Ultrafast all-optical toggle writing of magnetic bits without relying on heat

While in accordance with Curie's principle, one would intuitively expect that symmetry of the cause has to be found in the symmetry of the effect, ultrafast excitation of matter is able to violate this principle. For instance, it is believed that heating alone, obviously not having the symmetry of a magnetic field, cannot result in a deterministic reversal of magnetization. However, if the heating is induced by a femtosecond laser pulse and thus ultrafast, it does facilitate toggle switching of magnetization between stable bit-states without any magnetic field at all. Here we show that the regime of ultrafast toggle switching can be also realized via a mechanism without relying on any heat. The obvious mismatch between symmetries of the cause and the response can thus be seen as a violation of Curie's principle. In particular, ultrafast laser excitation of iron-garnet with linearly polarized light modifies magnetic anisotropy and thus causes toggling magnetization between two stable bit states. In contrast to the laser-heat-induced magnetization reversal, this new regime of 'cold' toggle switching can be observed in ferrimagnets without the compensation point and in an exceptionally broad temperature range. The control of magnetic anisotropy required for the toggle switching is accompanied by lower dissipations, than in the mechanism of laser-induced-heating, but the dissipations and the switching-time are shown to be competing parameters.Comment: 11 pages, 6 figure

Nonlinear sub-switching regime of magnetization dynamics in photo-magnetic garnets

We analyze, both experimentally and numerically, the nonlinear regime of the photo-induced coherent magnetization dynamics in cobalt-doped yttrium iron garnet films. Photo-magnetic excitation with femtosecond laser pulses reveals a strongly nonlinear response of the spin subsystem with a significant increase of the effective Gilbert damping. By varying both laser fluence and the external magnetic field, we show that this nonlinearity originates in the anharmonicity of the magnetic energy landscape. We numerically map the parameter workspace for the nonlinear photo-induced spin dynamics below the photo-magnetic switching threshold. Corroborated by numerical simulations of the Landau-Lifshitz-Gilbert equation, our results highlight the key role of the cubic symmetry of the magnetic subsystem in reaching the nonlinear spin precession regime. These findings expand the fundamental understanding of laser-induced nonlinear spin dynamics as well as facilitate the development of applied photo-magnetism

Photoinduced magnetic linear dichroism in a YIG:Co film

The spectra of linear dichroism induced by magnetic field are observed in a cobalt-doped yttrium iron garnet (YIG:Co) film grown in the (001) plane. The linear dichroism spectra are highly sensitive to the orientation of the magnetic field. The spectrum measured with the magnetic field directed along the crystallographic axis [100] turned out to have a form identical to the spectrum of the "rigid" photoinduced linear dichroism, known from earlier experiments. The similarity of these spectra may be regarded a sevidence of the magnetic origin of the major part of the optical anisotropy induced by light with polarization E | | [100] in the nonmagnetized YIG:Co film

Magnetic properties of ultrathin Co(0001) films on vicinal Si(111) substrate

In the present work we report on magnetization reversal process, anisotropy and domain structures in ultrathin Au/Co(0001)/Au films deposited on vicinal Si(111) substrates. The measurements were performed using a magneto-optical Kerr effect based magnetometer, a polarizing optical microscope and a ferromagnetic resonance spectrometer. Co thickness induced spin-reorientation from out-of-plane into in-plane magnetization was studied. Changes of in-plane magnetic anisotropy symmetry were deduced from shapes of magneto-optical hysteresis loops and from analysis of angular dependences of the resonance field. The experimental data have been discussed taking into account both uniaxial out-of-plane anisotropy and step-induced uniaxial in-plane anisotropy. A preferential orientation of domain walls in 3ML thick Co films was observed. The finding is explained by the step-induced magnetic anisotropy

Study of ultrathin Pt/Co/Pt trilayers modified by nanosecond XUV pulses from laser-driven plasma source

We have studied the structural mechanisms responsible for the magnetic reorientation between in-plane and out-of-plane magnetization in the (25 nm Pt)/(3 and 10 nm Co)/(3 nm Pt) trilayer systems irradiated with nanosecond XUV pulses generated with laser-driven gas-puff target plasma source of a narrow continuous spectrum peaked at wavelength of 11 nm. The thickness of individual layers, their density, chemical composition and irradiation-induced lateral strain were deduced from symmetric and asymmetric X-ray diffraction (XRD) patterns, grazing-incidence X-ray reflectometry (GIXR), grazing incidence X-ray fluorescence (GIXRF), extended X-ray absorption fine structure (EXAFS) and transmission electron microscopy (TEM) measurements. In the as grown samples we found, that the Pt buffer layers are relaxed and that the layer interfaces are sharp. As a result of a quasi-uniform irradiation of the samples, the XRD, EXAFS, GIXR and GIXRF data reveal the formation of two distinct layers composed of Pt1-xCox alloys with different Co concentrations, dependent on the thickness of the as grown magnetic Co film but with similar ∼1% lateral tensile residual strain. For smaller exposure dose (lower number of accumulated pulses) only partial interdiffusion at the interfaces takes place with the formation of a tri-layer composed of Co-Pt alloy sandwiched between thinned Pt layers, as revealed by TEM. The structural modifications are accompanied by magnetization changes, evidenced by means of magneto-optical microscopy. The difference in magnetic properties of the irradiated samples can be related to their modification in Pt1-xCox alloy composition, as the other parameters (lateral strain and alloy thickness) remain almost unchanged. The out-of-plane magnetization observed for the sample with initially 3 nm Co layer can be due to a significant reduction of demagnetization factor resulting from a lower Co concentration

Interface magnetic and optical anisotropy of ultrathin Co films grown on a vicinal Si substrate

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Three-Dimensional Micromagnetic Simulation of Spatial Distribution of Magnetization in Thick Cobalt Layers

Spatial magnetization distribution of cobalt layer is studied by means of three-dimensional micromagnetic simulations in the range of cobalt thickness d from 21 to 249 nm. In this range, a spin-reorientation phase transition occurs, while the cobalt thickness increases, from a state with in-plane magnetization, to a state with out-of-plane components of magnetization. An infinite cobalt layer is modelled by the 750 nm × 750 nm × d structure consisting of cubic cells of size of 3 nm and the periodic boundary conditions. For larger thicknesses, a labyrinth, partially closed, stripe structure has been found

Tunable magnetic properties in ultrathin co/garnet heterostructures

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