Mirrorless Negative-index Parametric Micro-oscillator

The feasibility and extraordinary properties of mirrorless parametric oscillations in strongly absorbing negative-index metamaterials are shown. They stem from the backwardness of electromagnetic waves inherent to this type of metamaterials.Comment: 4 pages, 2 figure

Dislocations in stacking and commensurate-incommensurate phase transition in bilayer graphene and hexagonal boron nitride

Dislocations corresponding to a change of stacking in two-dimensional hexagonal bilayers, graphene and boron nitride, and associated with boundaries between commensurate domains are investigated using the two-chain Frenkel-Kontorova model on top of ab initio calculations. Structural transformations of bilayers in which the bottom layer is stretched and the upper one is left to relax freely are considered for gradually increased elongation of the bottom layer. Formation energies of dislocations, dislocation width and orientation of the boundary between commensurate domains are analyzed depending on the magnitude and direction of elongation. The second-order phase transition from the commensurate phase to the incommensurate one with multiple dislocations is predicted to take place at some critical elongation. The order parameter for this transition corresponds to the density of dislocations, which grows continuously upon increasing the elongation of the bottom layer above the critical value. In graphene and metastable boron nitride with the layers aligned in the same direction, where elementary dislocations are partial, this transition, however, is preceded by formation of the first dislocation at the elongation smaller than the critical one. The phase diagrams including this intermediate state are plotted in coordinates of the magnitude and direction of elongation of the bottom layer.Comment: 15 pages, 9 figure

Comparison of performance of van der Waals-corrected exchange-correlation functionals for interlayer interaction in graphene and hexagonal boron nitride

Exchange-correlation functionals with corrections for van der Waals interactions (PBE-D2, PBE-D3, PBE-D3(BJ), PBE-TS, optPBE-vdW and vdW-DF2) are tested for graphene and hexagonal boron nitride, both in the form of bulk and bilayer. The characteristics of the potential energy surface, such as the barrier to relative sliding of the layers and magnitude of corrugation, and physically measurable properties associated with relative in-plane and out-of-plane motion of the layers including the shear modulus and modulus for axial compression, shear mode frequency and frequency of out-of-plane vibrations are considered. The PBE-D3(BJ) functional gives the best results for the stackings of hexagonal boron nitride and graphite that are known to be ground-state from the experimental studies. However, it fails to describe the order of metastable states of boron nitride in energy. The PBE-D3 and vdW-DF2 functionals, which reproduce this order correctly, are identified as the optimal choice for general studies. The vdW-DF2 functional is preferred for evaluation of the modulus for axial compression and frequency of out-of-plane vibrations, while the PBE-D3 functional is somewhat more accurate in calculations of the shear modulus and shear mode frequency. The best description of the latter properties, however, is achieved also using the vdW-DF2 functional combined with consideration of the experimental interlayer distance. In the specific case of graphene, the PBE-D2 functional works very well and can be further improved by adjustment of the parameters.Comment: 22 pages, 4 figue

Transformation of amorphous carbon clusters to fullerenes

Transformation of amorphous carbon clusters into fullerenes under high temperature is studied using molecular dynamics simulations at microsecond times. Based on the analysis of both structure and energy of the system, it is found that fullerene formation occurs in two stages. Firstly, fast transformation of the initial amorphous structure into a hollow sp$^2$ shell with a few chains attached occurs with a considerable decrease of the potential energy and the number of atoms belonging to chains and to the amorphous domain. Then, insertion of remaining carbon chains into the sp$^2$ network takes place at the same time with the fullerene shell formation. Two types of defects remaining after the formation of the fullerene shell are revealed: 7-membered rings and single one-coordinated atoms. One of the fullerene structures obtained contains no defects at all, which demonstrates that defect-free carbon cages can be occasionally formed from amorphous precursors directly without defect healing. No structural changes are observed after the fullerene formation, suggesting that defect healing is a slow process in comparison with the fullerene shell formation. The schemes of the revealed reactions of chain atoms insertion into the fullerene shell just before its completion are presented. The results of the performed simulations are summarized within the paradigm of fullerene formation due to selforganization of the carbon system.Comment: 35 pages, 9 figure

Four-wave mixing, quantum control and compensating losses in doped negative-index photonic metamaterials

The possibility of compensating absorption in negative-index metatamterials (NIMs) doped by resonant nonlinear-optical centers is shown. The role of quantum interference and extraordinary properties of four-wave parametric amplification of counter-propagating electromagnetic waves in NIMs are discussed.Comment: 3 pages, 3 figures, LaTeX, corrected typos in eqs. (1) and (2

Merging Nonlinear Optics and Negative-Index Metamaterials

The extraordinary properties of nonlinear optical propagation processes in double-domain positive/negative index metamaterials are reviewed. These processes include second harmonic generation, three- and four-wave frequency mixing, and optical parametric amplification. Striking contrasts with the properties of the counterparts in ordinary materials are shown. We also discuss the possibilities for compensating strong losses inherent to plasmonic metamaterials, which present a major obstacle in numerous exciting applications, and the possibilities for creation of unique ultracompact photonic devices such as data processing chips and nonlinear-optical sensors. Finally, we propose similar extraordinary three-wave mixing processes in crystals based on optical phonons with negative dispersion.Comment: A review paper, 27 pages, 16 figures, 81 reference

Explicit Non-Abelian Monopoles and Instantons in SU(N) Pure Yang-Mills Theory

It is well known that there are no static non-Abelian monopole solutions in pure Yang-Mills theory on Minkowski space R^{3,1}. We show that such solutions exist in SU(N) gauge theory on the spaces R^2\times S^2 and R^1\times S^1\times S^2 with Minkowski signature (-+++). In the temporal gauge they are solutions of pure Yang-Mills theory on T^1\times S^2, where T^1 is R^1 or S^1. Namely, imposing SO(3)-invariance and some reality conditions, we consistently reduce the Yang-Mills model on the above spaces to a non-Abelian analog of the \phi^4 kink model whose static solutions give SU(N) monopole (-antimonopole) configurations on the space R^{1,1}\times S^2 via the above-mentioned correspondence. These solutions can also be considered as instanton configurations of Yang-Mills theory in 2+1 dimensions. The kink model on R^1\times S^1 admits also periodic sphaleron-type solutions describing chains of n kink-antikink pairs spaced around the circle S^1 with arbitrary n>0. They correspond to chains of n static monopole-antimonopole pairs on the space R^1\times S^1\times S^2 which can also be interpreted as instanton configurations in 2+1 dimensional pure Yang-Mills theory at finite temperature (thermal time circle). We also describe similar solutions in Euclidean SU(N) gauge theory on S^1\times S^3 interpreted as chains of n instanton-antiinstanton pairs.Comment: 16 pages; v2: subsection on topological charges added, title expanded, some coefficients corrected, version to appear in PR

Enhanced four-wave mixing via elimination of inhomogeneous broadening by coherent driving of quantum transition with control fields

We show that atoms from wide velocity interval can be concurrently involved in Doppler-free two-photon resonant far from frequency degenerate four-wave mixing with the aid of auxiliary electromagnetic field. This gives rise to substantial enhancement of the output radiation generated in optically thick medium. Numerical illustrations addressed to typical experimental conditions are given.Comment: LaTeX2e, hyperref, 7 pages, 5 figures, to appear in PRA 1 august 200