366 research outputs found
Charge carrier density collapse in La_0.67Ca_0.33MnO_3 and La_0.67Sr_0.33MnO_3 epitaxial thin films
We measured the temperature dependence of the linear high field Hall
resistivity of La_0.67Ca_0.33MnO_3 (T_C=232K) and La_0.67Sr_0.33MnO_3
(T_C=345K) thin films in the temperature range from 4K up to 360K in magnetic
fields up to 20T. At low temperatures we find a charge carrier density of 1.3
and 1.4 holes per unit cell for the Ca- and Sr-doped compound, respectively. In
this temperature range electron-magnon scattering contributes to the
longitudinal resistivity. At the ferromagnetic transition temperature T_C a
dramatic drop in the number of current carriers down to 0.6 holes per unit
cell, accompanied by an increase in unit cell volume, is observed. Corrections
of the Hall data due to a non saturated magnetic state will lead a more
pronounced charge carrier density collapse.Comment: 5 pages, 5 EPS figures, submitted to Eur. Phys. J.
Disorder-induced melting of the charge order in thin films of Pr0.5Ca0.5MnO3
We have studied the magnetic-field-induced melting of the charge order in
thin films of Pr0.5Ca0.5MnO3 (PCMO) films on SrTiO3 (STO) by X-ray diffraction,
magnetization and transport measurement. At small thickness (25 nm) the films
are under tensile strain and the low-temperature melting fields are of the
order of 20 T or more, comparable to the bulk value. With increasing film
thickness the strain relaxes, which leads to a strong decrease of the melting
fields. For a film of 150 nm, with in-plane and out-of-plane lattice parameters
closer to the bulk value, the melting field has reduced to 4 T at 50 K, with a
strong increase in the hysteretic behavior and also an increasing fraction of
ferromagnetic material. Strain relaxation by growth on a template of
YBa2Cu3O(7-delta) or by post-annealing yields similar results with an even
stronger reduction of the melting field. Apparently, strained films behave
bulk-like. Relaxation leads to increasing suppression of the CO state,
presumably due to atomic scale disorder produced by the relaxation process.Comment: 7 pages, 4 fig
Extensive infrared spectroscopic study of CuO: signatures of strong spin-phonon interaction and structural distortion
Optical properties of single-crystal monoclinic CuO in the range 70 - 6000
\cm were studied at temperatures from 7 to 300 K. Normal reflection spectra
were obtained from the (001) and (010) crystal faces thus giving for the first
time separate data for the and phonon modes excited in the
purely transverse way (TO modes). Mode parameters, including polarizations of
the modes not determined by the crystal symmetry, were extracted by the
dispersion analysis of reflectivity curves as a function of temperature.
Spectra of all the components of the optical conductivity tensor were obtained
using the Kramers-Kronig method recently extended to the case of the
low-symmetry crystals. The number of strong phonon modes is in agreement with
the factor-group analysis for the crystal structure, currently accepted for the
CuO. However, several "extra" modes of minor intensity are detected. Comparison
of frequencies of "extra" modes with the available phonon dispersion curves
points to possible "diagonal" doubling of the unit cell \{{\bf a}, {\bf b},
{\bf c}\} \{{\bf a}+{\bf c}, {\bf b}, {\bf a}-{\bf c}\} and formation of
the superlattice. The previously reported softening of the mode
( 400 \cm) with cooling at is found to be 10 % for the TO
mode. The mode is very broad at high temperatures and strongly narrows in the
AFM phase. We attribute this effect to strong resonance coupling of this mode
to optical or acoustic bi-magnons and reconstruction of the magnetic
excitations spectrum at the N\'eel point. A significant anisotropy of
is observed: it was found to be 5.9 along the {\bf b}-axis,
6.2 along the {[}101{]} chains and 7.8 the {[}10{]} chains. The
"transverse" effective charge is value is about 2 electrons.Comment: 23 pages, 14 figures, REVTeX, submitted to PR
Infrared studies of a La_(0.67)Ca_(0.33)MnO_3 single crystal: Optical magnetoconductivity in a half-metallic ferromagnet
The infrared reflectivity of a La_(0.67)Ca_(0.33)MnO_3 single crystal is studied over a broad range of temperatures (78–340 K), magnetic fields (0–16 T), and wave numbers (20–9000cm^(-1)). The optical conductivity gradually changes from a Drude-like behavior to a broad peak feature near 5000cm-1 in the ferromagnetic state below the Curie temperature T_C=307K. Various features of the optical conductivity bear striking resemblance to recent theoretical predictions based on the interplay between the double exchange interaction and the Jahn-Teller electron-phonon coupling. A large optical magnetoconductivity is observed near T_C
Infrared Studies of a La_{0.67}Ca_{0.33}MnO_3 Single Crystal: Optical Magnetoconductivity in a Half-Metallic Ferromagnet
The infrared reflectivity of a single crystal
is studied over a broad range of temperatures (78-340 K), magnetic fields (0-16
T), and wavenumbers (20-9000 cm). The optical conductivity gradually
changes from a Drude-like behavior to a broad peak feature near 5000 cm
in the ferromagnetic state below the Curie temperature . Various
features of the optical conductivity bear striking resemblance to recent
theoretical predictions based on the interplay between the double exchange
interaction and the Jahn-Teller electron-phonon coupling. A large optical
magnetoconductivity is observed near .Comment: 4 pages, 4 figures, Latex, PostScript; The 7th Joint MMM-Intermag
Conference,San Francisco, January 6-9, 1998; The Int. Conf. on Strongly
Correlated Electron Systems, Paris, July 15-18,199
Treatment of Intrusive Suicidal Imagery Using Eye Movements
Suicide and suicidal behavior are major public health concerns, and affect 3–9% of the population worldwide. Despite increased efforts for national suicide prevention strategies, there are still few effective interventions available for reducing suicide risk. In this article, we describe various theoretical approaches for suicide ideation and behavior, and propose to examine the possible effectiveness of a new and innovative preventive strategy. A model of suicidal intrusion (mental imagery related to suicide, also referred to as suicidal flash-forwards) is presented describing one of the assumed mechanisms in the etiology of suicide and the mechanism of therapeutic change. We provide a brief rationale for an Eye Movement Dual Task (EMDT) treatment for suicidal intrusions, describing techniques that can be used to target these suicidal mental images and thoughts to reduce overall behavior. Based on the available empirical evidence for the mechanisms of suicidal intrusions, this approach appears to be a promising new treatment to prevent suicidal behavior as it potentially targets one of the linking pins between suicidal ideation and suicidal actions
The anomaly of the oxygen bond-bending mode at 320 cm and the additional absorption peak in the c-axis infrared conductivity of underdoped YBaCuO single crystals revisited by ellipsometricmeasurements
We have performed ellipsometric measurements of the far-infrared c-axis
dielectric response of underdoped YBaCuO single
crystals. Here we report a detailed analysis of the temperature-dependent
renormalization of the oxygen bending phonon mode at 320 cm and the
formation of the additional absorption peak around 400-500 cm. For a
strongly underdoped YBaCuO crystal with T=52 K we
find that, in agreement with previous reports based on conventional reflection
measurements, the gradual onset of both features occurs well above T at
T*150 K. Contrary to some of these reports, however, our data establish
that the phonon anomaly and the formation of the additional peak exhibit very
pronounced and steep changes right at T. For a less underdoped
YBaCuO crystal with T=80 K, the onset temperature of
the phonon anomaly almost coincides with T. Also in contrast to some
previous reports, we find for both crystals that a sizeable fraction of the
spectral weight of the additional absorption peak cannot be accounted for by
the spectral-weight loss of the phonon modes but instead arises from a
redistribution of the electronic continuum. Our ellipsometric data are
consistent with a model where the bilayer cuprate compounds are treated as a
superlattice of intra- and inter-bilayer Josephson-junctions
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