2,359 research outputs found
Direct correlation functions of the Widom-Rowlinson model
We calculate, through Monte Carlo numerical simulations, the partial total
and direct correlation functions of the three dimensional symmetric
Widom-Rowlinson mixture. We find that the differences between the partial
direct correlation functions from simulation and from the Percus-Yevick
approximation (calculated analytically by Ahn and Lebowitz) are well fitted by
Gaussians. We provide an analytical expression for the fit parameters as
function of the density. We also present Monte Carlo simulation data for the
direct correlation functions of a couple of non additive hard sphere systems to
discuss the modification induced by finite like diameters.Comment: 16 pages, 7 figure
Multimodal Speech Recognition for Language-Guided Embodied Agents
Benchmarks for language-guided embodied agents typically assume text-based
instructions, but deployed agents will encounter spoken instructions. While
Automatic Speech Recognition (ASR) models can bridge the input gap, erroneous
ASR transcripts can hurt the agents' ability to complete tasks. In this work,
we propose training a multimodal ASR model to reduce errors in transcribing
spoken instructions by considering the accompanying visual context. We train
our model on a dataset of spoken instructions, synthesized from the ALFRED task
completion dataset, where we simulate acoustic noise by systematically masking
spoken words. We find that utilizing visual observations facilitates masked
word recovery, with multimodal ASR models recovering up to 30% more masked
words than unimodal baselines. We also find that a text-trained embodied agent
successfully completes tasks more often by following transcribed instructions
from multimodal ASR models. github.com/Cylumn/embodied-multimodal-asrComment: 5 pages, 5 figures, 24th ISCA Interspeech Conference (INTERSPEECH
2023
Peierls Instability and Electron-Phonon Coupling in a One-dimensional Sodium Wire
We have studied Peierls instability in an atomically thin wire of sodium
atoms using first-principles density-functional methods. A Na wire has a stable
uniform linear structure over a range of inter-atomic distances. At smaller
inter-atomic distances it develops a zigzag distortion. At larger inter-atomic
distances, just before breaking, a Na wire undergoes a very weak Peierls
dimerization. This behavior of a Na wire is understood in terms of its
electron-phonon coupling properties
Novel nanorod precipitate formation in neodymium and titanium codoped bismuth ferrite
The discovery of unusual nanorod precipitates in bismuth ferrite doped with Nd and Ti is reported. The atomic structure and chemistry of the nanorods are determined using a combination of high angle annular dark field imaging, electron energy loss spectroscopy, and density functional calculations. It is found that the structure of the BiFeO3 matrix is strongly modified adjacent to the precipitates; the readiness of BiFeO3 to adopt different structural allotropes in turn explains why such a large axial ratio, uncommon in precipitates, is stabilized. In addition, a correlation is found between the alignment of the rods and the orientation of ferroelastic domains in the matrix, which is consistent with the system's attempt to minimize its internal strain. Density functional calculations indicate a finite density of electronic states at the Fermi energy within the rods, suggesting enhanced electrical conductivity along the rod axes, and motivating future investigations of nanorod functionalities
Polaronic Signatures in Mid-Infrared Spectra: Prediction for LaMnO3 and CaMnO3
Hole-doped LaMnO3 and electron-doped CaMnO3 form self-trapped electronic
states. The spectra of these states have been calculated using a two orbital
(Mn eg Jahn-Teller) model, from which the non-adiabatic optical conductivity
spectra are obtained. In both cases the optical spectrum contains weight in the
gap region, whose observation will indicate the self-trapped nature of the
carrier states. The predicted spectra are proportional to the concentration of
the doped carriers in the dilute regime, with coefficients calculated with no
further model parameters.Comment: 6 pages with 3 figures imbedde
Cosmic-Ray Proton and Helium Spectra from the First CREAM Flight
Cosmic-ray proton and helium spectra have been measured with the
balloon-borne Cosmic Ray Energetics And Mass experiment flown for 42 days in
Antarctica in the 2004-2005 austral summer season. High-energy cosmic-ray data
were collected at an average altitude of ~38.5 km with an average atmospheric
overburden of ~3.9 g cm. Individual elements are clearly separated with
a charge resolution of ~0.15 e (in charge units) and ~0.2 e for protons and
helium nuclei, respectively. The measured spectra at the top of the atmosphere
are represented by power laws with a spectral index of -2.66 0.02 for
protons from 2.5 TeV to 250 TeV and -2.58 0.02 for helium nuclei from 630
GeV/nucleon to 63 TeV/nucleon. They are harder than previous measurements at a
few tens of GeV/nucleon. The helium flux is higher than that expected from the
extrapolation of the power law fitted to the lower-energy data. The relative
abundance of protons to helium nuclei is 9.1 0.5 for the range from 2.5
TeV/nucleon to 63 TeV/nucleon. This ratio is considerably smaller than the
previous measurements at a few tens of GeV/nucleon.Comment: 20 pages, 4 figure
Temperature Dependence of Low-Lying Electronic Excitations of LaMnO_3
We report on the optical properties of undoped single crystal LaMnO_3, the
parent compound of the colossal magneto-resistive manganites. Near-Normal
incidence reflectance measurements are reported in the frequency range of
20-50,000 cm-1 and in the temperature range 10-300 K. The optical conductivity,
s_1(w), is derived by performing a Kramers-Kronig analysis of the reflectance
data. The far-infrared spectrum of s_1(w) displays the infrared active optical
phonons. We observe a shift of several of the phonon to high frequencies as the
temperature is lowered through the Neel temperature of the sample (T_N = 137
K). The high-frequency s_1(w) is characterized by the onset of absorption near
1.5 eV. This energy has been identified as the threshold for optical
transitions across the Jahn-Teller split e_g levels. The spectral weight of
this feature increases in the low-temperature state. This implies a transfer of
spectral weight from the UV to the visible associated with the paramagnetic to
antiferromagnetic state. We discuss the results in terms of the double exchange
processes that affect the optical processes in this magnetic material.Comment: 7 pages, 5 figure
2-(4-Chlorobenzoyl)-3,6-dimethoxynaphthalene
In the title compound, C19H15ClO3, the interplanar angle between the naphthalene and benzene ring systems is 62.67 (6)°. The carbonyl group is twisted from both ring planes, with torsion angles of −44.9 (2)° with respect to the naphthalene ring and −26.7 (2)° with respect to the phenylene ring. There is an intermolecular hydrogen bond between an H atom of one methoxy group and the O atom of the second methoxy group, forming chains along the ac diagonal
MLT and seasonal dependence of auroral electrojets: IMAGE magnetometer network observations
Total eastward and westward electrojet currents (EEJ and WEJ) and their central latitudes derived from the International Monitor for Auroral Geomagnetic Effects (IMAGE) network magnetic measurements are analyzed for the combined MLT (magnetic local time) and seasonal dependence during the period 1995–2009. EEJ shows a strong MLT variation with significant dependence on season. During summer months the maxima occur around 1600–1800 MLT, whereas during winter months the maxima occur around 1800–2000 MLT. Moreover, the summer maxima are much larger than the winter maxima and appear at higher latitudes. The summer maxima are mainly associated with the solar EUV conductivity effect, while the winter maxima are mainly due to the contribution of northward convective electric field. EEJ exhibits a dominant annual variation with maximum in summer and minimum in winter. WEJ also exhibits a strong MLT variation with significant dependence on season. The maxima occur around 0200–0400 MLT during summer months, around 0000–0200 MLT during winter months, and around 0000–0400 MLT during equinoctial months. Moreover, the equinoctial maxima are much larger than the summer and winter maxima and appear at relatively lower latitudes. The seasonal variations in WEJ are the combinations of annual variations and semiannual variations. Both annual and semiannual variations show significant dependence on MLT. These results increase our knowledge on what factors contribute to the auroral electrojets as well as their magnetic signatures and hence help us better understand the limitations of global auroral electrojet indices, such as the AE and SME indices.Peer reviewe
Ultrafast quasiparticle relaxation dynamics in normal metals and heavy fermion materials
We present a detailed theoretical study of the ultrafast quasiparticle
relaxation dynamics observed in normal metals and heavy fermion materials with
femtosecond time-resolved optical pump-probe spectroscopy. For normal metals, a
nonthermal electron distribution gives rise to a temperature (T) independent
electron-phonon relaxation time at low temperatures, in contrast to the
T^{-3}-divergent behavior predicted by the two-temperature model. For heavy
fermion compounds, we find that the blocking of electron-phonon scattering for
heavy electrons within the density-of-states peak near the Fermi energy is
crucial to explain the rapid increase of the electron-phonon relaxation time
below the Kondo temperature. We propose the hypothesis that the slower Fermi
velocity compared to the sound velocity provides a natural blocking mechanism
due to energy and momentum conservation laws.Comment: 10 pages, 11 figure
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