40 research outputs found
Resonant x-ray scattering reveals possible disappearance of magnetic order under hydrostatic pressure in the Kitaev candidate -LiIrO
Honeycomb iridates such as -LiIrO are argued to realize
Kitaev spin-anisotropic magnetic exchange, along with Heisenberg and possibly
other couplings. While systems with pure Kitaev interactions are candidates to
realize a quantum spin liquid ground state, in -LiIrO it has
been shown that the balance of magnetic interactions leads to the
incommensurate spiral spin order at ambient pressure below 38 K. We study the
fragility of this state in single crystals of -LiIrO using
resonant x-ray scattering (RXS) under applied hydrostatic pressures of up to
3.0 GPa. RXS is a direct probe of the underlying electronic order, and we
observe the abrupt disappearance of the =(0.57, 0, 0) spiral order at a
critical pressure GPa with no accompanying change in the symmetry
of the lattice. This dramatic disappearance is in stark contrast with recent
studies of -LiIrO that show continuous suppression of the spiral
order in magnetic field; under pressure, a new and possibly nonmagnetic ground
state emerges
Local orthorhombicity in the magnetic phase of the hole-doped iron-arsenide superconductor SrNaFeAs
We report temperature-dependent pair distribution function measurements of
SrNaFeAs, an iron-based superconductor system that
contains a magnetic phase with reentrant tetragonal symmetry, known as the
magnetic phase. Quantitative refinements indicate that the instantaneous
local structure in the phase is comprised of fluctuating orthorhombic
regions with a length scale of 2 nm, despite the tetragonal symmetry of
the average static structure. Additionally, local orthorhombic fluctuations
exist on a similar length scale at temperatures well into the paramagnetic
tetragonal phase. These results highlight the exceptionally large nematic
susceptibility of iron-based superconductors and have significant implications
for the magnetic phase and the neighboring and superconducting
phases
Disentangling transport mechanisms in a correlated oxide by photoinduced charge injection
We present a novel heterostructured approach to disentangle the mechanism of
electrical transport of the strongly correlated PrNiO3, by placing the
nickelate under the photoconductor CdS. This enables the injection of carriers
into PrNiO3 in a controlled way, which can be used to interrogate its intrinsic
transport mechanism. We find a non-volatile resistance decrease when
illuminating the system at temperatures below the PrNiO3 metal-insulator
transition. The photoinduced change becomes more volatile as the temperature
increases. These data help understand the intrinsic transport properties of the
nickelate-CdS bilayer. Together with data from a bare PrNiO3 film, we find that
the transport mechanism includes a combination of mechanisms including both
thermal activation and variable range hopping. At low temperatures without
photoinduced carriers the transport is governed by hopping, while at higher
temperatures and intense illumination the activation mechanism becomes
relevant. This work shows a new way to optically control the low-temperature
resistance of PrNiO3
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Local strain inhomogeneities during electrical triggering of a metal-insulator transition revealed by X-ray microscopy.
Electrical triggering of a metal-insulator transition (MIT) often results in the formation of characteristic spatial patterns such as a metallic filament percolating through an insulating matrix or an insulating barrier splitting a conducting matrix. When MIT triggering is driven by electrothermal effects, the temperature of the filament or barrier can be substantially higher than the rest of the material. Using X-ray microdiffraction and dark-field X-ray microscopy, we show that electrothermal MIT triggering leads to the development of an inhomogeneous strain profile across the switching device, even when the material does not undergo a pronounced, discontinuous structural transition coinciding with the MIT. Diffraction measurements further reveal evidence of unique features associated with MIT triggering including lattice distortions, tilting, and twinning, which indicate structural nonuniformity of both low- and high-resistance regions inside the switching device. Such lattice deformations do not occur under equilibrium, zero-voltage conditions, highlighting the qualitative difference between states achieved through increasing temperature and applying voltage in nonlinear electrothermal materials. Electrically induced strain, lattice distortions, and twinning could have important contributions in the MIT triggering process and drive the material into nonequilibrium states, providing an unconventional pathway to explore the phase space in strongly correlated electronic systems
Short-range nematic fluctuations in Sr1-xNaxFe2As2 superconductors
Interactions between nematic fluctuations, magnetic order and
superconductivity are central to the physics of iron-based superconductors.
Here we report on in-plane transverse acoustic phonons in hole-doped
SrNaFeAs measured via inelastic X-ray scattering, and
extract both the nematic susceptibility and the nematic correlation length. By
a self-contained method of analysis, for the underdoped () sample,
which harbors a magnetically-ordered tetragonal phase, we find it hosts a short
nematic correlation length ~ 10 and a large nematic susceptibility
. The optimal-doped () sample exhibits weaker phonon
softening effects, indicative of both reduced and . Our
results suggest short-range nematic fluctuations may favor superconductivity,
placing emphasis on the nematic correlation length for understanding the
iron-based superconductors
Discovery of Charge Order in the Transition Metal Dichalcogenide FeNbS
The Fe intercalated transition metal dichalcogenide (TMD), FeNbS,
exhibits remarkable resistance switching properties and highly tunable spin
ordering phases due to magnetic defects. We conduct synchrotron X-ray
scattering measurements on both under-intercalated ( = 0.32) and
over-intercalated ( = 0.35) samples. We discover a new charge order phase in
the over-intercalated sample, where the excess Fe atoms lead to a zigzag
antiferromagnetic order. The agreement between the charge and magnetic ordering
temperatures, as well as their intensity relationship, suggests a strong
magnetoelastic coupling as the mechanism for the charge ordering. Our results
reveal the first example of a charge order phase among the intercalated TMD
family and demonstrate the ability to stabilize charge modulation by
introducing electronic correlations, where the charge order is absent in bulk
2H-NbS compared to other pristine TMDs