2,330 research outputs found
Nutation versus angular dependent NQR spectroscopy and the impact of underdoping on charge inhomogeneities in YBaCuO
We describe two different nuclear quadrupole resonance (NQR) based
techniques, designed to measure the local asymmetry of the internal electric
field gradient, and the tilt angle of the main NQR principal axis z from the
crystallographic axis c. These techniques use the dependence of the NQR signal
on the duration of the radio frequency (rf) pulse and on the direction of the
rf field H1 with respect to the crystal axis. The techniques are applied to
oriented powder of YBaCuO fully enriched with 63Cu.
Measurements were performed at different frequencies, corresponding to
different in-plane copper sites with respect to the dopant. Combining the
results from both techniques, we conclude that oxygen deficiency in the chain
layer lead to a rotation of the NQR main principal axis at the nearby Cu on the
CuO2 planes by 20+-degrees. This occurs with no change to the asymmetry. The
axis rotation associated with oxygen deficiency means that there must be
electric field inhomogeneities in the CuO2 planes only in the vicinity of the
missing oxygen.Comment: 9 pages, 10 figure
The Herbertsmithite Hamiltonian: SR measurements on single crystals
We present transverse field muon spin rotation/relaxation measurements on
single crystals of the spin-1/2 kagome antiferromagnet Herbertsmithite. We find
that the spins are more easily polarized when the field is perpendicular to the
kagome plane. We demonstrate that the difference in magnetization between the
different directions cannot be accounted for by Dzyaloshinksii-Moriya type
interactions alone, and that anisotropic axial interaction is present.Comment: 8 pages, 3 figures, accepted to JPCM special issue on geometrically
frustrated magnetis
Ga NMR study of the local susceptibility in SrCr8Ga4O19: pseudogap and paramagnetic defects
We present the first Ga(4f) NMR study of the Cr susceptibility in the
archetype of Kagome based frustrated antiferromagnets,
SrCrGaO. Our major finding is that the susceptibility of the
frustrated lattice goes through a maximum around 50 K. Our data also supports
the existence of paramagnetic ``clusters'' of spins, responsible for the Curie
behavior observed in the macroscopic susceptibility at low T. These results set
novel features for the constantly debated physics of geometrically frustrated
magnets.Comment: 4 pages, 5 figures Submitted to Phys. Rev. Let
Spin Echo Decay in a Stochastic Field Environment
We derive a general formalism with which it is possible to obtain the time
dependence of the echo size for a spin in a stochastic field environment. Our
model is based on ``strong collisions''. We examine in detail three cases
where: (I) the local field is Ising-like, (II) the field distribution is
continuous and has a finite second moment, and (III) the distribution is
Lorentzian. The first two cases show a T2 minimum effect and are exponential in
time cubed for short times. The last case can be approximated by a
phenomenological stretched exponential.Comment: 11 pages + 3 postscript figure
Muon spin rotation study of the magnetic penetration depth in the intercalated graphite superconductor CaC6
We report temperature- and magnetic field-dependent bulk muon spin rotation
measurements in a c-axis oriented superconductor CaC6 in the mixed state. Using
both a simple second moment analysis and the more precise analytical
Ginzburg-Landau model, we obtained a field independent in-plane magnetic
penetration depth {\lambda}ab (0) = 72(3) nm. The temperature dependencies of
the normalized muon spin relaxation rate and of the normalized superfluid
density result to be identical, and both are well represented by the clean
limit BCS model with 2\Delta/kB Tc = 3.6(1), suggesting that CaC6 is a fully
gapped BCS superconductor in the clean limit regime.Comment: Accepted for publication in PR
Evolution from a nodeless gap to d(x2-y2) form in underdoped La(2-x)SrxCuO4
Using angle-resolved photoemission (ARPES), it is revealed that the
low-energy electronic excitation spectra of highly underdoped superconducting
and non-superconducting La(2-x)SrxCuO4 cuprates are gapped along the entire
underlying Fermi surface at low temperatures. We show how the gap function
evolves to a d(x2-y2) form as increasing temperature or doping, consistent with
the vast majority of ARPES studies of cuprates. Our results provide essential
information for uncovering the symmetry of the order parameter(s) in strongly
underdoped cuprates, which is a prerequisite for understanding the pairing
mechanism and how superconductivity emerges from a Mott insulator.Comment: 5 pages, 4 figure
Magnetic frustration in a stoichiometric spin-chain compound, CaCoIrO
The temperature dependent ac and dc magnetization and heat capacity data of
CaCoIrO, a spin-chain compound crystallizing in a KCdCl-derived
rhombohedral structure, show the features due to magnetic ordering of a
frustrated-type below about 30 K, however without exhibiting the signatures of
the so-called "partially disordered antiferromagnetic structure" encountered in
the isostructural compounds, CaCoO and CaCoRhO. This class
of compounds thus provides a variety for probing the consequences of magnetic
frustration due to topological reasons in stoichiometric spin-chain materials,
presumably arising from subtle differences in the interchain and intrachain
magnetic coupling strengths. This compound presents additional interesting
situations in the sense that, ac susceptibility exhibits a large frequency
dependence in the vicinity of 30 K uncharacteristic of conventional
spin-glasses, with this frustrated magnetic state being robust to the
application of external magnetic fields.Comment: Physical Review (Rapid Communications), in pres
Ultrafast optical nonlinearity in quasi-one-dimensional Mott-insulator
We report strong instantaneous photoinduced absorption (PA) in the
quasi-one-dimensional Mott insulator in the IR spectral
region. The observed PA is to an even-parity two-photon state that occurs
immediately above the absorption edge. Theoretical calculations based on a
two-band extended Hubbard model explains the experimental features and
indicates that the strong two-photon absorption is due to a very large
dipole-coupling between nearly degenerate one- and two-photon states. Room
temperature picosecond recovery of the optical transparency suggests the strong
potential of for all-optical switching.Comment: 10 pages, 4 figure
The temporal representation of experience in subjective mood
Humans refer to their mood state regularly in day-to-day as well as clinical interactions. Theoretical accounts suggest that when reporting on our mood we integrate over the history of our experiences; yet, the temporal structure of this integration remains unexamined. Here, we use a computational approach to quantitatively answer this question and show that early events exert a stronger influence on reported mood (a primacy weighting) compared to recent events. We show that a Primacy model accounts better for mood reports compared to a range of alternative temporal representations across random, consistent, or dynamic reward environments, different age groups, and in both healthy and depressed participants. Moreover, we find evidence for neural encoding of the Primacy, but not the Recency, model in frontal brain regions related to mood regulation. These findings hold implications for the timing of events in experimental or clinical settings and suggest new directions for individualized mood interventions
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