495 research outputs found
A perturbative approach to J mixing in f-electron systems: Application to actinide dioxides
We present a perturbative model for crystal-field calculations, which keeps
into account the possible mixing of states labelled by different quantum number
J. Analytical J-mixing results are obtained for a Hamiltonian of cubic symmetry
and used to interpret published experimental data for actinide dioxides. A
unified picture for all the considered compounds is proposed by taking into
account the scaling properties of the crystal-field potential.Comment: 16 pages + 4 figures; will appear http://prb.aps.or
Enhancement of rare-earth--transition-metal exchange interaction in PrFe probed by inelastic neutron scattering
The fundamental magnetic interactions of PrFe are studied by
inelastic neutron scattering and anisotropy field measurements. Data analysis
confirms the presence of three magnetically inequivalent sites, and reveals an
exceptionally large value of the exchange field. The unexpected importance of
-mixing effects in the description of the ground-state properties of
PrFe is evidenced, and possible applications of related compounds
are envisaged.Comment: 4 RevTeX pages, 4 EPS figures. Accepted for publication by Appl.
Phys. Lett. (will be found at http://apl.aip.org
The First Cold Antihydrogen
Antihydrogen, the atomic bound state of an antiproton and a positron, was
produced at low energy for the first time by the ATHENA experiment, marking an
important first step for precision studies of atomic antimatter. This paper
describes the first production and some subsequent developments.Comment: Invitated Talk at COOL03, International Workshop on Beam Cooling and
Related Topics, to be published in NIM
Magnetic Susceptibility of Multiorbital Systems
Effects of orbital degeneracy on magnetic susceptibility in paramagnetic
phases are investigated within a mean-field theory. Under certain crystalline
electric fields, the magnetic moment consists of two independent moments, e.g.,
spin and orbital moments. In such a case, the magnetic susceptibility is given
by the sum of two different Curie-Weiss relations, leading to deviation from
the Curie-Weiss law. Such behavior may be observed in d- and f-electron systems
with t_{2g} and Gamma_8 ground states, respectively. As a potential application
of our theory, we attempt to explain the difference in the temperature
dependence of magnetic susceptibilities of UO_2 and NpO_2.Comment: 4 pages, 3 figure
A Scalable and Secure Publish/Subscribe-based Framework for Industrial IoT
In the emerging Industrial Internet of Things (IIoT) scenario machine-to-machine communication is a key technology to set up environments wherein sensors, actuators, and controllers can exchange information autonomously. However, many current communication frameworks do not provide enough dynamic interoperability and security. Hence, we propose a novel communication framework, based on MQTT broker bridging, which, in an Industrial IoT scenario, can foster dynamic interoperability across different production lines or industrial sites, guaranteeing, at the same time, a higher degree of isolation and control over the information flows, thereby increasing the overall security of the whole scenario. The solution we propose does also support dynamic authentication and authorization and has been practically implemented and evaluated in a proper small-scale IIoT testbed, encompassing PLCs, IIoT gateways, as well as MQTT brokers with novel and extended capabilities. The evaluation results demonstrate a linear time complexity for all the considered implementations and bridging modes of the extended brokers. Moreover, all considered access token encapsulation techniques demonstrate a minimum overhead in comparison with standard MQTT brokers
Antihydrogen formation dynamics in a multipolar neutral anti-atom trap
Antihydrogen production in a neutral atom trap formed by an octupole-based
magnetic field minimum is demonstrated using field-ionization of weakly bound
anti-atoms. Using our unique annihilation imaging detector, we correlate
antihydrogen detection by imaging and by field-ionization for the first time.
We further establish how field-ionization causes radial redistribution of the
antiprotons during antihydrogen formation and use this effect for the first
simultaneous measurements of strongly and weakly bound antihydrogen atoms.
Distinguishing between these provides critical information needed in the
process of optimizing for trappable antihydrogen. These observations are of
crucial importance to the ultimate goal of performing CPT tests involving
antihydrogen, which likely depends upon trapping the anti-atom
Spin dynamics of heterometallic Cr7M wheels (M = Mn, Zn, Ni) probed by inelastic neutron scattering
Inelastic neutron scattering has been applied to the study of the spin
dynamics of Cr-based antiferromagnetic octanuclear rings where a finite total
spin of the ground state is obtained by substituting one Cr(III) ion (s = 3/2)
with Zn (s = 0), Mn (s = 5/2) or Ni (s = 1) di-cations. Energy and intensity
measurements for several intra-multiplet and inter-multiplet magnetic
excitations allow us to determine the spin wavefunctions of the investigated
clusters. Effects due to the mixing of different spin multiplets have been
considered. Such effects proved to be important to correctly reproduce the
energy and intensity of magnetic excitations in the neutron spectra. On the
contrary to what is observed for the parent homonuclear Cr8 ring, the symmetry
of the first excited spin states is such that anticrossing conditions with the
ground state can be realized in the presence of an external magnetic field.
Heterometallic Cr7M wheels are therefore good candidates for macroscopic
observations of quantum effects.Comment: 9 pages, 11 figures, submitted to Phys. Rev. B, corrected typos and
added references, one sentence change
Molecular engineering of antiferromagnetic rings for quantum computation
The substitution of one metal ion in a Cr-based molecular ring with dominant
antiferromagnetic couplings allows to engineer its level structure and
ground-state degeneracy. Here we characterize a Cr7Ni molecular ring by means
of low-temperature specific-heat and torque-magnetometry measurements, thus
determining the microscopic parameters of the corresponding spin Hamiltonian.
The energy spectrum and the suppression of the leakage-inducing S-mixing render
the Cr7Ni molecule a suitable candidate for the qubit implementation, as
further substantiated by our quantum-gate simulations.Comment: To appear in Physical Review Letter
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