159 research outputs found

    On the transport and thermodynamic properties of quasi-two-dimensional purple bronzes A0.9_{0.9}Mo6_6O17_{17} (A=Na, K)

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    We report a comparative study of the specific heat, electrical resistivity and thermal conductivity of the quasi-two-dimensional purple bronzes Na0.9_{0.9}Mo6_6O17_{17} and K0.9_{0.9}Mo6_6O17_{17}, with special emphasis on the behavior near their respective charge-density-wave transition temperatures TPT_P. The contrasting behavior of both the transport and the thermodynamic properties near TPT_P is argued to arise predominantly from the different levels of intrinsic disorder in the two systems. A significant proportion of the enhancement of the thermal conductivity above TPT_P in Na0.9_{0.9}Mo6_6O17_{17}, and to a lesser extent in K0.9_{0.9}Mo6_6O17_{17}, is attributed to the emergence of phason excitations.Comment: 8 pages, 6 figures, To appear in Physical Review

    Fermiology and electronic homogeneity of the superconducting overdoped cuprate Tl-2201 revealed by quantum oscillations

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    We report an angular quantum oscillation study of Tl_2Ba_2CuO_{6+delta} for two different doping levels (Tc = 10K and 26 K) and determine the Fermi surface size and topology in considerable detail. Our results show that Fermi liquid behavior is not confined to the edge of the superconducting dome and is robust up to at least T_c^{max}/3.5. Superconductivity is found to survive up to a larger doping p_c = 0.31 than in La_{2-x}Sr_xCuO_4. Our data imply that electronic inhomogeneity does not play a significant role in the loss of superconductivity and superfluid density in overdoped cuprates, and point towards a purely magnetic or electronic pairing mechanismComment: 4 page

    Quantum oscillations in the parent pnictide BaFe2_2As2_2 : itinerant electrons in the reconstructed state

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    We report quantum oscillation measurements that enable the direct observation of the Fermi surface of the low temperature ground state of \ba122. From these measurements we characterize the low energy excitations, revealing that the Fermi surface is reconstructed in the antiferromagnetic state, but leaving itinerant electrons in its wake. The present measurements are consistent with a conventional band folding picture of the antiferromagnetic ground state, placing important limits on the topology and size of the Fermi surface.Comment: 5 pages, 3 figure

    Fermi-surface reconstruction and two-carrier model for the Hall effect in YBa2Cu4O8

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    Pulsed field measurements of the Hall resistivity and magnetoresistance of underdoped YBa2Cu4O8 are analyzed self-consistently using a simple model based on coexisting electron and hole carriers. The resultant mobilities and Hall numbers are found to vary markedly with temperature. The conductivity of the hole carriers drops by one order of magnitude below 30 K, explaining the absence of quantum oscillations from these particular pockets. Meanwhile the Hall coefficient of the electron carriers becomes strongly negative below 50 K. The overall quality of the fits not only provides strong evidence for Fermi-surface reconstruction in Y-based cuprates, it also strongly constrains the type of reconstruction that might be occurring.Comment: 5 pages, 4 figures, updated after publication in Physical Review B (Rapid Communication

    Topological change of the Fermi surface in ternary iron-pnictides with reduced c/a ratio: A dHvA study of CaFe2P2

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    We report a de Haas-van Alphen effect study of the Fermi surface of CaFe2P2 using low temperature torque magnetometry up to 45 T. This system is a close structural analogue of the collapsed tetragonal non-magnetic phase of CaFe2As2. We find the Fermi surface of CaFe2P2 to differ from other related ternary phosphides in that its topology is highly dispersive in the c-axis, being three-dimensional in character and with identical mass enhancement on both electron and hole pockets (~1.5). The dramatic change in topology of the Fermi surface suggests that in a state with reduced (c/a) ratio, when bonding between pnictogen layers becomes important, the Fermi surface sheets are unlikely to be nested

    Enhanced electron correlations in the new binary stannide PdSn4: a homologue of the Dirac nodal arc semimetal PtSn4

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    The advent of nodal-line semi-metals, i.e. systems in which the conduction and valence bands cross each other along a closed trajectory (line or loop) inside the Brillouin zone, has opened up a new arena for the exploration of topological condensed matter in which, due to a vanishing density of states near the Fermi level, electron correlation effects may also play an important role. In spite of this conceptual richness however, material realization of nodal-line (loop) fermions is rare, with PbTaSe2, ZrSiS and PtSn4 the only promising known candidates. Here we report the synthesis and physical properties of a new compound PdSn4 that is isostructural with PtSn4 yet possesses quasiparticles with significantly enhanced effective masses. In addition, PdSn4 displays an unusual polar angular magnetoresistance which at a certain field orientation, varies linearly with field up to 55 Tesla. Our study suggests that, in association with its homologue PtSn4 whose low-lying excitations were recently claimed to possess Dirac node arcs, PdSn4 may be a promising candidate in the search for novel topological states with enhanced correlation effects.Comment: 6 figures, 1 tabl
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