Electron Confinement, Orbital Ordering, and Orbital Moments in d0d^0-d1d^1 Oxide Heterostructures

The (SrTiO$_3$)$_m$/(SrVO$_3$)$_n$ $d^0-d^1$ multilayer system is studied with first principles methods through the observed insulator-to-metal transition with increasing thickness of the SrVO$_3$ layer. When correlation effects with reasonable magnitude are included, crystal field splittings from the structural relaxations together with spin-orbit coupling (SOC) determines the behavior of the electronic and magnetic structures. These confined slabs of SrVO$_3$ prefer $Q_{orb}$=($\pi,\pi$) orbital ordering of $\ell_z = 0$ and $\ell_z = -1$ ($j_z=-1/2$) orbitals within the plane, accompanied by $Q_{spin}$=(0,0) spin order (ferromagnetic alignment). The result is a SOC-driven ferromagnetic Mott insulator. The orbital moment of 0.75 $\mu_B$ strongly compensates the spin moment on the $\ell_z = -1$ sublattice. The insulator-metal transition for $n = 1 \to 5$ (occurring between $n$=4 and $n$=5) is reproduced. Unlike in the isoelectronic $d^0-d^1$ TiO$_2$/VO$_2$ (rutile structure) system and in spite of some similarities in orbital ordering, no semi-Dirac point [{\it Phys. Rev. Lett.} {\bf 102}, 166803 (2009)] is encountered, but the insulator-to-metal transition occurs through a different type of unusual phase. For n=5 this system is very near (or at) a unique semimetallic state in which the Fermi energy is topologically determined and the Fermi surface consists of identical electron and hole Fermi circles centered at $k$=0. The dispersion consists of what can be regarded as a continuum of radially-directed Dirac points, forming a "Dirac circle".Comment: 9 pages, 8 figure

Statistics on Graphs, Exponential Formula and Combinatorial Physics

The concern of this paper is a famous combinatorial formula known under the name "exponential formula". It occurs quite naturally in many contexts (physics, mathematics, computer science). Roughly speaking, it expresses that the exponential generating function of a whole structure is equal to the exponential of those of connected substructures. Keeping this descriptive statement as a guideline, we develop a general framework to handle many different situations in which the exponential formula can be applied

Reversible strain effect on the magnetization of LaCoO3 films

The magnetization of ferromagnetic LaCoO3 films grown epitaxially on piezoelectric substrates has been found to systematically decrease with the reduction of tensile strain. The magnetization change induced by the reversible strain variation reveals an increase of the Co magnetic moment with tensile strain. The biaxial strain dependence of the Curie temperature is estimated to be below 4K/% in the as-grown tensile strain state of our films. This is in agreement with results from statically strained films on various substrates

High Energy Positrons From Annihilating Dark Matter

Recent preliminary results from the PAMELA experiment indicate the presence of an excess of cosmic ray positrons above 10 GeV. In this letter, we consider possibility that this signal is the result of dark matter annihilations taking place in the halo of the Milky Way. Rather than focusing on a specific particle physics model, we take a phenomenological approach and consider a variety of masses and two-body annihilation modes, including W+W-, ZZ, b bbar, tau+ tau-, mu+ mu-, and e+e. We also consider a range of diffusion parameters consistent with current cosmic ray data. We find that a significant upturn in the positron fraction above 10 GeV is compatible with a wide range of dark matter annihilation modes, although very large annihilation cross sections and/or boost factors arising from inhomogeneities in the local dark matter distribution are required to produce the observed intensity of the signal. We comment on constraints from gamma rays, synchrotron emission, and cosmic ray antiproton measurements.Comment: 4 pages, 1 figur

The Case for a 700+ GeV WIMP: Cosmic Ray Spectra from PAMELA, Fermi and ATIC

Multiple lines of evidence indicate an anomalous injection of high-energy e+- in the Galactic halo. The recent $e^+$ fraction spectrum from the Payload for Antimatter Matter Exploration and Light-nuclei Astrophysics (PAMELA) shows a sharp rise up to 100 GeV. The Fermi Gamma-ray Space Telescope has found a significant hardening of the e+e- cosmic ray spectrum above 100 GeV, with a break, confirmed by HESS at around 1 TeV. The Advanced Thin Ionization Calorimeter (ATIC) has also detected detected a similar excess, falling back to the expected spectrum at 1 TeV and above. Excess microwaves towards the galactic center in the WMAP data are consistent with hard synchrotron radiation from a population of 10-100 GeV e+- (the WMAP ``Haze''). We argue that dark matter annihilations can provide a consistent explanation of all of these data, focusing on dominantly leptonic modes, either directly or through a new light boson. Normalizing the signal to the highest energy evidence (Fermi and HESS), we find that similar cross sections provide good fits to PAMELA and the Haze, and that both the required cross section and annihilation modes are achievable in models with Sommerfeld-enhanced annihilation. These models naturally predict significant production of gamma rays in the galactic center via a variety of mechanisms. Most notably, there is a robust inverse-Compton scattered (ICS) gamma-ray signal arising from the energetic electrons and positrons, detectable at Fermi/GLAST energies, which should provide smoking gun evidence for this production.Comment: 28 pages; v2 plots corrected, references added; v3 included Fermi electron data at reviewer request, references adde

Research for preparation of cation-conducting solids by high-pressure synthesis and other methods

It was shown that two body-centered-cubic skeleton structures, the Im3 KSbO3 phase and the defect-pyrochlore phase A(+)B2X6, do exhibit fast Na(+)-ion transport. The placement of anions at the tunnel intersection sites does not impede Na(+)-ion transport in (NaSb)3)(1/6 NaF), and may not in (Na(1+2x)Ta2 5F)(Ox). The activation energies are higher than those found in beta-alumina. There are two possible explanations for the higher activation energy: breathing of the bottleneck (site face or edge) through which the A(+) ions must pass on jumping from one site to another may be easier in a layer structure and/or A(+)-O bonding may be stronger in the cubic structures because the O(2-) ion bonds with two (instead of three) cations of the skeleton. If the former explanation is dominant, a lower activation energy may be achieved by optimizing the lattice parameter. If the latter is dominant, a new structural principle may have to be explored

First principles investigation of the electronic structure of La2MnNiO6: A room-temperature insulating ferromagnet

Using first principles calculations within DFT based on the full potential APW+lo method, we calculated the electronic and magnetic structures for the ferromagnetic and antiferromagnetic states of La2MnNiO6 and analyzed the site projected density of states and electronic band structures. Our calculations show that the ground state of La2MnNiO6 is ferromagnetic insulating with the magnetization in agreement with Hund's first rule and experimental findings.Comment: 10 pages, 3 figure

Rational Hadamard products via Quantum Diagonal Operators

We use the remark that, through Bargmann-Fock representation, diagonal operators of the Heisenberg-Weyl algebra are scalars for the Hadamard product to give some properties (like the stability of periodic fonctions) of the Hadamard product by a rational fraction. In particular, we provide through this way explicit formulas for the multiplication table of the Hadamard product in the algebra of rational functions in \C[[z]]

The structure and petrology of the Cnoc nan Cuilean Intrusion, Loch Loyal Syenite Complex, NW Scotland

In NW Scotland, several alkaline intrusive complexes of Silurian age intrude the Caledonian orogenic front. The most northerly is the Loch Loyal Syenite Complex, which is divided into three separate intrusions (Ben Loyal, Beinn Stumanadh and Cnoc nan Cuilean). Mapping of the Cnoc nan Cuilean intrusion shows two main zones: a Mixed Syenite Zone (MZ) and a Massive Leucosyenite Zone (LZ), with a gradational contact. The MZ forms a lopolith, with multiple syenitic lithologies, including early basic melasyenites and later felsic leucosyenites. Leucosyenite melts mixed and mingled with melasyenites, resulting in extreme heterogeneity within the MZ. Continued felsic magmatism resulted in formation of the relatively homogeneous LZ, invading western parts of the MZ and now forming the topographically highest terrane. The identification of pegmatites, microgranitic veins and unusual biotite-magnetite veins demonstrates the intrusion's complex petrogenesis. Cross-sections have been used to create a novel 3D GoCad™ model contributing to our understanding of the intrusion. The Loch Loyal Syenite Complex is known to have relatively high concentrations of rare earth elements (REEs), and thus the area has potential economic and strategic value. At Cnoc nan Cuilean, abundant REE-bearing allanite is present within melasyenites of the MZ. Extensive hydrothermal alteration of melasyenites here formed steeply dipping biotite-magnetite veins, most enriched in allanite and other REE-bearing accessories. This study has thus identified the area of greatest importance for further study of REE enrichment processes in the Cnoc nan Cuilean intrusion

Magnetic ground state and 2D behavior in pseudo-Kagome layered system Cu3Bi(SeO3)2O2Br

Anisotropic magnetic properties of a layered kagome-like system Cu3Bi(SeO3)2O2Br have been studied by bulk magnetization and magnetic susceptibility measurements as well as powder and single-crystal neutron diffraction. At T_N = 27.4 K the system develops an alternating antiferromagnetic order of (ab) layers, which individually exhibit canted ferrimagnetic moment arrangement, resulting from the competing ferro- and antiferro-magnetic intralayer exchange interactions. A magnetic field B_C ~ 0.8 T applied along the c axis (perpendicular to the layers) triggers a metamagnetic transition, when every second layer flips, i.e., resulting in a ferrimagnetic structure. Significantly higher fields are required to rotate the ferromagnetic component towards the b axis (~7 T) or towards the a axis (~15 T). The estimates of the exchange coupling constants and features indicative of an XY character of this quasi-2D system are presented.Comment: 7 pages, 6 figures, final versio