168 research outputs found
Scaled Spectroscopy of 1Se and 1Po Highly Excited States of Helium
In this paper, we examine the properties of the 1Se and 1Po states of helium,
combining perimetric coordinates and complex rotation methods. We compute
Fourier transforms of quantities of physical interest, among them the average
of the operator cos(theta_12), which measures the correlation between the two
electrons. Graphs obtained for both 1Se and 1Po states show peaks at action of
classical periodic orbits, either "frozen planet" orbit or asymmetric stretch
orbits. This observation legitimates the semiclassical quantization of helium
with those orbits only, not just for S states but also for P states, which is a
new result. To emphasize the similarity between the S and P states we show
wavefunctions of 1Po states, presenting the same structure as 1Se states,
namely the "frozen planet" and asymmetric stretch configurations.Comment: revtex 15 pages with 6 figures, 2 figures (large) are available on
request at email address [email protected]. to appear in J. Phys. B
(April 98
Coherent Backscattering with Nonlinear Atomic Scatterers
We study coherent backscattering of a quasi-monochromatic laser by a dilute
gas of cold two-level atoms. We consider the perturbative regime of weak
intensities, where nonlinear effects arise from {\em inelastic} two-photon
scattering processes. Here, coherent backscattering can be formed by
interference between {\em three} different scattering amplitudes. Consequently,
if elastically scattered photons are filtered out from the photodetection
signal by means of suitable frequency-selective detection, we find the
nonlinear backscattering enhancement factor to exceed the linear barrier two.Comment: 4 pages, 3 figure
Comment on ``Intensity correlations and mesoscopic fluctuations of diffusing photons in cold atoms''
In a recent Letter (Phys. Rev. Lett. \textbf{98}, 083601 (2007),
arXiv:cond-mat/0610804), O. Assaf and E. Akkermans claim that the angular
correlations of the light intensity scattered by a cloud of cold atoms with
internal degeneracy (Zeeman sublevels) of the ground state overcome the usual
Rayleigh law. More precisely, they found that they become exponentially large
with the size of the sample. In what follows, we will explain why their results
are wrong and, in contrary, why the internal degeneracy leads to lower
intensity correlations.Comment: 1 page. Comment submitted to PR
Finite temperature QMC study of the one-dimensional polarized Fermi gas
Quantum Monte Carlo (QMC) techniques are used to provide an
approximation-free investigation of the phases of the one-dimensional
attractive Hubbard Hamiltonian in the presence of population imbalance. The
temperature at which the "Fulde-Ferrell-Larkin-Ovchinnikov" (FFLO) phase is
destroyed by thermal fluctuations is determined as a function of the
polarization. It is shown that the presence of a confining potential does not
dramatically alter the FFLO regime, and that recent experiments on trapped
atomic gases likely lie just within the stable temperature range.Comment: 10 pages, 13 figures We added a discussion of the behaviour of the
FFLO peak as a function of the attractive interaction strengt
Attractive Hubbard Model on a Honeycomb Lattice
We study the attractive fermionic Hubbard model on a honeycomb lattice using
determinantal quantum Monte Carlo simulations. By increasing the interaction
strength U (relative to the hopping parameter t) at half-filling and zero
temperature, the system undergoes a quantum phase transition at 5.0 < U_c/t <
5.1 from a semi-metal to a phase displaying simultaneously superfluid behavior
and density order. Doping away from half-filling, and increasing the
interaction strength at finite but low temperature T, the system always appears
to be a superfluid exhibiting a crossover between a BCS and a molecular regime.
These different regimes are analyzed by studying the spectral function. The
formation of pairs and the emergence of phase coherence throughout the sample
are studied as U is increased and T is lowered
An optical method to determine the thermodynamics of hydrogen absorption and desorption in metals
Hydrogenography, an optical high-throughput combinatorial technique to find hydrogen storage materials, has so far been applied only to materials undergoing a metal-to-semiconductor transition during hydrogenation. We show here that this technique works equally well for metallic hydrides. Additionally, we find that the thermodynamic data obtained optically on thin Pd-H films agree very well with Pd-H bulk data. This confirms that hydrogenography is a valuable general method to determine the relevant parameters for hydrogen storage in metal hydrides. © 2007 American Institute of Physics
Structural and optical properties of Mg<sub>x</sub>Al<sub>1-x</sub>H<sub>y</sub> gradient thin films: a combinatorial approach
The structural, optical and dc electrical properties of MgxAl1-x (0.2≤x≤0.9) gradient thin films covered with Pd/Mg are investigated before and after exposure to hydrogen. We use hydrogenography, a novel high-throughput optical technique, to map simultaneously all the hydride forming compositions and the kinetics thereof in the gradient thin film. Metallic Mg in the MgxAl1-x layer undergoes a metal-to-semiconductor transition and MgH₂ is formed for all Mg fractions x investigated. The presence of an amorphous Mg-Al phase in the thin film phase diagram enhances strongly the kinetics of hydrogenation. In the Al-rich part of the film, a complex H-induced segregation of MgH₂ and Al occurs. This uncommon large-scale segregation is evidenced by metal and hydrogen profiling using Rutherford backscattering spectrometry and resonant nuclear analysis based on the reaction ¹H(¹⁵N,αγ)¹²C. Besides MgH₂, an additional semiconducting phase is found by electrical conductivity measurements around an atomic [Al]/[Mg] ratio of 2 (x=0.33). This suggests that the film is partially transformed into Mg(AlH₄)₂ at around this composition
Statistics of S-matrix poles in Few-Channel Chaotic Scattering: Crossover from Isolated to Overlapping Resonances
We derive the explicit expression for the distribution of resonance widths in
a chaotic quantum system coupled to continua via M equivalent open channels. It
describes a crossover from the distribution (regime of isolated
resonances) to a broad power-like distribution typical for the regime of
overlapping resonances. The first moment is found to reproduce exactly the
Moldauer-Simonius relation between the mean resonance width and the
transmission coefficient. This fact may serve as another manifestation of
equivalence between the spectral and the ensemble averaging.Comment: 4 two-column pages, RevTex. text is slightly modified; some misprints
are correcte
Electronic structure and optical properties of lightweight metal hydrides
We study the electronic structures and dielectric functions of the simple
hydrides LiH, NaH, MgH2 and AlH3, and the complex hydrides Li3AlH6, Na3AlH6,
LiAlH4, NaAlH4 and Mg(AlH4)2, using first principles density functional theory
and GW calculations. All these compounds are large gap insulators with GW
single particle band gaps varying from 3.5 eV in AlH3 to 6.5 eV in the MAlH4
compounds. The valence bands are dominated by the hydrogen atoms, whereas the
conduction bands have mixed contributions from the hydrogens and the metal
cations. The electronic structure of the aluminium compounds is determined
mainly by aluminium hydride complexes and their mutual interactions. Despite
considerable differences between the band structures and the band gaps of the
various compounds, their optical responses are qualitatively similar. In most
of the spectra the optical absorption rises sharply above 6 eV and has a strong
peak around 8 eV. The quantitative differences in the optical spectra are
interpreted in terms of the structure and the electronic structure of the
compounds.Comment: 13 pages, 10 figure
- …