NOVEL COMPACT NARROW-LINEWIDTH MID-INFRARED LASERS FOR SENSING APPLICATIONS

The mid-infrared (2-14 μm) spectral region contains the strong absorption lines of many important molecular species, which make this region crucial for several well-know applications such as spectroscopy, chemical and biochemical sensing, security, and industrial monitoring. To fully exploit this region through absorption spectroscopic techniques, compact and low-cost narrow-linewidth (NLW) mid-infrared (MIR) laser sources are of primary importance. This thesis is focused on three novel compact NLW MIR lasers: demonstration and characterization of a new glass-based spherical microlaser, investigation of the performance of a novel fiber laser, and the design of a monolithic laser on a silicon chip. Starting with fabrication of spherical microcavities based on MIR transparent materials, I showed the feasibility of achieving quality factors of more than 10 million in whispering- gallery mode (WGM) microresonators made of different types of fluoride glasses. Next using Erbium doped ZBLAN glass spherical microresonators, I demonstrated a new ultra- low threshold NLW MIR microlaser. In particular, all aspects of this room temperature continuous-wave (CW) microlaser with a wavelength of 2.71 μm are carefully characterized and studied and the origin of the measured mode structure and polarization is described using a simple analysis. To amplify the output power of this laser, I designed and fabricated a MIR fiber amplifier with a record gain of about 30 dB at 2.71 μm that facilitated the characterization process and boosted the MIR power level to usable level while preserving the laser linewidth. To demonstrate the application of MIR microresonators and microlasers, I studied intracavity absorption spectroscopy based on active and passive high quality WGM MIR microlasers and microresonators. I also estimated the sensitivity and detection limit of gas sensors based on these devices. The outcome of my analysis shows that ppm level sensitivity should be achievable using both active and passive microresonators. Next, I modeled the performance of two newly proposed configurations for NLW MIR generation based on stimulated Raman scattering. First, I studied a new family of Raman fiber lasers that are capable of generating any NLW MIR line in the 2.5-9.5 μm spectral region. I demonstrated the feasibility of this MIR laser family, calculated the threshold conditions, identified the condition for its single-mode operation, and laid the foundation for the first experimental demonstration of such lasers. Finally, I explored the performance of silicon-based on-chip Raman lasers and the parameters that have prevented expanding their wavelength to MIR range. Using the outcomes of this study, I proposed and then analyzed a new architecture for on-chip silicon Raman lasers capable of generating single NLW lines around 3.2 μm with sub-mW threshold pump power

Photonic Jet: Science and Application

Photonic jets (PJs) are important mesoscale optical phenomena arising from electromagnetic waves interacting with dielectric particles. PJs have applications in super-resolution imaging, sensing, detection, patterning, trapping, manipulation, waveguiding, signal amplification and high-efficiency signal collection, among others. This reprint provides an overview of the field and highlights recent advances and trends in PJ research

Glassy Materials Based Microdevices

Microtechnology has changed our world since the last century, when silicon microelectronics revolutionized sensor, control and communication areas, with applications extending from domotics to automotive, and from security to biomedicine. The present century, however, is also seeing an accelerating pace of innovation in glassy materials; as an example, glass-ceramics, which successfully combine the properties of an amorphous matrix with those of micro- or nano-crystals, offer a very high flexibility of design to chemists, physicists and engineers, who can conceive and implement advanced microdevices. In a very similar way, the synthesis of glassy polymers in a very wide range of chemical structures offers unprecedented potential of applications. The contemporary availability of microfabrication technologies, such as direct laser writing or 3D printing, which add to the most common processes (deposition, lithography and etching), facilitates the development of novel or advanced microdevices based on glassy materials. Biochemical and biomedical sensors, especially with the lab-on-a-chip target, are one of the most evident proofs of the success of this material platform. Other applications have also emerged in environment, food, and chemical industries. The present Special Issue of Micromachines aims at reviewing the current state-of-the-art and presenting perspectives of further development. Contributions related to the technologies, glassy materials, design and fabrication processes, characterization, and, eventually, applications are welcome

Spectroscopic study of optical confinement and transport effects in coupled microspheres and pillar cavities

In this thesis we investigated the spatial and spectral mode profiles, and the optical transport properties of single and multiple coupled cavities. We performed numerical modeling of whispering gallery modes (WGMs) in such cavities in order to explain recent experiments on semiconductor micropillars. High quality (Q up to 20 000) WGMs with small mode volumes V ~0.3 µm3 in 4-5 µm micropillars were reproduced. The WGM spectra were found to be in a good agreement with the experimental data. The coupling between size-matched spheres from 2.9 to 6.0 µm in diameter was characterized using spectroscopy. We observed peculiar kites in the spectral images of such coherently coupled bispheres. The origin of these kites was explained due to the coupling of multiple pairs of azimuthal modes. We quantified the coupling constant for WGMs located in the equatorial plane of spheres parallel to the substrate which plays the most important role in the transport of WGMs in such structures. It was shown that in long (>10 spheres) chains of size-disordered polystyrene microspheres the transmission properties are dominated by photonic nanojet-induced modes (NIMs) leading to periodic focusing of light along the chain. In the transmission spectra of such chains we observed Fabry-Pe´rot fringes with propagation losses of only 0.08 dB per sphere at the maxima of the transmission peaks. The fringes of NIMs are found to be in a good agreement with the results of numerical modeling. These modes can be used in various biomedical applications requiring tight focusing of the beams

Tuning the effective coupling of an AFM lever to a thermal bath

Fabrication of Nano-Electro-Mechanical-Systems (NEMS) of high quality is nowadays extremely efficient. These NEMS will be used as sensors and actuators in integrated systems. Their use however raises questions about their interface (actuation, detection, read out) with external detection and control systems. Their operation implies many fundamental questions related to single particle effects such as Coulomb blockade, light matter interactions such as radiation pressure, thermal effects, Casimir forces and the coupling of nanosystems to external world (thermal fluctuations, back action effect). Here we specifically present how the damping of an oscillating cantilever can be tuned in two radically different ways: i) through an electro-mechanical coupling in the presence of a strong Johnson noise, ii) through an external feedback control of thermal fluctuations which is the cold damping closely related to Maxwell's demon. This shows how the interplay between MEMS or NEMS external control and their coupling to a thermal bath can lead to a wealth of effects that are nowadays extensively studied in different areas

Towards quantum computing with single atoms and optical cavities on atom chips

We report on recent developments in the integration of optical microresonators into atom chips and describe some fabrication and implementation challenges. We also review theoretical proposals for quantum computing with single atoms based on the observation of photons leaking through the cavity mirrors. The use of measurements to generate entanglement can result in simpler, more robust and scalable quantum computing architectures. Indeed, we show that quantum computing with atom-cavity systems is feasible even in the presence of relatively large spontaneous decay rates and finite photon detector efficiencies.Comment: 14 pages, 6 figure