolution of their size distribution and chemical composition. Six out of the seven modes are mutually interacting, allowing for the transfer of mass and number among them. Separate modes for the different mixing states of BC and dust particles in EMAC/MADEin allow for explicit simulations of the relevant aging processes, i.e. condensation, coagulation and cloud processing. EMAC/MADE-in has been evaluated with surface and airborne measurements and mostly performs well both in the planetary boundary layer and in the upper troposphere and lowermost stratosphere

    Polar wandering in mantle convection models

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    cited By 44International audienceWe calculate polar motion in models of 3-D spherical mantle convection at Rayleigh numbers up to 108 which include internal heating, radial viscosity variations, and an endothermic phase change. Isoviscous models yield rapid polar motion of order 3°/Myr, but a factor of 30 increase in viscosity with depth reduces the rate of polar motion to about 0.5°/Myr due to stabilization of the large-scale pattern of convection. Avalanching due to an endothermic phase change causes pulsating inertial interchange polar excursions of order 80-110° and of duration 20-70 Myr. A layered viscosity model with an endothermic phase change yields only one inertial interchange event in 600 million years. These models show that the slow observed rate of post-Paleozoic true polar wander is not incompatible with higher rates inferred for earlier times. Copyright 1999 by the American Geophysical Union

    Mantle dynamics - A case study

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    Solid state convection in the rocky mantles is a key to understanding the thermochemical evolution and tectonics of terrestrial planets and moons. It is driven by internal heat and can be described by a system of coupled partial differential equations. There are no analytic solutions for realistic configurations and numerical models are an indispensable tool for researching mantle convection. After a brief general introduction, we introduce the basic equations that govern mantle convection and discuss some common approximations. The following case study is a contribution towards a self-consistent thermochemical evolution model of the Earth. A crude approximation for crustal differentiation is coupled to numerical models of global mantle convection, focussing on geometrical effects and the influence of rheology on stirring. We review Earth-specific geochemical and geophysical constraints, proposals for their reconciliation, and discuss the implications of our models for scenarios of the Earth’s evolution. Specific aspects of this study include the use of passive Lagrangian tracers, highly variable viscosity in 3-d spherical geometry, phase boundaries in the mantle and a parameterised model of the core as boundary condition at the bottom of the mantle

    MADE-in: a new aerosol microphysics submodel for global simulation of insoluble particles and their mixing state

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    Black carbon (BC) and mineral dust are among the most abundant insoluble aerosol components in the atmosphere. When released, most BC and dust particles are externally mixed with other aerosol species. Through coagulation with particles containing soluble material and condensation of gases, the externally mixed particles may obtain a liquid coating and be transferred into an internal mixture. The mixing state of BC and dust aerosol particles influences their radiative and hygroscopic properties, as well as their ability of forming ice crystals. We introduce the new aerosol microphysics submodel MADE-in, implemented within the ECHAM/MESSy Atmospheric Chemistry global model (EMAC). MADE-in is able to track mass and number concentrations of BC and dust particles in their different mixing states, as well as particles free of BC and dust. MADE-in describes these three classes of particles through a superposition of seven log-normally distributed modes, and predicts the evolution of their size distribution and chemical composition. Six out of the seven modes are mutually interacting, allowing for the transfer of mass and number among them. Separate modes for the different mixing states of BC and dust particles in EMAC/MADE-in allow for explicit simulations of the relevant aging processes, i.e. condensation, coagulation and cloud processing. EMAC/MADE-in has been evaluated with surface and airborne measurements and mostly performs well both in the planetary boundary layer and in the upper troposphere and lowermost stratosphere

    Observations of large reductions in NO/NOy ratio near the mid-latitude tropopause and the role of heterogeneous chemistry

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    Geophysical Research Letters, Vol. 23, No. 22, pp. 3223-3226, November 1, 1996.During the 1993 NASA Stratospheric Photochemistry, Aerosols and Dynamics Expedition (SPADE), anomalously low nitric oxide (NO) was found in a distinct sunlit layer located above the mid-latitude tropopause..

    Evaluating the role of NAT, NAD, and liquid H2SO4/H2O/HNO3 solutions in Antarctic polar stratospheric cloud aerosol: Observations and implications

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    Journal of Geophysical Research, Vol. 102, No. D11 pp. 13,255-13,282.Airborne measurements of total reactive nitrogen (NOy) and polar stratospheric cloud (PSC) aerosol particles were made in the Antarctic (68 degrees S) as part of the NASA Airborne Southern Hemisphere Ozone Experiment/Measurements for Assessing the Effects of the Stratospheric Aircraft (ASHOE/MAESA) campaign in late July 1994..
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