Atomic fountains and optical clocks at SYRTE: status and perspectives

In this article, we report on the work done with the LNE-SYRTE atomic clock ensemble during the last 10 years. We cover progress made in atomic fountains and in their application to timekeeping. We also cover the development of optical lattice clocks based on strontium and on mercury. We report on tests of fundamental physical laws made with these highly accurate atomic clocks. We also report on work relevant to a future possible redefinition of the SI second

An Optical Lattice Clock with Spin-polarized 87Sr Atoms

We present a new evaluation of an 87Sr optical lattice clock using spin polarized atoms. The frequency of the 1S0-3P0 clock transition is found to be 429 228 004 229 873.6 Hz with a fractional accuracy of 2.6 10^{-15}, a value that is comparable to the frequency difference between the various primary standards throughout the world. This measurement is in excellent agreement with a previous one of similar accuracy

Near-to mid-IR spectral purity transfer with a tunable frequency comb: methanol frequency metrology over a record frequency span

We report the development and operation of a frequency-comb-assisted high-resolution mid-infrared molecular spectrometer combining high spectral purity, SI-traceability, wide tunability and high sensitivity. An optical frequency comb is used to transfer the spectral purity of a SI-traceable 1.54 $\mu$m metrology-grade frequency reference to a 10.3 $\mu$m quantum cascade laser (QCL). The near-infrared reference is operated at the French time/frequency metrology institute, calibrated there to primary frequency standards, and transferred to Laboratoire de Physique des Lasers via the REFIMEVE fiber network. The QCL exhibits a sub-10 --15 frequency stability from 0.1 to 10 s and its frequency is traceable to the SI with a total uncertainty better than 4 x 10 --14 after 1-s averaging time. We have developed the instrumentation allowing comb modes to be continuously tuned over 9 GHz resulting in a QCL of record spectral purity uninterruptedly tunable at the precision of the reference over an unprecedented span of 1.4 GHz. We have used our apparatus to conduct sub-Doppler spectroscopy of methanol in a multi-pass cell, demonstrating state-of-art frequency uncertainties down to the few kilohertz level. We have observed weak intensity resonances unreported so far, resolved subtle doublets never seen before and brought to light discrepancies with the HITRAN database. This demonstrates the potential of our apparatus for probing subtle internal molecular processes, building accurate spectroscopic models of polyatomic molecules of atmospheric or astrophysical interest, and carrying out precise spectroscopic tests of fundamental physics

Experimenting an optical second with strontium lattice clocks

Progress in realizing the SI second had multiple technological impacts and enabled to further constraint theoretical models in fundamental physics. Caesium microwave fountains, realizing best the second according to its current definition with a relative uncertainty of 2-4x10^(-16), have already been superseded by atomic clocks referenced to an optical transition, both more stable and more accurate. Are we ready for a new definition of the second? Here we present an important step in this direction: our system of five clocks connects with an unprecedented consistency the optical and the microwave worlds. For the first time, two state-of-the-art strontium optical lattice clocks are proven to agree within their accuracy budget, with a total uncertainty of 1.6x10^(-16). Their comparison with three independent caesium fountains shows a degree of reproducibility henceforth solely limited at the level of 3.1x10^(-16) by the best realizations of the microwave-defined second.Comment: 9 pages, 4 figures, 2 table

Development of a strontium optical lattice clock for the SOC mission on the ISS

Ultra-precise optical clocks in space will allow new studies in fundamental physics and astronomy. Within an European Space Agency (ESA) program, the Space Optical Clocks (SOC) project aims to install and to operate an optical lattice clock on the International Space Station (ISS) towards the end of this decade. It would be a natural follow-on to the ACES mission, improving its performance by at least one order of magnitude. The payload is planned to include an optical lattice clock, as well as a frequency comb, a microwave link, and an optical link for comparisons of the ISS clock with ground clocks located in several countries and continents. Within the EU-FP7-SPACE-2010-1 project no. 263500, during the years 2011-2015 a compact, modular and robust strontium lattice optical clock demonstrator has been developed. Goal performance is a fractional frequency instability below 1x10^{-15}, tau^{-1/2} and a fractional inaccuracy below 5x10^{-17}. Here we describe the current status of the apparatus' development, including the laser subsystems. Robust preparation of cold {88}^Sr atoms in a second stage magneto-optical trap (MOT) is achieved.Comment: 27 Pages, 15 figures, Comptes Rendus Physique 201

Development of a strontium optical lattice clock for the SOC mission on the ISS

The ESA mission "Space Optical Clock" project aims at operating an optical lattice clock on the ISS in approximately 2023. The scientific goals of the mission are to perform tests of fundamental physics, to enable space-assisted relativistic geodesy and to intercompare optical clocks on the ground using microwave and optical links. The performance goal of the space clock is less than $1 \times 10^{-17}$ uncertainty and $1 \times 10^{-15} {\tau}^{-1/2}$ instability. Within an EU-FP7-funded project, a strontium optical lattice clock demonstrator has been developed. Goal performances are instability below $1 \times 10^{-15} {\tau}^{-1/2}$ and fractional inaccuracy $5 \times 10^{-17}$. For the design of the clock, techniques and approaches suitable for later space application are used, such as modular design, diode lasers, low power consumption subunits, and compact dimensions. The Sr clock apparatus is fully operational, and the clock transition in $^{88}$Sr was observed with linewidth as small as 9 Hz.Comment: 12 pages, 8 figures, SPIE Photonics Europe 201

First-order thermal insensitivity of the frequency of a narrow spectral hole in a crystal

International audienc

First-order thermal insensitivity of the frequency of a narrow spectral hole in a crystal

International audienc