569 research outputs found
Ground state properties of ferromagnetic metal/conjugated polymer interfaces
We theoretically investigate the ground state properties of ferromagnetic
metal/conjugated polymer interfaces. The work is partially motivated by recent
experiments in which injection of spin polarized electrons from ferromagnetic
contacts into thin films of conjugated polymers was reported. We use a
one-dimensional nondegenerate Su-Schrieffer-Heeger (SSH) Hamiltonian to
describe the conjugated polymer and one-dimensional tight-binding models to
describe the ferromagnetic metal. We consider both a model for a conventional
ferromagnetic metal, in which there are no explicit structural degrees of
freedom, and a model for a half-metallic ferromagnetic colossal
magnetoresistance (CMR) oxide which has explicit structural degrees of freedom.
The Fermi energy of the magnetic metallic contact is adjusted to control the
degree of electron transfer into the polymer. We investigate electron charge
and spin transfer from the ferromagnetic metal to the organic polymer, and
structural relaxation near the interface. Bipolarons are the lowest energy
charge state in the bulk polymer for the nondegenerate SSH model Hamiltonian.
As a result electrons (or holes) transferred into the bulk of the polymer form
spinless bipolarons. However, there can be spin density in the polymer
localized near the interface.Comment: 7 figure
Dynamical mean field theory for transition temperature and optics of CMR manganites
A tight binding parametrization of local spin density functional band theory
is combined with a dynamical mean field treatment of correlations to obtain a
theory of the magnetic transition temperature, optical conductivity and T=0
spinwave stiffness of a minimal model for the pseudocubic metallic
manganites such a . The results indicate that previous
estimates of obtained by one of us (Phys. Rev. \textbf{B61} 10738-49
(2000)) are in error, that in fact the materials are characterized by Hunds
coupling , and that magnetic-order driven changes in the
kinetic energy may not be the cause of the observed 'colossal' magnetoresistive
and multiphase behavior in the manganites, raising questions about our present
understanding of these materials.Comment: Published version; 10 pages, 9 figure
Parity Effects in Stacked Nanoscopic Quantum Rings
The ground state and the dielectric response of stacked quantum rings are
investigated in the presence of an applied magnetic field along the ring axis.
For odd number of rings and an electric field perpendicular to the axis, a
linear Stark effect occurs at distinct values of the magnetic field. At those
fields energy levels cross in the absence of electric field. For even values of
a quadratic Stark effect is expected in all cases, but the induced electric
polarization is discontinuous at those special magnetic fields. Experimental
consequences for related nanostructures are discussed.Comment: typos corrected, to appear Phys. Rev. B (Rapid Communication) 15 Au
Temperature Dependence of Low-Lying Electronic Excitations of LaMnO_3
We report on the optical properties of undoped single crystal LaMnO_3, the
parent compound of the colossal magneto-resistive manganites. Near-Normal
incidence reflectance measurements are reported in the frequency range of
20-50,000 cm-1 and in the temperature range 10-300 K. The optical conductivity,
s_1(w), is derived by performing a Kramers-Kronig analysis of the reflectance
data. The far-infrared spectrum of s_1(w) displays the infrared active optical
phonons. We observe a shift of several of the phonon to high frequencies as the
temperature is lowered through the Neel temperature of the sample (T_N = 137
K). The high-frequency s_1(w) is characterized by the onset of absorption near
1.5 eV. This energy has been identified as the threshold for optical
transitions across the Jahn-Teller split e_g levels. The spectral weight of
this feature increases in the low-temperature state. This implies a transfer of
spectral weight from the UV to the visible associated with the paramagnetic to
antiferromagnetic state. We discuss the results in terms of the double exchange
processes that affect the optical processes in this magnetic material.Comment: 7 pages, 5 figure
Polaronic Signatures in Mid-Infrared Spectra: Prediction for LaMnO3 and CaMnO3
Hole-doped LaMnO3 and electron-doped CaMnO3 form self-trapped electronic
states. The spectra of these states have been calculated using a two orbital
(Mn eg Jahn-Teller) model, from which the non-adiabatic optical conductivity
spectra are obtained. In both cases the optical spectrum contains weight in the
gap region, whose observation will indicate the self-trapped nature of the
carrier states. The predicted spectra are proportional to the concentration of
the doped carriers in the dilute regime, with coefficients calculated with no
further model parameters.Comment: 6 pages with 3 figures imbedde
Essential Role of the Cooperative Lattice Distortion in the Charge, Orbital and Spin Ordering in doped Manganites
The role of lattice distortion in the charge, orbital and spin ordering in
half doped manganites has been investigated. For fixed magnetic ordering, we
show that the cooperative lattice distortion stabilize the experimentally
observed ordering even when the strong on-site electronic correlation is taken
into account. Furthermore, without invoking the magnetic interactions, the
cooperative lattice distortion alone may lead to the correct charge and orbital
ordering including the charge stacking effect, and the magnetic ordering can be
the consequence of such a charge and orbital ordering. We propose that the
cooperative nature of the lattice distortion is essential to understand the
complicated charge, orbital and spin ordering observed in doped manganites.Comment: 5 pages,4 figure
Reversible Random Sequential Adsorption of Dimers on a Triangular Lattice
We report on simulations of reversible random sequential adsorption of dimers
on three different lattices: a one-dimensional lattice, a two-dimensional
triangular lattice, and a two-dimensional triangular lattice with the nearest
neighbors excluded. In addition to the adsorption of particles at a rate K+, we
allow particles to leave the surface at a rate K-. The results from the
one-dimensional lattice model agree with previous results for the continuous
parking lot model. In particular, the long-time behavior is dominated by
collective events involving two particles. We were able to directly confirm the
importance of two-particle events in the simple two-dimensional triangular
lattice. For the two-dimensional triangular lattice with the nearest neighbors
excluded, the observed dynamics are consistent with this picture. The
two-dimensional simulations were motivated by measurements of Ca++ binding to
Langmuir monolayers. The two cases were chosen to model the effects of changing
pH in the experimental system.Comment: 9 pages, 10 figure
Large and Unified Description of Quark and Lepton Mixing Matrices
We present a revised version of the so-called "yukawaon model", which was
proposed for the purpose of a unified description of the lepton mixing matrix
and the quark mixing matrix . It is assumed from a
phenomenological point of view that the neutrino Dirac mass matrix is
given with a somewhat different structure from the charged lepton mass matrix
, although was assumed in the previous model. As a result, the
revised model predicts a reasonable value with
keeping successful results for other parameters in as well as
and quark and lepton mass ratios.Comment: 13 pages, 3 figures, version accepted by EPJ
Optical Investigations of Charge Gap in Orbital Ordered La1/2Sr3/2MnO4
Temperature and polarization dependent electronic structure of La1/2Sr3/2MnO4
were investigated by optical conductivity analyses. With decreasing
temperature, for E//ab, a broad mid-infrared (MIR) peak of La1/2Sr3/2MnO4
becomes narrower and moves to the higher frequency, while that of
Nd1/2Sr3/2MnO4 nearly temperature independent. We showed that the MIR peak in
La1/2Sr3/2MnO4 originates from orbital ordering associated with CE-type
magnetic ordering and that the Jahn-Teller distortion has a significant
influence on the width and the position of the MIR peak.Comment: 10 pages, 4 figure
Electromagnetic Response of Layered Superconductors with Broken Lattice Inversion Symmetry
We investigate the macroscopic effects of charge density waves (CDW) and
superconductivity in layered superconducting systems with broken lattice
inversion symmetry (allowing for piezoelectricity) such as two dimensional (2D)
transition metal dichalcogenides (TMD). We work with the low temperature time
dependent Ginzburg-Landau theory and study the coupling of lattice distortions
and low energy CDW collective modes to the superconducting order parameter in
the presence of electromagnetic fields. We show that superconductivity and
piezoelectricity can coexist in these singular metals. Furthermore, our study
indicates the nature of the quantum phase transition between a commensurate CDW
phase and the stripe phase that has been observed as a function of applied
pressure.Comment: 9 pages, 1 figure. Final version. Accepted in Phys.Rev.
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