302 research outputs found

    Superconductivity in Weyl semimetal NbP: Bulk vs. surface

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    Transition metal monopnictides belong to the new class of semimetals where the bulk properties are determined by the presence of pairs of nodes with different chirality formed by linear dispersive states in the k-space. Beside the anomaly in the bulk magnetotransport superconductivity is frequently found in some Weyl semimetals. We found signatures of superconductivity in ac and dc magnetization measurements of highly pure and stoichiometric NbP powder. We determined the lower and upper critical field and the Ginzburg-Landau parameter. The relative small superconducting volume fraction is related to either effect of finite grain size and/or surface superconductivity. The last mentioned may originate from either off stoichiometric (Nb-rich) surface layers or a strained surface with different electronic properties. Furthermore the intrinsic normal state susceptibility is determined taking into account a paramagnetic contribution of a few ppm of magnetic impurities

    Nuclear spin-lattice relaxation time in TaP and the Knight shift of Weyl semimetals

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    We first analyze the recent experimental data on the nuclear spin-lattice relaxation rate of the Weyl semimetal TaP. We argue that its non-monotonic temperature dependence is explained by the temperature dependent chemical potential of Weyl fermions. We also develop the theory of the Knight shift in Weyl semimetals, which contains two counteracting terms. The diamagnetic term follows ln[W/max(μ,kBT)]-\ln[W/\max(|\mu|,k_BT)] with WW, μ\mu and TT being the high energy cutoff, chemical potential and temperature, respectively, and is always negative. The paramagnetic term scales with μ\mu and changes sign depending on the doping level. Altogether, the Knight shift is predicted to vanish or even change sign upon changing the doping or the temperature, making it a sensitive tool to identify Weyl points. We also calculate the Korringa relation for Weyl semimetals which shows an unusual energy dependence rather than being constant as expected for a non-interacting Fermi system.Comment: 9 pages, 3 figure

    Quantum phase transition in the dioptase magnetic lattice

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    The study of quantum phase transitions, which are zero-temperature phase transitions between distinct states of matter, is of current interest in research since it allows for a description of low-temperature properties based on universal relations. Here we show that the crystal green dioptase Cu_6Si_6O_18 . 6H_2O, known to the ancient Roman as the gem of Venus, has a magnetic crystal structure, formed by the Cu(II) ions, which allows for a quantum phase transition between an antiferromagnetically ordered state and a quantum spin liquid.Comment: 6 pages, 5 figures, EPL, in pres

    121,123Sb NQR as a microscopic probe in Te doped correlated semimetal FeSb2 : emergence of electronic Griffith phase, magnetism and metallic behavior %

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    121,123Sb^{121,123}Sb nuclear quadrupole resonance (NQR) was applied to Fe(Sb1xTex)2Fe(Sb_{1-x}Te_x)_2 in the low doping regime (\emph{x = 0, 0.01} and \emph{0.05}) as a microscopic zero field probe to study the evolution of \emph{3d} magnetism and the emergence of metallic behavior. Whereas the NQR spectra itself reflects the degree of local disorder via the width of the individual NQR lines, the spin lattice relaxation rate (SLRR) 1/T1(T)1/T_1(T) probes the fluctuations at the SbSb - site. The fluctuations originate either from conduction electrons or from magnetic moments. In contrast to the semi metal FeSb2FeSb_2 with a clear signature of the charge and spin gap formation in 1/T1(T)T(exp/(ΔkBT))1/T_1(T)T ( \sim exp/ (\Delta k_BT) ) , the 1\% TeTe doped system exhibits almost metallic conductivity and a almost filled gap. A weak divergence of the SLRR coefficient 1/T1(T)TTnT0.21/T_1(T)T \sim T^{-n} \sim T^{-0.2} points towards the presence of electronic correlations towards low temperatures wheras the \textit{5\%} TeTe doped sample exhibits a much larger divergence in the SLRR coefficient showing 1/T1(T)TT0.721/T_1(T)T \sim T^{-0.72} . According to the specific heat divergence a power law with n = 2 m = 0.56n\ =\ 2\ m\ =\ 0.56 is expected for the SLRR. Furthermore TeTe-doped FeSb2FeSb_2 as a disordered paramagnetic metal might be a platform for the electronic Griffith phase scenario. NQR evidences a substantial asymmetric broadening of the 121,123Sb^{121,123}Sb NQR spectrum for the \emph{5\%} sample. This has purely electronic origin in agreement with the electronic Griffith phase and stems probably from an enhanced SbSb-TeTe bond polarization and electronic density shift towards the TeTe atom inside SbSb-TeTe dumbbell

    Complex Chiral Modulations in FeGe close to Magnetic Ordering

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    We report on detailed polarized small-angle neutron scattering on cubic FeGe in magnetic fields applied either along (transverse) the scattering vector or parallel (longitudinal)to the neutron beam. The (H,TH,T) phase diagrams for all principal axes contain a segmented AA-phase region just below the onset of magnetic order. Hexagonal Bragg-spot patterns were observed across the entire AA-phase region for the longitudinal geometry. Scattering intensity was observed in parts of the A phase for both scattering configurations. Only in a distinct pocket (A1A_1) vanishing scattering intensity was found in the transverse geometry.Comment: This paper has been withdrawn by the author due to misunderstanding with some of the co-author

    Field tuned critical fluctuations in YFe2Al10: Evidence from magnetization, 27Al (NMR, NQR) investigations

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    We report magnetization, specific heat, and NMR investigations on YFe2Al10 over a wide range in temperature and magnetic field and zero field (NQR) measurements. Magnetic susceptibility, specific heat and spin-lattice relaxation rate divided by T (1/T1T) follow a weak power law (T^-0.4) temperature dependence, which is a signature of critical fluctuations of Fe moments. The value of the Sommerfeld-Wilson ratio and linear relation between 1/T1T and chi(T) suggest the existence of ferromagnetic correlations in this system. No magnetic ordering down to 50 mK in Cp(T) and the unusual temperature and field scaling of the bulk and NMR data are associated with a magnetic instability which drives the system to quantum criticality. The magnetic properties of the system are tuned by field wherein ferromagnetic fluctuations are suppressed and a crossover from quantum critical to FL behavior is observed with increasing magnetic field

    Magnetism and superconductivity in Eu0.2Sr0.8(Fe0.86Co0.14)2As2 probed by 75As NMR

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    We report bulk superconductivity (SC) in Eu0.2_{0.2}Sr0.8_{0.8}(Fe0.86_{0.86}Co0.14_{0.14})2_{2}As2_{2} single crystals by means of electrical resistivity, magnetic susceptibility, and specific heat measurements with TTc_{\mathrm{c}} \simeq 20 K with an antiferromagnetic (AFM) ordering of Eu2+^{2+} moments at TTN_{\mathrm{N}} \simeq 2.0 K in zero field. 75^{75}As NMR experiments have been performed in the two external field directions (Hab\|ab) and (Hc\|c). 75^{75}As-NMR spectra are analyzed in terms of first order quadrupolar interaction. Spin-lattice relaxation rates (1/T1T_{1}) follow a T3T^{3} law in the temperature range 4.2-15 K. There is no signature of Hebel-Slichter coherence peak just below the SC transition indicating a non s-wave or s±_{\pm} type of superconductivity. The increase of 1/T1TT_{1}T with lowering the temperature in the range 160-18 K following CT+θ\frac{C}{T+\theta} law reflecting 2D AFM spin fluctuations
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