168 research outputs found
Magnetic structure of the edge-sharing copper oxide chain compound NaCu2O2
Single-crystal neutron diffraction has been used to determine the
incommensurate magnetic structure of NaCu2O2, a compound built up of chains of
edge-sharing CuO4 plaquettes. Magnetic structures compatible with the lattice
symmetry were identified by a group-theoretical analysis, and their magnetic
structure factors were compared to the experimentally observed Bragg
intensities. In conjunction with other experimental data, this analysis yields
an elliptical helix structure in which both the helicity and the polarization
plane alternate among copper-oxide chains. This magnetic ground state is
discussed in the context of the recently reported multiferroic properties of
other copper-oxide chain compounds
Incommensurate spin density modulation in a copper-oxide chain compound with commensurate charge order
Neutron diffraction has been used to determine the magnetic structure of
NaCuO, a stoichiometric compound containing chains based on
edge-sharing CuO plaquettes. The chains are doped with 2/5 hole per Cu site
and exhibit long-range commensurate charge order with an onset well above room
temperature. Below K, the neutron data indicate long-range collinear
magnetic order with a spin density modulation whose propagation vector is
commensurate along and incommensurate perpendicular to the chains. Competing
interchain exchange interactions are discussed as a possible origin of the
incommensurate magnetic order
Helicoidal magnetic order in a clean copper oxide spin chain compound
We report susceptibility, specific heat, and neutron diffraction measurements
on NaCuO, a spin-1/2 chain compound isostructural to LiCuO,
which has been extensively investigated. Below 13 K, we find a long-range
ordered, incommensurate magnetic helix state with a propagation vector similar
to that of LiCuO. In contrast to the Li analogue, substitutional
disorder is negligible in NaCuO. We can thus rule out that the helix is
induced by impurities, as was claimed on the basis of prior work on
LiCuO. A spin Hamiltonian with frustrated longer-range exchange
interactions provides a good description of both the ordered state and the
paramagnetic susceptibility.Comment: 4 pages, 4 figures Improved Fig.1 and 4. Minor rephrasing. Reference
adde
Hall Effect in Nested Antiferromagnets Near the Quantum Critical Point
We investigate the behavior of the Hall coefficient in the case of
antiferromagnetism driven by Fermi surface nesting, and find that the Hall
coefficient should abruptly increase with the onset of magnetism, as recently
observed in vanadium doped chromium. This effect is due to the sudden removal
of flat portions of the Fermi surface upon magnetic ordering. Within this
picture, the Hall coefficient should scale as the square of the residual
resistivity divided by the impurity concentration, which is consistent with
available data.Comment: published version; an accidental interchange in the quoting of
analytic dependencies was correcte
Magnetic excitations and phonons in the spin-chain compound NaCu2O2
We report an inelastic light scattering study of single-crystalline
NaCuO, a spin-chain compound known to exhibit a phase with helical
magnetic order at low temperatures. Phonon excitations were studied as a
function of temperature and light polarization, and the phonon frequencies are
compared to the results of ab-initio lattice dynamical calculations, which are
also reported here. The good agreement between the observed and calculated
modes allows an assignment of the phonon eigenvectors. Two distinct high-energy
two-magnon features as well as a sharp low-energy one-magnon peak were also
observed. These features are discussed in terms of the magnon modes expected in
a helically ordered state. Their polarization dependence provides evidence of
substantial exchange interactions between two closely spaced spin chains within
a unit cell. At high temperatures, the spectral features attributable to
magnetic excitations are replaced by a broad, quasielastic mode due to
overdamped spin excitations
Dispersion of the odd magnetic resonant mode in near-optimally doped Bi2Sr2CaCu2O8+d
We report a neutron scattering study of the spin excitation spectrum in the
superconducting state of slightly overdoped Bi2Sr2CaCu2O8+d system (Tc=87 K).
We focus on the dispersion of the resonance peak in the superconducting state
that is due to a S=1 collective mode. The measured spin excitation spectrum
bears a strong similarity to the spectrum of the YBa2Cu3O6+x system for a
similar doping level i.e. x= 0.95-1), which consists of intersecting upward-
and downward-dispersing branches. A close comparison of the threshold of the
electron-hole spin flip continuum, deduced from angle resolved photo-emission
measurements in the same system, indicates that the magnetic response in the
superconducting state is confined, in both energy and momentum, below the
gapped Stoner continuum. In contrast to YBa2Cu3O6+x, the spin excitation
spectrum is broader than the experimental resolution. In the framework of an
itinerant-electron model, we quantitatively relate this intrinsic energy width
to the superconducting gap distribution observed in scanning tunnelling
microscopy experiments. Our study further suggests a significant in-plane
anisotropy of the magnetic response.Comment: 10 figure
Dipole-active optical phonons in YTiO_3: ellipsometry study and lattice-dynamics calculations
The anisotropic complex dielectric response was accurately extracted from
spectroscopic ellipsometry measurements at phonon frequencies for the three
principal crystallographic directions of an orthorhombic (Pbnm) YTiO_3 single
crystal. We identify all twenty five infrared-active phonon modes allowed by
symmetry, 7B_1u, 9B_2u, and 9B_3u, polarized along the c-, b-, and a-axis,
respectively. From a classical dispersion analysis of the complex dielectric
functions \tilde\epsilon(\omega) and their inverses -1/\tilde\epsilon(\omega)
we define the resonant frequencies, widths, and oscillator strengths of the
transverse (TO) and longitudinal (LO) phonon modes. We calculate
eigenfrequencies and eigenvectors of B_1u, B_2u, and B_3u normal modes and
suggest assignments of the TO phonon modes observed in our ellipsometry spectra
by comparing their frequencies and oscillator strengths with those resulting
from the present lattice-dynamics study. Based on these assignments, we
estimate dynamical effective charges of the atoms in the YTiO_3 lattice. We
find that, in general, the dynamical effective charges in YTiO_3 lattice are
typical for a family of perovskite oxides. By contrast to a ferroelectric
BaTiO_3, the dynamical effective charge of oxygen related to a displacement
along the c-axis does not show the anomalously large value. At the same time,
the dynamical effective charges of Y and ab-plane oxygen exhibit anisotropy,
indicating strong hybridization along the a-axis.Comment: 8 pages, 7 figure
On the Alexandrov Topology of sub-Lorentzian Manifolds
It is commonly known that in Riemannian and sub-Riemannian Geometry, the
metric tensor on a manifold defines a distance function. In Lorentzian
Geometry, instead of a distance function it provides causal relations and the
Lorentzian time-separation function. Both lead to the definition of the
Alexandrov topology, which is linked to the property of strong causality of a
space-time. We studied three possible ways to define the Alexandrov topology on
sub-Lorentzian manifolds, which usually give different topologies, but agree in
the Lorentzian case. We investigated their relationships to each other and the
manifold's original topology and their link to causality.Comment: 20 page
First and second variation formulae for the sub-Riemannian area in three-dimensional pseudo-hermitian manifolds
We calculate the first and the second variation formula for the
sub-Riemannian area in three dimensional pseudo-hermitian manifolds. We
consider general variations that can move the singular set of a C^2 surface and
non-singular variation for C_H^2 surfaces. These formulas enable us to
construct a stability operator for non-singular C^2 surfaces and another one
for C2 (eventually singular) surfaces. Then we can obtain a necessary condition
for the stability of a non-singular surface in a pseudo-hermitian 3-manifold in
term of the pseudo-hermitian torsion and the Webster scalar curvature. Finally
we classify complete stable surfaces in the roto-traslation group RT .Comment: 36 pages. Misprints corrected. Statement of Proposition 9.8 slightly
changed and Remark 9.9 adde
Metamagnetism and critical fluctuations in high quality single crystals of the bilayer ruthenate Sr3Ru2O7
We report the results of low temperature transport, specific heat and
magnetisation measurements on high quality single crystals of the bilayer
perovskite Sr3Ru2O7, which is a close relative of the unconventional
superconductor Sr2RuO4. Metamagnetism is observed, and transport and
thermodynamic evidence for associated critical fluctuations is presented. These
relatively unusual fluctuations might be pictured as variations in the Fermi
surface topography itself. No equivalent behaviour has been observed in the
metallic state of Sr2RuO4.Comment: 4 pages, 4 figures, Revtex 3.
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