Continuous monitoring of the boundary-layer top with lidar

International audienceContinuous lidar observations of the top height of the boundary layer (BL top) have been performed at Leipzig (51.3° N, 12.4° E), Germany, since August 2005. The results of measurements taken with a compact, automated Raman lidar over a one-year period (February 2006 to January 2007) are presented. Four different methods for the determination of the BL top are discussed. The most promising technique, the wavelet covariance algorithm, is improved by implementing some modifications so that an automated, robust retrieval of BL depths from lidar data is possible. Three case studies of simultaneous observations with the Raman lidar, a vertical-wind Doppler lidar, and accompanying radiosonde profiling of temperature and humidity are discussed to demonstrate the potential and the limits of the four lidar techniques at different aerosol and meteorological conditions. The lidar-derived BL top heights are compared with respective values derived from predictions of the regional weather forecast model COSMO of the German Meteorological Service. The comparison shows a general underestimation of the BL top by about 20% by the model. The statistical analysis of the one-year data set reveals that the seasonal mean of the daytime maximum BL top is 1400 m in spring, 1800 m in summer, 1200 m in autumn, and 800 m in winter at the continental, central European site. BL top typically increases by 100?300 m per hour in the morning of convective days

Radiative effect of aerosols above the northern and southern Atlantic Ocean as determined from shipborne lidar observations

The direct solar radiative effect of aerosols over the Atlantic Ocean was investigated on the basis of aerosol Raman/polarization lidar observations aboard the research vessel Polarsternbetween Germany (50°N) and either South America (50°S) or South Africa (40°S) in 2009 and 2010. First, a case study of complex aerosol conditions with marine aerosol, dust, and smoke particles in the boundary layer and free troposphere is presented to demonstrate that detailed knowledge of aerosol layering (boundary layer, free troposphere) and aerosol mixing state is required for an accurate determination of the resulting radiative effects. A statistical analysis based on all lidar observations revealed the highest daily mean radiative effect (−43±59 W m−2at the surface, −14±18 W m−2at top of atmosphere) in the latitudinal belt from 0°N–15°N in the Saharan dust outflow region. Mean aerosol radiative effects of the polluted northern and clean southern midlatitudes were contrasted. In the northern midlatitudes, the averaged aerosol radiative effect of all simulations was −24±33 W m−2at the surface which is a factor of 1.6 higher than at similar southern hemispheric latitudes. The simulations based on the lidar observations are in good agreement with colocated pyranometer measurements

1064 nm rotational Raman lidar for particle extinction and lidar-ratio profiling: cirrus case study

For the first time, vertical profiles of the 1064 nm particle extinction coefficient obtained from Raman lidar observations at 1058 nm (nitrogen and oxygen rotational Raman backscatter) are presented. We applied the new technique in the framework of test measurements and performed several cirrus observations of particle backscatter and extinction coefficients, and corresponding extinction-to-backscatter ratios at the wavelengths of 355, 532, and 1064 nm. The cirrus backscatter coefficients were found to be equal for all three wavelengths keeping the retrieval uncertainties in mind. The multiple-scattering-corrected cirrus extinction coefficients at 355 nm were on average about 20–30 % lower than the ones for 532 and 1064 nm. The cirrus-mean extinction-to-backscatter ratio (lidar ratio) was 31 ± 5 sr (355 nm), 36 ± 5 sr (532 nm), and 38 ± 5 sr (1064 nm) in this single study. We further discussed the requirements needed to obtain aerosol extinction profiles in the lower troposphere at 1064 nm with good accuracy (20 % relative uncertainty) and appropriate temporal and vertical resolution

Depolarization and lidar ratios at 355, 532, and 1064 nm and microphysical properties of aged tropospheric and stratospheric Canadian wildfire smoke

We present spectrally resolved optical and microphysical properties of western Canadian wildfire smoke observed in a tropospheric layer from 5-6.5 km height and in a stratospheric layer from 15-16 km height during a recordbreaking smoke event on 22 August 2017. Three polarization/ Raman lidars were run at the European Aerosol Research Lidar Network (EARLINET) station of Leipzig, Germany, after sunset on 22 August. For the first time, the linear depolarization ratio and extinction-to-backscatter ratio (lidar ratio) of aged smoke particles were measured at all three important lidar wavelengths of 355, 532, and 1064 nm. Very different particle depolarization ratios were found in the troposphere and in the stratosphere. The obviously compact and spherical tropospheric smoke particles caused almost no depolarization of backscattered laser radiation at all three wavelengths ( 500nm). The stratospheric smoke particles formed a pronounced accumulation mode (in terms of particle volume or mass) centered at a particle radius of 350-400 nm. The effective particle radius was 0.32 μm. The tropospheric smoke particles were much smaller (effective radius of 0.17 μm). Mass concentrations were of the order of 5.5 μgm-3 (tropospheric layer) and 40 μgm-3 (stratospheric layer) in the night of 22 August 2017. The single scattering albedo of the stratospheric particles was estimated to be 0.74, 0.8, and 0.83 at 355, 532, and 1064 nm, respectively

Adaption of the MODIS aerosol retrieval algorithm using airborne spectral surface reflectance measurements over urban areas: A case study

MODIS (MOderate-resolution Imaging Spectroradiometer) retrievals of aerosol optical depth (AOD) are biased over urban areas, primarily because the reflectance characteristics of urban surfaces are different than that assumed by the retrieval algorithm. Specifically, the operational "dark-target" retrieval is tuned towards vegetated (dark) surfaces and assumes a spectral relationship to estimate the surface reflectance in blue and red wavelengths. From airborne measurements of surface reflectance over the city of Zhongshan, China, were collected that could replace the assumptions within the MODIS retrieval algorithm. The subsequent impact was tested upon two versions of the operational algorithm, Collections 5 and 6 (C5 and C6). AOD retrieval results of the operational and modified algorithms were compared for a specific case study over Zhongshan to show minor differences between them all. However, the Zhongshan-based spectral surface relationship was applied to a much larger urban sample, specifically to the MODIS data taken over Beijing between 2010 and 2014. These results were compared directly to ground-based AERONET (AErosol RObotic NETwork) measurements of AOD. A significant reduction of the differences between the AOD retrieved by the modified algorithms and AERONET was found, whereby the mean difference decreased from 0.27±0.14 for the operational C5 and 0.19±0.12 for the operational C6 to 0.10±0.15 and -0.02±0.17 by using the modified C5 and C6 retrievals. Since the modified algorithms assume a higher contribution by the surface to the total measured reflectance from MODIS, consequently the overestimation of AOD by the operational methods is reduced. Furthermore, the sensitivity of the MODIS AOD retrieval with respect to different surface types was investigated. Radiative transfer simulations were performed to model reflectances at top of atmosphere for predefined aerosol properties. The reflectance data were used as input for the retrieval methods. It was shown that the operational MODIS AOD retrieval over land reproduces the AOD reference input of 0.85 for dark surface types (retrieved AOD = 0.87 (C5)). An overestimation of AOD = 0.99 is found for urban surfaces, whereas the modified C5 algorithm shows a good performance with a retrieved value of AOD = 0.86

Continuous vertical aerosol profiling with a multi-wavelength Raman polarization lidar over the Pearl River Delta, China

A dataset of particle optical properties of the highly polluted atmosphere over the Pearl River Delta (PRD), Guangzhou, China, is presented in this paper. The data were derived from the measurements of a multi-wavelength Raman and depolarization lidar PollyXT and a co-located AERONET sun photometer. The measurement campaign was conducted from November 2011 to mid-June 2012. These are the first Raman lidar measurements in the PRD that lasted for several months. A mean value of aerosol optical depth (AOD) of 0.54 ± 0.33 was observed by the sun photometer at 500 nm in the polluted atmosphere over this megacity for the whole measurement period. The lidar profiles frequently show lofted aerosol layers, which reach altitudes of up to 2 to 3 km and, especially during the spring season, up to 5 km. These layers contain between 12 and 56 % of the total AOD, with the highest values in spring. The aerosol types in these lofted layers are classified by their optical properties. The observed lidar ratio values range from 30 to 80 sr with a mean value of 48.0 ± 10.7 sr at 532 nm. The linear particle depolarization ratio at 532 nm lies mostly below 5 %, with a mean value of 3.6 ± 3.7 %. The majority of the Ångström exponents lie between 0.5 and 1.5, indicating a mixture of fine- and coarse-mode aerosols. These results reveal that mostly urban pollution particles mixed with particles produced from biomass and industrial burning are present in the atmosphere above the Pearl River Delta. Trajectory analyses show that these pollution mixtures arise mainly from local and regional sources

Surface matters: Limitations of CALIPSO V3 aerosol typing in coastal regions

In the CALIPSO data analysis, surface type (land/ocean) is used to augment the aerosol characterization. However, this surface-dependent aerosol typing prohibits a correct classification of marine aerosol over land that is advected from ocean to land. This might result in a systematic overestimation of the particle extinction coefficient and of the aerosol optical thickness (AOT) of up to a factor of 3.5 over land in coastal areas. We present a long-term comparison of CALIPSO and ground-based lidar observations of the aerosol conditions in the coastal environment of southern South America (Punta Arenas, Chile, 53° S), performed in December 2009–April 2010. Punta Arenas is almost entirely influenced by marine particles throughout the year, indicated by a rather low AOT of 0.02–0.04. However, we found an unexpectedly high fraction of continental aerosol in the aerosol types inferred by means of CALIOP observations and, correspondingly, too high values of particle extinction. Similar features of the CALIOP data analysis are presented for four other coastal areas around the world. Since CALIOP data serve as important input for global climate models, the influence of this systematic error was estimated by means of simplified radiative-transfer calculations

Numerical simulations of optical properties of Saharan dust aerosols with emphasis on lidar applications

In the framework of the Saharan Mineral Dust Experiment (SAMUM) for the first time the spectral dependence of particle linear depolarization ratios was measured by combining four lidar systems. In this paper these measurements are compared with results from scattering theory based on the T-matrix method. For this purpose, in situ measurements—size distribution, shape distribution and refractive index—were used as input parameters; particle shape was approximated by spheroids. A sensitivity study showed that lidar-related parameters—lidar ratio Sp and linear depolarization ratio δp—are very sensitive to changes of all parameters. The simulated values of the δp are in the range of 20% and 31% and thus in the range of the measurements. The spectral dependence is weak, so that it could not be resolved by the measurements. Calculated lidar ratios based on the measured microphysics and considering equivalent radii up to 7.5μm show a range of possible values between 29 and 50 sr at λ = 532 nm. Larger Sp might be possible if the real part of the refractive index is small and the imaginary part is large. A strict validation was however not possible as too many microphysical parameters influence Sp and δp that could not be measured with the required accuracy

Spectral surface albedo over Morocco and its impact on radiative forcing of Saharan dust

In May-June 2006, airborne and ground-based solar (0.3-2.2 μm) and thermal infrared (4-42 μm) radiation measurements have been performed in Morocco within the Saharan Mineral Dust Experiment (SAMUM). Upwelling and downwelling solar irradiances have been measured using the Spectral Modular Airborne Radiation Measurement System (SMART)-Albedometer. With these data, the areal spectral surface albedo for typical surface types in southeastern Morocco was derived from airborne measurements for the first time. The results are compared to the surface albedo retrieved from collocated satellite measurements, and partly considerable deviations are observed. Using measured surface and atmospheric properties, the spectral and broad-band dust radiative forcing at top-of-atmosphere (TOA) and at the surface has been estimated. The impact of the surface albedo on the solar radiative forcing of Saharan dust is quantified. In the SAMUM case of 19 May 2006, TOA solar radiative forcing varies by 12 W m-2 per 0.1 surface-albedo change. For the thermal infrared component, values of up to +22 W m-2 were derived. The net (solar plus thermal infrared) TOA radiative forcing varies between -19 and +24 W m-2 for a broad-band solar surface albedo of 0.0 and 0.32, respectively. Over the bright surface of southeastern Morocco, the Saharan dust always has a net warming effect. © 2008 The Author Journal compilation © 2008 Blackwell Munksgaard

New-particle formation events in a continental boundary layer: first results from the SATURN experiment

International audienceDuring the SATURN experiment, which took place from 27 May to 14 June 2002, new particle formation in the continental boundary layer was investigated. Simultaneous ground-based and tethered-balloon-borne measurements were performed, including meteorological parameters, particle number concentrations and size distributions, gaseous precursor concentrations and SODAR and LIDAR observations. Newly formed particles were observed inside the residual layer, before the break-up process of the nocturnal inversion, and inside the mixing layer throughout the break-up of the nocturnal inversion and during the evolution of the planetary boundary layer.</p