1,392 research outputs found
Phonon quarticity induced by changes in phonon-tracked hybridization during lattice expansion and its stabilization of rutile TiO
Although the rutile structure of TiO is stable at high temperatures, the
conventional quasiharmonic approximation predicts that several acoustic phonons
decrease anomalously to zero frequency with thermal expansion, incorrectly
predicting a structural collapse at temperatures well below 1000\,K. Inelastic
neutron scattering was used to measure the temperature dependence of the phonon
density of states (DOS) of rutile TiO from 300 to 1373\,K. Surprisingly,
these anomalous acoustic phonons were found to increase in frequency with
temperature. First-principles calculations showed that with lattice expansion,
the potentials for the anomalous acoustic phonons transform from quadratic to
quartic, stabilizing the rutile phase at high temperatures. In these modes, the
vibrational displacements of adjacent Ti and O atoms cause variations in
hybridization of electrons of Ti and electrons of O atoms. With
thermal expansion, the energy variation in this "phonon-tracked hybridization"
flattens the bottom of the interatomic potential well between Ti and O atoms,
and induces a quarticity in the phonon potential.Comment: 7 pages, 6 figures, supplemental material (3 figures
Neutron Scattering Measurements of Spatially Anisotropic Magnetic Exchange Interactions in Semiconducting K0.85Fe1.54Se2 (TN=280 K)
We use neutron scattering to study the spin excitations associated with the
stripe antiferromagnetic (AFM) order in semiconducting
KFeSe (= K). We show that the spin wave spectra
can be accurately described by an effective Heisenberg Hamiltonian with highly
anisotropic in-plane couplings at = K. At high temperature (=
K) above , short range magnetic correlation with anisotropic correlation
lengths are observed. Our results suggest that, despite the dramatic difference
in the Fermi surface topology, the in-plane anisotropic magnetic couplings are
a fundamental property of the iron based compounds; this implies that their
antiferromagnetism may originate from local strong correlation effects rather
than weak coupling Fermi surface nesting.Comment: 5 pages, 4 figure
Higgs mode and its decay in a two dimensional antiferromagnet
Condensed-matter analogs of the Higgs boson in particle physics allow
insights into its behavior in different symmetries and dimensionalities.
Evidence for the Higgs mode has been reported in a number of different
settings, including ultracold atomic gases, disordered superconductors, and
dimerized quantum magnets. However, decay processes of the Higgs mode (which
are eminently important in particle physics) have not yet been studied in
condensed matter due to the lack of a suitable material system coupled to a
direct experimental probe. A quantitative understanding of these processes is
particularly important for low-dimensional systems where the Higgs mode decays
rapidly and has remained elusive to most experimental probes. Here, we discover
and study the Higgs mode in a two-dimensional antiferromagnet using
spin-polarized inelastic neutron scattering. Our spin-wave spectra of
CaRuO directly reveal a well-defined, dispersive Higgs mode, which
quickly decays into transverse Goldstone modes at the antiferromagnetic
ordering wavevector. Through a complete mapping of the transverse modes in the
reciprocal space, we uniquely specify the minimal model Hamiltonian and
describe the decay process. We thus establish a novel condensed matter platform
for research on the dynamics of the Higgs mode.Comment: original submitted version, Nature Physics (2017). arXiv admin note:
substantial text overlap with arXiv:1510.0701
Carrier-mediated ferromagnetic ordering in Mn ion-implanted p+GaAs:C
Highly p-type GaAs:C was ion-implanted with Mn at differing doses to produce
Mn concentrations in the 1 - 5 at.% range. In comparison to LT-GaAs and
n+GaAs:Si samples implanted under the same conditions, transport and magnetic
properties show marked differences. Transport measurements show anomalies,
consistent with observed magnetic properties and with epi- LT-(Ga,Mn)As, as
well as the extraordinary Hall Effect up to the observed magnetic ordering
temperature (T_C). Mn ion-implanted p+GaAs:C with as-grown carrier
concentrations > 10^20 cm^-3 show remanent magnetization up to 280 K
Magnetic excitations in underdoped Ba(Fe1-xCox)2As2 with x=0.047
The magnetic excitations in the paramagnetic-tetragonal phase of underdoped
Ba(Fe0.953Co0.047)2As2, as measured by inelastic neutron scattering, can be
well described by a phenomenological model with purely diffusive spin dynamics.
At low energies, the spectrum around the magnetic ordering vector Q_AFM
consists of a single peak with elliptical shape in momentum space. At high
energies, this inelastic peak is split into two peaks across the direction
perpendicular to Q_AFM. We use our fittings to argue that such a splitting is
not due to incommensurability or propagating spin-wave excitations, but is
rather a consequence of the anisotropies in the Landau damping and in the
magnetic correlation length, both of which are allowed by the tetragonal
symmetry of the system. We also measure the magnetic spectrum deep inside the
magnetically-ordered phase, and find that it is remarkably similar to the
spectrum of the paramagnetic phase, revealing the strongly overdamped character
of the magnetic excitations.Comment: 12 pages, 7 figure
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