322 research outputs found
Cr-doping effect on the orbital fluctuation of heavily doped Nd1-xSrxMnO3 (x ~ 0.625)
We have investigated the Cr-doping effect of Nd0.375Sr0.625MnO3 near the
phase boundary between the x2-y2 and 3z2-r2 orbital ordered states, where a
ferromagnetic correlation and concomitant large magnetoresistance are observed
owing to orbital fluctuation. Cr-doping steeply suppresses the ferromagnetic
correlation and magnetoresistance in Nd0.375Sr0.625Mn1-yCryO3 with 0 < y <
0.05, while they reappear in 0.05 < y < 0.10. Such a reentrant behavior implies
that a phase boundary is located at y = 0.05, or a phase crossover occurs
across y = 0.05.Comment: 3 pages, 3 figures, to be published in Journal of Applied Physic
Electron- and Hole-Doping Effects on -site Ordered NdBaMnO
We have investigated electron- and hole-doping effects on -site ordered
perovskite manganite NdBaMnO, which has the -type (layered)
antiferromagnetic (AFM) ground state. Electrons (holes) are introduced by
partial substitution of Ba (Nd) with Nd (Ba).
Electron-doping generates ferromagnetic (FM) clusters in the -type AFM
matrix. With increasing the electron-doping level, the volume fraction of the
FM phase or the number of the FM clusters is abruptly increasing. In contrast,
the -type AFM phase is robust against the hole-doping, and no FM correlation
is observed in the hole-doped NdBaMnO.Comment: 8 pages, 5 figures, to be published in Journal of the Physical
Society of Japa
Enhancement of the anomalous Hall effect and spin glass behavior in the bilayered manganite La(2-2x)Sr(1+2x)Mn2O7
The Hall resistivity and magnetization have been investigated in the
ferromagnetic state of the bilayered manganite La(2-2x)Sr(1+2x)Mn2O7 (x=0.36).
The Hall resistivity shows an increase in both the ordinary and anomalous Hall
coefficients at low temperatures below 50K, a region in which experimental
evidence for the spin glass state has been found in a low magnetic field of
1mT. The origin of the anomalous behavior of the Hall resistivity relevant to
magnetic states may lie in the intrinsic microscopic inhomogeneity in a
quasi-two-dimensional electron system.Comment: 7 pages, 4 figures, Solid State Communications (in press
Magnetic Structures of High Temperature Phases of TbBaCo2O5.5
Neutron diffraction studies have been carried out on a single crystal of
oxygen-deficient perovskite TbBaCo2O5.5 in the temperature range of 7-370 K.
There have been observed several magnetic or structural transitions. Among
these, the existence of the transitions to the insulating phase from the
metallic one at ~340 K, to the one with the ferromagnetic moment at ~280 K and
possibly to the antiferromagnetic one at ~260 K, with decreasing temperature T
correspond to those reported in former works. We have studied the magnetic
structures at 270 K and 250 K and found that all Co3+ ions of the CoO6
octahedra are in the low spin state and those of the CoO5 pyramids carry spins
which are possibly in the intermediate spin state. Non-collinear magnetic
structures are proposed at these temperatures. Two other transitions have also
been observed at the temperatures, ~100 K and ~250 K.Comment: 9 pages, 2 tables, 10 figure
A-site Randomness Effect on Structural and Physical Properties of Ba-based Perovskite Manganites
The discovery of novel structural and physical properties in the -site
ordered manganite BaMnO ( = Y and rare earth elements) has
demanded new comprehension about perovskite manganese oxides. In the present
study, the -site disordered form, BaMnO, has been
investigated and compared with both BaMnO and
MnO (: Sr, Ca) in the structures and electromagnetic
properties. BaMnO has a primitive cubic perovskite cell
in the structure and magnetic glassy states are dominant as its ground state,
in contrast to the ordinary disordered MnO (: Sr, Ca).
In Pr-compounds with various degrees of Pr/Ba randomness at the -sites, the
-site disorder gradually suppresses both ferromagnetic and A-type
antiferromagnetic transitions and finally leads to a magnetic glassy state in
PrBaMnO. A peculiar behavior, multi-step magnetization
and resistivity change, has been observed in PrBaMnO.
These properties could be closely related to any spatial heterogeneity caused
by the random distribution of Ba and with much different
ionic radius.Comment: 9 pages, to be published in J. Phys. Soc. Jpn. 73 Aug. (2004
Endoscopic Management of Gastric Polyp with Outlet Obstruction without Polypectomy
Although gastric polyp is usually an incidental endoscopic finding, large-sized polyps can cause symptoms ranging from epigastralgia to bleeding from ulcerated polyps and gastric outlet obstruction. Although the gold standard of treatment is removal of the polyp either through endoscopic polypectomy or surgical excision, complications associated with these procedures cannot be ignored. The risk becomes a major concern for patients at high risk for surgery when complications arise. We describe a debilitated 74-year-old woman who presented with early satiety, intermittent postprandial nausea and vomiting for three months. Upper endoscopy revealed a 2.5 cm pedunculated polyp over the gastric antrum causing intermittent obstruction. Considering her high risk for polypectomy, detachable snaring was performed without polypectomy in an outpatient setting. The patient was complication-free with complete relief of obstructive symptoms one week after the procedure. Subsequent follow-ups showed satisfactory healing without signs of mucosal disruption or recurrence. The results suggest that detachable snaring without polypectomy may be a therapeutic option for high-risk patients with benign symptomatic gastric polyps
Transport and Magnetic Properties of R1-xAxCoO3 (R=La, Pr and Nd; A=Ba, Sr and Ca)
Transport and magnetic measurements have been carried out on perovskite
Co-oxides R1-xAxCoO3 (R=La, Pr, and Nd; A=Ba, Sr and Ca; 0<x<0.5: All sets of
the R and A species except Nd1-xBaxCoO3 have been studied.). With increasing
the Sr- or Ba-concentration x, the system becomes metallic ferromagnet with
rather large magnetic moments. For R=Pr and Nd and A=Ca, the system approaches
the metal- insulator phase boundary but does not become metallic. The magnetic
moments of the Ca-doped systems measured with the magnetic field H=0.1 T are
much smaller than those of the Ba- and Sr-doped systems. The thermoelectric
powers of the Ba- and Sr-doped systems decrease from large positive values of
lightly doped samples to negative ones with increasing doping level, while
those of Ca-doped systems remain positive. These results can be understood by
considering the relationship between the average ionic radius of R1-xAx and the
energy difference between the low spin and intermediate spin states. We have
found the resistivity-anomaly in the measurements of Pr1-xCaxCoO3 under
pressure in the wide region of x, which indicates the existence of a phase
transition different from the one reported in the very restricted region of
x~0.5 at ambient pressure [Tsubouchi et al. Phys. Rev. B 66 (2002) 052418.]. No
indication of this kind of transition has been observed in other species of R.Comment: 9 pages, 8 figures. J. Phys. Soc. Jpn. 72 (2003) No.
Experimentação no Ensino de QuÃmica e na Divulgação CientÃfica – Propostas do GEPEQ-IQUSP em materiais produzidos coletivamente.
Perturbative calculation of the spin-wave dispersion in a disordered double-exchange model
We study the spin-wave dispersion of localized spins in a disordered
double-exchange model using the perturbation theory with respect to the
strength of the disorder potential. We calculate the dispersion upto the
next-leading order, and extensively examine the case of one-dimension. We show
that in that case, disorder yields anomalous gapped-like behavior at the Fermi
wavenumber of the conduction electrons.Comment: 9 pages, 5 figure
The nanoscale phase separation in hole-doped manganites
A macroscopic phase separation, in which ferromagnetic clusters are observed
in an insulating matrix, is sometimes observed, and believed to be essential to
the colossal magnetoresistive (CMR) properties of manganese oxides. The
application of a magnetic field may indeed trigger large magnetoresistance
effects due to the percolation between clusters allowing the movement of the
charge carriers. However, this macroscopic phase separation is mainly related
to extrinsic defects or impurities, which hinder the long-ranged charge-orbital
order of the system. We show in the present article that rather than the
macroscopic phase separation, an homogeneous short-ranged charge-orbital order
accompanied by a spin glass state occurs, as an intrinsic result of the
uniformity of the random potential perturbation induced by the solid solution
of the cations on the -sites of the structure of these materials. Hence the
phase separation does occur, but in a more subtle and interesting nanoscopic
form, here referred as ``homogeneous''. Remarkably, this ``nanoscale phase
separation'' alone is able to bring forth the colossal magnetoresistance in the
perovskite manganites, and is potentially relevant to a wide variety of other
magnetic and/or electrical properties of manganites, as well as many other
transition metal oxides, in bulk or thin film form as we exemplify throughout
the article.Comment: jpsj2 TeX style (J. Phys. Soc. Jpn); 18 pages, 7 figure
- …