257 research outputs found
Landau-Ginzburg-Devonshire theory for electromechanical hysteresis loop formation in piezoresponse force microscopy of thin films
Electromechanical hysteresis loop formation in piezoresponse force microscopy
of thin ferroelectric films is studied with special emphasis on the effects of
tip size and film thickness, as well as dependence on the tip voltage
frequency. Here, we use a combination of Landau-Ginzburg-Devonshire (LGD)
theory for the description of the local polarization reversal with decoupling
approximation for the calculation of the local piezoresponse loops shape,
coercive voltages and amplitude. LGD approach enables addressing both
thermodynamics and kinetics of hysteresis loop formation. In contrast to the
"rigid" ferroelectric approximation, this approach allows for the piezoelectric
tensor components dependence on the ferroelectric polarization and dielectric
permittivity. This model rationalizes the non-classical shape of the dynamic
piezoelectric force microscopy (PFM) loops.Comment: 23 pages, 5 figures, 1 appendix,to be submitted to J. Appl. Phy
Magnetic Moment Softening and Domain Wall Resistance in Ni Nanowires
Magnetic moments in atomic scale domain walls formed in nanoconstrictions and
nanowires are softened which affects dramatically the domain wall resistance.
We perform ab initio calculations of the electronic structure and conductance
of atomic-size Ni nanowires with domain walls only a few atomic lattice
constants wide. We show that the hybridization between noncollinear spin states
leads to a reduction of the magnetic moments in the domain wall. This magnetic
moment softening strongly enhances the domain wall resistance due to scattering
produced by the local perturbation of the electronic potential.Comment: 4 pages, 5 figure
Thermodynamics of nanodomain formation and breakdown in Scanning Probe Microscopy: Landau-Ginzburg-Devonshire approach
Thermodynamics of tip-induced nanodomain formation in scanning probe
microscopy of ferroelectric films and crystals is studied using the
Landau-Ginzburg-Devonshire phenomenological approach. The local redistribution
of polarization induced by the biased probe apex is analyzed including the
effects of polarization gradients, field dependence of dielectric properties,
intrinsic domain wall width, and film thickness. The polarization distribution
inside subcritical nucleus of the domain preceding the nucleation event is very
smooth and localized below the probe, and the electrostatic field distribution
is dominated by the tip. In contrast, polarization distribution inside the
stable domain is rectangular-like, and the associated electrostatic fields
clearly illustrate the presence of tip-induced and depolarization field
components. The calculated coercive biases of domain formation are in a good
agreement with available experimental results for typical ferroelectric
materials. The microscopic origin of the observed domain tip elongation in the
region where the probe electric field is much smaller than the intrinsic
coercive field is the positive depolarization field in front of the moving
counter domain wall. For infinitely thin domain walls local domain breakdown
through the sample depth appears. The results obtained here are complementary
to the Landauer-Molotskii energetic approach.Comment: 35 pages, 8 figures, suplementary attached, to be submitted to Phys.
Rev.
Domain wall conduction in multiaxial ferroelectrics
The conductance of domain wall structures consisting of either stripes or
cylindrical domains in multi-axial ferroelectric-semiconductors is analyzed.
The effects of the domain size, wall tilt and curvature, on charge
accumulation, are analyzed using the Landau-Ginsburg Devonshire (LGD) theory
for polarization combined with Poisson equation for charge distributions. Both
the classical ferroelectric parameters including expansion coefficients in
2-4-6 Landau potential and gradient terms, as well as flexoelectric coupling,
inhomogeneous elastic strains and electrostriction are included in the present
analysis. Spatial distributions of the ionized donors, free electrons and holes
were found self-consistently using the effective mass approximation for the
respective densities of states. The proximity and size effect of the electron
and donor accumulation/depletion by thin stripe domains and cylindrical
nanodomains are revealed. In contrast to thick domain stripes and thicker
cylindrical domains, in which the carrier accumulation (and so the static
conductivity) sharply increases at the domain walls only, small nanodomains of
radius less then 5-10 correlation length appeared conducting across entire
cross-section. Implications of such conductive nanosized channels may be
promising for nanoelectronics.Comment: 39 pages, 11 figures, 3 tables, 4 appendice
Electron Spin for Classical Information Processing: A Brief Survey of Spin-Based Logic Devices, Gates and Circuits
In electronics, information has been traditionally stored, processed and
communicated using an electron's charge. This paradigm is increasingly turning
out to be energy-inefficient, because movement of charge within an
information-processing device invariably causes current flow and an associated
dissipation. Replacing charge with the "spin" of an electron to encode
information may eliminate much of this dissipation and lead to more
energy-efficient "green electronics". This realization has spurred significant
research in spintronic devices and circuits where spin either directly acts as
the physical variable for hosting information or augments the role of charge.
In this review article, we discuss and elucidate some of these ideas, and
highlight their strengths and weaknesses. Many of them can potentially reduce
energy dissipation significantly, but unfortunately are error-prone and
unreliable. Moreover, there are serious obstacles to their technological
implementation that may be difficult to overcome in the near term.
This review addresses three constructs: (1) single devices or binary switches
that can be constituents of Boolean logic gates for digital information
processing, (2) complete gates that are capable of performing specific Boolean
logic operations, and (3) combinational circuits or architectures (equivalent
to many gates working in unison) that are capable of performing universal
computation.Comment: Topical Revie
Mutations in the NS1 C-terminal tail do not enhance replication or virulence of the 2009 pandemic H1N1 influenza A virus
The ‘classical’ swine H1N1 influenza A virus lineage was established after the devastating 1918 human pandemic virus entered domestic pig herds. A descendent of this lineage recently re-emerged in humans as the 2009 pandemic H1N1 virus. Adaptation in pigs has led to several changes in the multifunctional viral NS1 protein as compared with the parental 1918 virus, most notably a K217E substitution that abolishes binding to host Crk/CrkL signalling adapters, and an 11 aa C-terminal truncation. Using reverse genetics, we reintroduced both these features into a prototype 2009 H1N1 strain, A/California/04/09. Restoration of Crk/CrkL binding or extension of NS1 to 230 aa had no impact on virus replication in human or swine cells. In addition, minimal effects on replication, pathogenicity and transmission were observed in mouse and ferret models. Our data suggest that the currently circulating 2009 H1N1 virus is optimized to replicate efficiently without requiring certain NS1 functions
Application of elastostatic Green function tensor technique to electrostriction in cubic, hexagonal and orthorhombic crystals
The elastostatic Green function tensor approach, which was recently used to
treat electrostriction in numerical simulation of domain structure formation in
cubic ferroelectrics, is reviewed and extended to the crystals of hexagonal and
orthorhombic symmetry. The tensorial kernels appearing in the expressions for
effective nonlocal interaction of electrostrictive origin are derived
explicitly and their physical meaning is illustrated on simple examples. It is
argued that the bilinear coupling between the polarization gradients and
elastic strain should be systematically included in the Ginzburg-Landau free
energy expansion of electrostrictive materials.Comment: 4 page
First-principles investigation of 180-degree domain walls in BaTiO_3
We present a first-principles study of 180-degree ferroelectric domain walls
in tetragonal barium titanate. The theory is based on an effective Hamiltonian
that has previously been determined from first-principles
ultrasoft-pseudopotential calculations. Statistical properties are investigated
using Monte Carlo simulations. We compute the domain-wall energy, free energy,
and thickness, analyze the behavior of the ferroelectric order parameter in the
interior of the domain wall, and study its spatial fluctuations. An abrupt
reversal of the polarization is found, unlike the gradual rotation typical of
the ferromagnetic case.Comment: Revtex (preprint style, 13 pages) + 3 postscript figures. A version
in two-column article style with embedded figures is available at
http://electron.rutgers.edu/~dhv/preprints/index.html#pad_wal
"Head-to-head" and "tail-to-tail" 180-degree domain walls in an isolated ferroelectric
"Head-to-head" and "tail-to-tail" 180-degree domain-walls in a finite
isolated ferroelectric sample are theoretically studied using Landau theory.
The full set of equations, suitable for numerical calculations is developed.
The explicit expressions for the polarization profile across the walls are
derived for several limiting cases and wall-widths are estimated. It is shown
analytically that different regimes of screening and different dependences for
width of charged domain walls on the temperature and parameters of the system
are possible, depending on spontaneous polarization and concentration of
carriers in the material. It is shown that the half-width of charged domain
walls in typical perovskites is about the nonlinear Thomas-Fermi
screening-length and about one order of magnitude larger than the half-width of
neutral domain-walls. The formation energies of "head-to-head" walls under
different regimes of screening are obtained, neglecting the poling ability of
the surface. It is shown that either "head-to-head" or "tail-to-tail"
configuration can be energetically favorable in comparison with the monodomain
state of the ferroelectric if the poling ability of the surface is large
enough. If this is not the case, the existence of charged domain walls in bulk
ferroelectrics is merely a result of the domain-growth kinetics. Size-effect
corresponding to the competition between state with charged domain wall, single
domain state, multidomain state, and the state with the zero polarization is
considered. The results obtained for the case of an isolated ferroelectric
sample were compared with the results for an electroded sample. It was shown
that charged domain wall in electroded sample can be either metastable or
stable, depends on the work function difference between electrodes and
ferroelectric and the poling ability of the electrode/ferroelectric interface.Comment: 47 pages, 10 figure
Er:Yb phosphate glass laser with nonlinear absorber for phase-sensitive optical time domain reflectometry
A novel laser for phase-sensitive optical time-domain reflectometry (Φ-OTDR) is presented. The advantages of a compact solid-state laser are listed, current problems are shown. Experiments with a microchip single-optical-element laser, from setup construction to usage in Φ-OTDR system, are presented. New laser scheme with two-photon intracavity absorber is suggested and its advantages are described
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